{"title":"在沼气净化中培育基于自然的解决方案和循环方法:强化多级人工湿地硝化的沼液浓缩液在缺氧生物脱硫中作为电子受体的验证","authors":"Rubén Hervás-Martínez, Núria Oliver, Tatiana Montoya, Feliu Sempere","doi":"10.1016/j.biortech.2025.133012","DOIUrl":null,"url":null,"abstract":"<div><div>Anoxic biodesulphurisation using a biogenic nitrified source as an electron acceptor is a potential alternative to aerobic H<sub>2</sub>S biotreatment. This work reports the successful combination of nitrified centrate obtained from innovative constructed wetlands (CWs) with anoxic suspended biomass bioreactors (SBBs) treating real biogas. The quality of the liquid medium on the biodesulphurisation process was evaluated. The SBBs (of 48 L and 130 L, respectively) shifted seamlessly from using nitrified centrate from activated sludge to nitrified centrate from CWs, but its low orthophosphate content did limit H<sub>2</sub>S removal. To overcome this limitation, raw centrate was supplied. When nitrate + nitrite and orthophosphate concentrations were above 10 mgN L<sup>−1</sup> and 10 mgP L<sup>−1</sup>, 92 % of the H<sub>2</sub>S was removed in SBB1 (H<sub>2</sub>S elimination capacity (EC) of 3.0 gH<sub>2</sub>S Nm<sup>−3</sup>h<sup>−1</sup>), and 95 % in SBB2 (H<sub>2</sub>S-EC of 13.1 gH<sub>2</sub>S Nm<sup>−3</sup>h<sup>−1</sup>) at a gas residence time of 4.0 min and 3.1 min respectively.</div></div>","PeriodicalId":258,"journal":{"name":"Bioresource Technology","volume":"436 ","pages":"Article 133012"},"PeriodicalIF":9.7000,"publicationDate":"2025-07-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Fostering nature-based solutions and circular approaches in biogas purification: validation of digestate centrate nitrified by intensified multi-stage constructed wetlands as electron acceptor in anoxic biodesulphurisation\",\"authors\":\"Rubén Hervás-Martínez, Núria Oliver, Tatiana Montoya, Feliu Sempere\",\"doi\":\"10.1016/j.biortech.2025.133012\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><div>Anoxic biodesulphurisation using a biogenic nitrified source as an electron acceptor is a potential alternative to aerobic H<sub>2</sub>S biotreatment. This work reports the successful combination of nitrified centrate obtained from innovative constructed wetlands (CWs) with anoxic suspended biomass bioreactors (SBBs) treating real biogas. The quality of the liquid medium on the biodesulphurisation process was evaluated. The SBBs (of 48 L and 130 L, respectively) shifted seamlessly from using nitrified centrate from activated sludge to nitrified centrate from CWs, but its low orthophosphate content did limit H<sub>2</sub>S removal. To overcome this limitation, raw centrate was supplied. When nitrate + nitrite and orthophosphate concentrations were above 10 mgN L<sup>−1</sup> and 10 mgP L<sup>−1</sup>, 92 % of the H<sub>2</sub>S was removed in SBB1 (H<sub>2</sub>S elimination capacity (EC) of 3.0 gH<sub>2</sub>S Nm<sup>−3</sup>h<sup>−1</sup>), and 95 % in SBB2 (H<sub>2</sub>S-EC of 13.1 gH<sub>2</sub>S Nm<sup>−3</sup>h<sup>−1</sup>) at a gas residence time of 4.0 min and 3.1 min respectively.</div></div>\",\"PeriodicalId\":258,\"journal\":{\"name\":\"Bioresource Technology\",\"volume\":\"436 \",\"pages\":\"Article 133012\"},\"PeriodicalIF\":9.7000,\"publicationDate\":\"2025-07-17\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Bioresource Technology\",\"FirstCategoryId\":\"5\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S0960852425009782\",\"RegionNum\":1,\"RegionCategory\":\"环境科学与生态学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"AGRICULTURAL ENGINEERING\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Bioresource Technology","FirstCategoryId":"5","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S0960852425009782","RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"AGRICULTURAL ENGINEERING","Score":null,"Total":0}
Fostering nature-based solutions and circular approaches in biogas purification: validation of digestate centrate nitrified by intensified multi-stage constructed wetlands as electron acceptor in anoxic biodesulphurisation
Anoxic biodesulphurisation using a biogenic nitrified source as an electron acceptor is a potential alternative to aerobic H2S biotreatment. This work reports the successful combination of nitrified centrate obtained from innovative constructed wetlands (CWs) with anoxic suspended biomass bioreactors (SBBs) treating real biogas. The quality of the liquid medium on the biodesulphurisation process was evaluated. The SBBs (of 48 L and 130 L, respectively) shifted seamlessly from using nitrified centrate from activated sludge to nitrified centrate from CWs, but its low orthophosphate content did limit H2S removal. To overcome this limitation, raw centrate was supplied. When nitrate + nitrite and orthophosphate concentrations were above 10 mgN L−1 and 10 mgP L−1, 92 % of the H2S was removed in SBB1 (H2S elimination capacity (EC) of 3.0 gH2S Nm−3h−1), and 95 % in SBB2 (H2S-EC of 13.1 gH2S Nm−3h−1) at a gas residence time of 4.0 min and 3.1 min respectively.
期刊介绍:
Bioresource Technology publishes original articles, review articles, case studies, and short communications covering the fundamentals, applications, and management of bioresource technology. The journal seeks to advance and disseminate knowledge across various areas related to biomass, biological waste treatment, bioenergy, biotransformations, bioresource systems analysis, and associated conversion or production technologies.
Topics include:
• Biofuels: liquid and gaseous biofuels production, modeling and economics
• Bioprocesses and bioproducts: biocatalysis and fermentations
• Biomass and feedstocks utilization: bioconversion of agro-industrial residues
• Environmental protection: biological waste treatment
• Thermochemical conversion of biomass: combustion, pyrolysis, gasification, catalysis.