毫波厚柔性石墨烯的高选择性电磁吸收

IF 31.6 1区 材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY
Qihao Lv , Ruopeng Cui , Peihang Li , Xuefei Zhang , Yongjian Zhang , Chunlei Wan , Renchao Che , Yue Li
{"title":"毫波厚柔性石墨烯的高选择性电磁吸收","authors":"Qihao Lv ,&nbsp;Ruopeng Cui ,&nbsp;Peihang Li ,&nbsp;Xuefei Zhang ,&nbsp;Yongjian Zhang ,&nbsp;Chunlei Wan ,&nbsp;Renchao Che ,&nbsp;Yue Li","doi":"10.1016/j.mser.2025.101067","DOIUrl":null,"url":null,"abstract":"<div><div>Pursuing extremely-thin, high-selectivity, and flexible absorbers is strongly required for mitigating the electromagnetic pollution in various miniaturized and space-limited scenarios, such as flexible electronic devices, cloaking systems, and anechoic chambers. Traditional synthetic methods, focusing on enhancing the real part of the absorbing materials’ permittivity through compositional and microstructural modifications, are however confronted with many limitations and have only reached centi-wavelength thick or even larger, impeding their integration into compact and flexible devices. Herein, we propose an interdisciplinary flexible <em>metagraphene</em> architecture, in which electromagnetic waves are selectively induced by the upper anomalous resonant-antiresonant metasurface into the lower ultrahigh-loss nitrogen-doped wavy graphene-based material for flexible, extremely-thin, and high-selectivity absorption. By overcoming the inherent physical contradiction of high loss and extremely-thin absorption, <em>metagraphene</em> achieves a perfect absorption with a top-class selectivity of 357.1 at a record-breaking thickness down to 0.001<em>λ</em><sub>0</sub> (<em>λ</em><sub>0</sub> represents the wavelength with the minimum reflection), surpassing state-of-the-art absorbers by 1–2 orders of magnitude. Furthermore, <em>metagraphene</em> offers further thinning potential, large-scale manufacturability, angular stability, and frequency universality, thus promising diversified applications in extremely-miniaturized electronic devices and space-constrained equipment.</div></div>","PeriodicalId":386,"journal":{"name":"Materials Science and Engineering: R: Reports","volume":"166 ","pages":"Article 101067"},"PeriodicalIF":31.6000,"publicationDate":"2025-07-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"High-selectivity electromagnetic absorption with milli-wavelength-thick flexible metagraphene\",\"authors\":\"Qihao Lv ,&nbsp;Ruopeng Cui ,&nbsp;Peihang Li ,&nbsp;Xuefei Zhang ,&nbsp;Yongjian Zhang ,&nbsp;Chunlei Wan ,&nbsp;Renchao Che ,&nbsp;Yue Li\",\"doi\":\"10.1016/j.mser.2025.101067\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><div>Pursuing extremely-thin, high-selectivity, and flexible absorbers is strongly required for mitigating the electromagnetic pollution in various miniaturized and space-limited scenarios, such as flexible electronic devices, cloaking systems, and anechoic chambers. Traditional synthetic methods, focusing on enhancing the real part of the absorbing materials’ permittivity through compositional and microstructural modifications, are however confronted with many limitations and have only reached centi-wavelength thick or even larger, impeding their integration into compact and flexible devices. Herein, we propose an interdisciplinary flexible <em>metagraphene</em> architecture, in which electromagnetic waves are selectively induced by the upper anomalous resonant-antiresonant metasurface into the lower ultrahigh-loss nitrogen-doped wavy graphene-based material for flexible, extremely-thin, and high-selectivity absorption. By overcoming the inherent physical contradiction of high loss and extremely-thin absorption, <em>metagraphene</em> achieves a perfect absorption with a top-class selectivity of 357.1 at a record-breaking thickness down to 0.001<em>λ</em><sub>0</sub> (<em>λ</em><sub>0</sub> represents the wavelength with the minimum reflection), surpassing state-of-the-art absorbers by 1–2 orders of magnitude. Furthermore, <em>metagraphene</em> offers further thinning potential, large-scale manufacturability, angular stability, and frequency universality, thus promising diversified applications in extremely-miniaturized electronic devices and space-constrained equipment.</div></div>\",\"PeriodicalId\":386,\"journal\":{\"name\":\"Materials Science and Engineering: R: Reports\",\"volume\":\"166 \",\"pages\":\"Article 101067\"},\"PeriodicalIF\":31.6000,\"publicationDate\":\"2025-07-24\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Materials Science and Engineering: R: Reports\",\"FirstCategoryId\":\"5\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S0927796X25001445\",\"RegionNum\":1,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"MATERIALS SCIENCE, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Materials Science and Engineering: R: Reports","FirstCategoryId":"5","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S0927796X25001445","RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"MATERIALS SCIENCE, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0

摘要

在各种小型化和空间有限的情况下,如柔性电子设备、隐身系统和消声室,迫切需要追求极薄、高选择性和柔性吸收器来减轻电磁污染。传统的合成方法侧重于通过成分和微观结构的改变来提高吸收材料的实部介电常数,但面临许多限制,只能达到厘米波长甚至更大的厚度,阻碍了它们集成到紧凑和灵活的器件中。在此,我们提出了一种跨学科的柔性石墨烯结构,其中电磁波被上部异常共振-反共振超表面选择性地诱导到下部超高损耗氮掺杂的波纹石墨烯基材料中,以实现柔性,极薄和高选择性吸收。通过克服高损耗和极薄吸收的固有物理矛盾,石墨烯实现了完美的吸收,在破纪录的厚度低至0.001λ0 (λ0表示反射最小的波长)的情况下,具有357.1的顶级选择性,超过了目前最先进的吸收剂1-2个数量级。此外,石墨烯具有进一步减薄的潜力、可大规模制造性、角稳定性和频率通用性,因此在极小型化电子设备和空间受限设备中有广泛的应用前景。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
High-selectivity electromagnetic absorption with milli-wavelength-thick flexible metagraphene
Pursuing extremely-thin, high-selectivity, and flexible absorbers is strongly required for mitigating the electromagnetic pollution in various miniaturized and space-limited scenarios, such as flexible electronic devices, cloaking systems, and anechoic chambers. Traditional synthetic methods, focusing on enhancing the real part of the absorbing materials’ permittivity through compositional and microstructural modifications, are however confronted with many limitations and have only reached centi-wavelength thick or even larger, impeding their integration into compact and flexible devices. Herein, we propose an interdisciplinary flexible metagraphene architecture, in which electromagnetic waves are selectively induced by the upper anomalous resonant-antiresonant metasurface into the lower ultrahigh-loss nitrogen-doped wavy graphene-based material for flexible, extremely-thin, and high-selectivity absorption. By overcoming the inherent physical contradiction of high loss and extremely-thin absorption, metagraphene achieves a perfect absorption with a top-class selectivity of 357.1 at a record-breaking thickness down to 0.001λ0 (λ0 represents the wavelength with the minimum reflection), surpassing state-of-the-art absorbers by 1–2 orders of magnitude. Furthermore, metagraphene offers further thinning potential, large-scale manufacturability, angular stability, and frequency universality, thus promising diversified applications in extremely-miniaturized electronic devices and space-constrained equipment.
求助全文
通过发布文献求助,成功后即可免费获取论文全文。 去求助
来源期刊
Materials Science and Engineering: R: Reports
Materials Science and Engineering: R: Reports 工程技术-材料科学:综合
CiteScore
60.50
自引率
0.30%
发文量
19
审稿时长
34 days
期刊介绍: Materials Science & Engineering R: Reports is a journal that covers a wide range of topics in the field of materials science and engineering. It publishes both experimental and theoretical research papers, providing background information and critical assessments on various topics. The journal aims to publish high-quality and novel research papers and reviews. The subject areas covered by the journal include Materials Science (General), Electronic Materials, Optical Materials, and Magnetic Materials. In addition to regular issues, the journal also publishes special issues on key themes in the field of materials science, including Energy Materials, Materials for Health, Materials Discovery, Innovation for High Value Manufacturing, and Sustainable Materials development.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
确定
请完成安全验证×
copy
已复制链接
快去分享给好友吧!
我知道了
右上角分享
点击右上角分享
0
联系我们:info@booksci.cn Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。 Copyright © 2023 布克学术 All rights reserved.
京ICP备2023020795号-1
ghs 京公网安备 11010802042870号
Book学术文献互助
Book学术文献互助群
群 号:604180095
Book学术官方微信