Qihao Lv , Ruopeng Cui , Peihang Li , Xuefei Zhang , Yongjian Zhang , Chunlei Wan , Renchao Che , Yue Li
{"title":"毫波厚柔性石墨烯的高选择性电磁吸收","authors":"Qihao Lv , Ruopeng Cui , Peihang Li , Xuefei Zhang , Yongjian Zhang , Chunlei Wan , Renchao Che , Yue Li","doi":"10.1016/j.mser.2025.101067","DOIUrl":null,"url":null,"abstract":"<div><div>Pursuing extremely-thin, high-selectivity, and flexible absorbers is strongly required for mitigating the electromagnetic pollution in various miniaturized and space-limited scenarios, such as flexible electronic devices, cloaking systems, and anechoic chambers. Traditional synthetic methods, focusing on enhancing the real part of the absorbing materials’ permittivity through compositional and microstructural modifications, are however confronted with many limitations and have only reached centi-wavelength thick or even larger, impeding their integration into compact and flexible devices. Herein, we propose an interdisciplinary flexible <em>metagraphene</em> architecture, in which electromagnetic waves are selectively induced by the upper anomalous resonant-antiresonant metasurface into the lower ultrahigh-loss nitrogen-doped wavy graphene-based material for flexible, extremely-thin, and high-selectivity absorption. By overcoming the inherent physical contradiction of high loss and extremely-thin absorption, <em>metagraphene</em> achieves a perfect absorption with a top-class selectivity of 357.1 at a record-breaking thickness down to 0.001<em>λ</em><sub>0</sub> (<em>λ</em><sub>0</sub> represents the wavelength with the minimum reflection), surpassing state-of-the-art absorbers by 1–2 orders of magnitude. Furthermore, <em>metagraphene</em> offers further thinning potential, large-scale manufacturability, angular stability, and frequency universality, thus promising diversified applications in extremely-miniaturized electronic devices and space-constrained equipment.</div></div>","PeriodicalId":386,"journal":{"name":"Materials Science and Engineering: R: Reports","volume":"166 ","pages":"Article 101067"},"PeriodicalIF":31.6000,"publicationDate":"2025-07-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"High-selectivity electromagnetic absorption with milli-wavelength-thick flexible metagraphene\",\"authors\":\"Qihao Lv , Ruopeng Cui , Peihang Li , Xuefei Zhang , Yongjian Zhang , Chunlei Wan , Renchao Che , Yue Li\",\"doi\":\"10.1016/j.mser.2025.101067\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><div>Pursuing extremely-thin, high-selectivity, and flexible absorbers is strongly required for mitigating the electromagnetic pollution in various miniaturized and space-limited scenarios, such as flexible electronic devices, cloaking systems, and anechoic chambers. Traditional synthetic methods, focusing on enhancing the real part of the absorbing materials’ permittivity through compositional and microstructural modifications, are however confronted with many limitations and have only reached centi-wavelength thick or even larger, impeding their integration into compact and flexible devices. Herein, we propose an interdisciplinary flexible <em>metagraphene</em> architecture, in which electromagnetic waves are selectively induced by the upper anomalous resonant-antiresonant metasurface into the lower ultrahigh-loss nitrogen-doped wavy graphene-based material for flexible, extremely-thin, and high-selectivity absorption. By overcoming the inherent physical contradiction of high loss and extremely-thin absorption, <em>metagraphene</em> achieves a perfect absorption with a top-class selectivity of 357.1 at a record-breaking thickness down to 0.001<em>λ</em><sub>0</sub> (<em>λ</em><sub>0</sub> represents the wavelength with the minimum reflection), surpassing state-of-the-art absorbers by 1–2 orders of magnitude. Furthermore, <em>metagraphene</em> offers further thinning potential, large-scale manufacturability, angular stability, and frequency universality, thus promising diversified applications in extremely-miniaturized electronic devices and space-constrained equipment.</div></div>\",\"PeriodicalId\":386,\"journal\":{\"name\":\"Materials Science and Engineering: R: Reports\",\"volume\":\"166 \",\"pages\":\"Article 101067\"},\"PeriodicalIF\":31.6000,\"publicationDate\":\"2025-07-24\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Materials Science and Engineering: R: Reports\",\"FirstCategoryId\":\"5\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S0927796X25001445\",\"RegionNum\":1,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"MATERIALS SCIENCE, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Materials Science and Engineering: R: Reports","FirstCategoryId":"5","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S0927796X25001445","RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"MATERIALS SCIENCE, MULTIDISCIPLINARY","Score":null,"Total":0}
High-selectivity electromagnetic absorption with milli-wavelength-thick flexible metagraphene
Pursuing extremely-thin, high-selectivity, and flexible absorbers is strongly required for mitigating the electromagnetic pollution in various miniaturized and space-limited scenarios, such as flexible electronic devices, cloaking systems, and anechoic chambers. Traditional synthetic methods, focusing on enhancing the real part of the absorbing materials’ permittivity through compositional and microstructural modifications, are however confronted with many limitations and have only reached centi-wavelength thick or even larger, impeding their integration into compact and flexible devices. Herein, we propose an interdisciplinary flexible metagraphene architecture, in which electromagnetic waves are selectively induced by the upper anomalous resonant-antiresonant metasurface into the lower ultrahigh-loss nitrogen-doped wavy graphene-based material for flexible, extremely-thin, and high-selectivity absorption. By overcoming the inherent physical contradiction of high loss and extremely-thin absorption, metagraphene achieves a perfect absorption with a top-class selectivity of 357.1 at a record-breaking thickness down to 0.001λ0 (λ0 represents the wavelength with the minimum reflection), surpassing state-of-the-art absorbers by 1–2 orders of magnitude. Furthermore, metagraphene offers further thinning potential, large-scale manufacturability, angular stability, and frequency universality, thus promising diversified applications in extremely-miniaturized electronic devices and space-constrained equipment.
期刊介绍:
Materials Science & Engineering R: Reports is a journal that covers a wide range of topics in the field of materials science and engineering. It publishes both experimental and theoretical research papers, providing background information and critical assessments on various topics. The journal aims to publish high-quality and novel research papers and reviews.
The subject areas covered by the journal include Materials Science (General), Electronic Materials, Optical Materials, and Magnetic Materials. In addition to regular issues, the journal also publishes special issues on key themes in the field of materials science, including Energy Materials, Materials for Health, Materials Discovery, Innovation for High Value Manufacturing, and Sustainable Materials development.