与核热能相结合的纸浆和造纸工业碳捕获和储存的成本分析

Edgar Carrejo , Jhonny Alejandro Poveda-Giraldo , Sam J. Root , Nahuel Guaita , Elizabeth Worsham , Sunkyu Park
{"title":"与核热能相结合的纸浆和造纸工业碳捕获和储存的成本分析","authors":"Edgar Carrejo ,&nbsp;Jhonny Alejandro Poveda-Giraldo ,&nbsp;Sam J. Root ,&nbsp;Nahuel Guaita ,&nbsp;Elizabeth Worsham ,&nbsp;Sunkyu Park","doi":"10.1016/j.ccst.2025.100468","DOIUrl":null,"url":null,"abstract":"<div><div>The pulp and paper industry generates approximately 150 million tons of CO<sub>2</sub> emissions annually, ranking among the top three industry sectors in terms of CO<sub>2</sub> emissions in the United States, when biogenic CO<sub>2</sub> is included, followed by the chemical and petroleum industries. Carbon Capture and Storage (CCS) technologies can be implemented to decrease these emissions; however, mature CCS technologies such as amine-based capture are energy-intensive. Nuclear energy can provide this energy to CCS operations without producing point source emissions. This study evaluates the economic feasibility of integrating a Small Modular Nuclear Reactor (SMNR) to power an amine-based CCS technology in three types of pulp and paper mills in the southeast of the United States: a bleached softwood kraft mill, an unbleached softwood kraft mill, and a recycling mill with an assumption of an annual production capacity of 500,000 metric tons. The presented scenarios compare the carbon capture potential and costs of a CCS system for these mills when integrated with heat from either a nuclear reactor or a natural gas boiler. Two 200 MW-thermal (MW<sub>th</sub>) small modular reactors were found to be sufficient to cover the demand for steam and power for coupling CCS and decommissioning the natural gas boiler in the bleached softwood kraft mill, while one 200 MW<sub>th</sub> SMNR module was sufficient for the other mill types. Nuclear heat integration into a CCS system, coupled with a typical kraft paper mill, can decrease CO<sub>2</sub> emissions by 91 % with the remaining 9 % being primarily biogenic. Accordingly, recycling mills powered by nuclear energy can achieve almost zero emissions. In the nuclear heat integration scenarios, the CO<sub>2</sub> capture costs are lower if high-pressure nuclear steam is integrated into the mill’s existing CHP system to replace the natural gas boiler, compared to if medium- and low-pressure steam is delivered to the mill to meet process needs directly. The CCS cost and steam requirements were used to determine the maximum price at which the mill would need to purchase nuclear steam to be competitive with steam costs from a natural gas boiler. Although the steam requirements for the nuclear cases are slightly lower than the natural gas cases, nuclear steam would need to cost a maximum of approximately $16 per metric ton to compete with natural gas steam production, roughly half the expected levelized cost of heat of $31.21 for HP steam and $25.84 for LP steam from a nuclear power plant. Although the cost of the system investigated in this study is not competitive compared to other fuel options, integrating CCS and SMNRs can help the pulp and paper industry reduce CO<sub>2</sub> emissions.</div></div>","PeriodicalId":9387,"journal":{"name":"Carbon Capture Science & Technology","volume":"16 ","pages":"Article 100468"},"PeriodicalIF":0.0000,"publicationDate":"2025-07-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Cost analysis of carbon capture and storage in the pulp and paper industry integrated with nuclear heat\",\"authors\":\"Edgar Carrejo ,&nbsp;Jhonny Alejandro Poveda-Giraldo ,&nbsp;Sam J. Root ,&nbsp;Nahuel Guaita ,&nbsp;Elizabeth Worsham ,&nbsp;Sunkyu Park\",\"doi\":\"10.1016/j.ccst.2025.100468\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><div>The pulp and paper industry generates approximately 150 million tons of CO<sub>2</sub> emissions annually, ranking among the top three industry sectors in terms of CO<sub>2</sub> emissions in the United States, when biogenic CO<sub>2</sub> is included, followed by the chemical and petroleum industries. Carbon Capture and Storage (CCS) technologies can be implemented to decrease these emissions; however, mature CCS technologies such as amine-based capture are energy-intensive. Nuclear energy can provide this energy to CCS operations without producing point source emissions. This study evaluates the economic feasibility of integrating a Small Modular Nuclear Reactor (SMNR) to power an amine-based CCS technology in three types of pulp and paper mills in the southeast of the United States: a bleached softwood kraft mill, an unbleached softwood kraft mill, and a recycling mill with an assumption of an annual production capacity of 500,000 metric tons. The presented scenarios compare the carbon capture potential and costs of a CCS system for these mills when integrated with heat from either a nuclear reactor or a natural gas boiler. Two 200 MW-thermal (MW<sub>th</sub>) small modular reactors were found to be sufficient to cover the demand for steam and power for coupling CCS and decommissioning the natural gas boiler in the bleached softwood kraft mill, while one 200 MW<sub>th</sub> SMNR module was sufficient for the other mill types. Nuclear heat integration into a CCS system, coupled with a typical kraft paper mill, can decrease CO<sub>2</sub> emissions by 91 % with the remaining 9 % being primarily biogenic. Accordingly, recycling mills powered by nuclear energy can achieve almost zero emissions. In the nuclear heat integration scenarios, the CO<sub>2</sub> capture costs are lower if high-pressure nuclear steam is integrated into the mill’s existing CHP system to replace the natural gas boiler, compared to if medium- and low-pressure steam is delivered to the mill to meet process needs directly. The CCS cost and steam requirements were used to determine the maximum price at which the mill would need to purchase nuclear steam to be competitive with steam costs from a natural gas boiler. Although the steam requirements for the nuclear cases are slightly lower than the natural gas cases, nuclear steam would need to cost a maximum of approximately $16 per metric ton to compete with natural gas steam production, roughly half the expected levelized cost of heat of $31.21 for HP steam and $25.84 for LP steam from a nuclear power plant. Although the cost of the system investigated in this study is not competitive compared to other fuel options, integrating CCS and SMNRs can help the pulp and paper industry reduce CO<sub>2</sub> emissions.</div></div>\",\"PeriodicalId\":9387,\"journal\":{\"name\":\"Carbon Capture Science & Technology\",\"volume\":\"16 \",\"pages\":\"Article 100468\"},\"PeriodicalIF\":0.0000,\"publicationDate\":\"2025-07-17\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Carbon Capture Science & Technology\",\"FirstCategoryId\":\"1085\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S2772656825001071\",\"RegionNum\":0,\"RegionCategory\":null,\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"\",\"JCRName\":\"\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Carbon Capture Science & Technology","FirstCategoryId":"1085","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S2772656825001071","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"","JCRName":"","Score":null,"Total":0}
引用次数: 0

摘要

纸浆和造纸工业每年产生约1.5亿吨的二氧化碳排放量,在美国二氧化碳排放量排名前三的工业部门中,如果包括生物二氧化碳,其次是化学和石油工业。碳捕集与封存(CCS)技术可以减少这些排放;然而,成熟的CCS技术,如基于胺的捕集是能源密集型的。核能可以在不产生点源排放的情况下为CCS操作提供这种能源。本研究评估了将小型模块化核反应堆(SMNR)集成到美国东南部三种类型的纸浆和造纸厂的胺基CCS技术的经济可行性:漂白针叶木硫酸盐厂、未漂白针叶木硫酸盐厂和假设年产能为50万吨的回收厂。所提出的方案比较了这些工厂在与核反应堆或天然气锅炉的热量相结合时,CCS系统的碳捕获潜力和成本。发现两个200兆瓦热(MWth)小型模块化反应堆足以满足耦合CCS和漂白软木硫酸盐厂天然气锅炉退役的蒸汽和电力需求,而一个200兆瓦带SMNR模块足以满足其他类型的工厂。核热集成到CCS系统中,再加上一个典型的牛皮造纸厂,可以减少91%的二氧化碳排放,剩下的9%主要是生物源的。因此,以核能为动力的回收工厂几乎可以实现零排放。在核热集成方案中,如果将高压核蒸汽集成到电厂现有的热电联产系统中,以取代天然气锅炉,那么与直接将中低压蒸汽输送到电厂以满足工艺需求相比,二氧化碳捕集成本更低。CCS成本和蒸汽需求被用来确定电厂购买核蒸汽所需的最高价格,以便与天然气锅炉的蒸汽成本竞争。尽管核电对蒸汽的需求略低于天然气,但核电蒸汽每公吨的成本最高约为16美元,才能与天然气蒸汽竞争,大约是核电站高压蒸汽31.21美元和低压蒸汽25.84美元的预期热能成本的一半。虽然本研究中所研究的系统成本与其他燃料选择相比没有竞争力,但将CCS和SMNRs结合起来可以帮助纸浆和造纸工业减少二氧化碳排放。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Cost analysis of carbon capture and storage in the pulp and paper industry integrated with nuclear heat

Cost analysis of carbon capture and storage in the pulp and paper industry integrated with nuclear heat
The pulp and paper industry generates approximately 150 million tons of CO2 emissions annually, ranking among the top three industry sectors in terms of CO2 emissions in the United States, when biogenic CO2 is included, followed by the chemical and petroleum industries. Carbon Capture and Storage (CCS) technologies can be implemented to decrease these emissions; however, mature CCS technologies such as amine-based capture are energy-intensive. Nuclear energy can provide this energy to CCS operations without producing point source emissions. This study evaluates the economic feasibility of integrating a Small Modular Nuclear Reactor (SMNR) to power an amine-based CCS technology in three types of pulp and paper mills in the southeast of the United States: a bleached softwood kraft mill, an unbleached softwood kraft mill, and a recycling mill with an assumption of an annual production capacity of 500,000 metric tons. The presented scenarios compare the carbon capture potential and costs of a CCS system for these mills when integrated with heat from either a nuclear reactor or a natural gas boiler. Two 200 MW-thermal (MWth) small modular reactors were found to be sufficient to cover the demand for steam and power for coupling CCS and decommissioning the natural gas boiler in the bleached softwood kraft mill, while one 200 MWth SMNR module was sufficient for the other mill types. Nuclear heat integration into a CCS system, coupled with a typical kraft paper mill, can decrease CO2 emissions by 91 % with the remaining 9 % being primarily biogenic. Accordingly, recycling mills powered by nuclear energy can achieve almost zero emissions. In the nuclear heat integration scenarios, the CO2 capture costs are lower if high-pressure nuclear steam is integrated into the mill’s existing CHP system to replace the natural gas boiler, compared to if medium- and low-pressure steam is delivered to the mill to meet process needs directly. The CCS cost and steam requirements were used to determine the maximum price at which the mill would need to purchase nuclear steam to be competitive with steam costs from a natural gas boiler. Although the steam requirements for the nuclear cases are slightly lower than the natural gas cases, nuclear steam would need to cost a maximum of approximately $16 per metric ton to compete with natural gas steam production, roughly half the expected levelized cost of heat of $31.21 for HP steam and $25.84 for LP steam from a nuclear power plant. Although the cost of the system investigated in this study is not competitive compared to other fuel options, integrating CCS and SMNRs can help the pulp and paper industry reduce CO2 emissions.
求助全文
通过发布文献求助,成功后即可免费获取论文全文。 去求助
来源期刊
自引率
0.00%
发文量
0
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
确定
请完成安全验证×
copy
已复制链接
快去分享给好友吧!
我知道了
右上角分享
点击右上角分享
0
联系我们:info@booksci.cn Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。 Copyright © 2023 布克学术 All rights reserved.
京ICP备2023020795号-1
ghs 京公网安备 11010802042870号
Book学术文献互助
Book学术文献互助群
群 号:604180095
Book学术官方微信