Xinru Zhang , Yijie Wang , Lei Zhang , Xiaohai Zhang , Bao Hao , Xiaorui Liang , Helei Dong , Yongqiang Qin , Qiulin Tan
{"title":"一种GA-BP补偿PEDOT:PSS/MXene可穿戴式NH3检测装置,用于食品安全、环境监测和疾病诊断","authors":"Xinru Zhang , Yijie Wang , Lei Zhang , Xiaohai Zhang , Bao Hao , Xiaorui Liang , Helei Dong , Yongqiang Qin , Qiulin Tan","doi":"10.1016/j.snb.2025.138326","DOIUrl":null,"url":null,"abstract":"<div><div>The real-time and accurate detection of ammonia is critical for food freshness testing, agricultural monitoring, and respiratory health diagnostics. Recently, flexible gas sensors have garnered attention owing to their potential for integration into smart wearable electronics and display devices. However, the development of high-performance, low-power, and stable devices remains challenging. In this study, a chemoresistive sensor based on poly(3,4-ethylenedioxythiophene):poly(styrenesulfonate) (PEDOT:PSS)/MXene composites is designed, wherein the application of a genetic algorithm-optimized back propagation neural network to compensate for humidity leads to a significantly enhanced detection accuracy. Notably, the use of a genetic algorithm-optimized back propagation neural network reduces the detection error from 8.06 % to 1.3 % in the presence of 50 ppm NH<sub>3</sub>. A wireless Bluetooth monitoring system is integrated to enable real-time data transmission and remote monitoring. This sensor detects ammonia within the range of 0.6–1000 ppm, demonstrating an excellent stability, selectivity, and flexibility, thereby confirming the synergistic effects between PEDOT:PSS and MXene. Importantly, in application tests, the developed system reliably assesses meat spoilage and farm ventilation levels, indicating its high applicability and reliability. Successful human breath tests also open new possibilities for the application of this sensor in respiratory health monitoring. Ultimately, this study offers a convenient and efficient approach for food quality assurance, disease diagnosis, and environmental monitoring.</div></div>","PeriodicalId":425,"journal":{"name":"Sensors and Actuators B: Chemical","volume":"444 ","pages":"Article 138326"},"PeriodicalIF":8.0000,"publicationDate":"2025-07-14","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"A GA-BP compensated PEDOT:PSS/MXene wearable NH3 detection device for food safety, environmental monitoring, and disease diagnosis\",\"authors\":\"Xinru Zhang , Yijie Wang , Lei Zhang , Xiaohai Zhang , Bao Hao , Xiaorui Liang , Helei Dong , Yongqiang Qin , Qiulin Tan\",\"doi\":\"10.1016/j.snb.2025.138326\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><div>The real-time and accurate detection of ammonia is critical for food freshness testing, agricultural monitoring, and respiratory health diagnostics. Recently, flexible gas sensors have garnered attention owing to their potential for integration into smart wearable electronics and display devices. However, the development of high-performance, low-power, and stable devices remains challenging. In this study, a chemoresistive sensor based on poly(3,4-ethylenedioxythiophene):poly(styrenesulfonate) (PEDOT:PSS)/MXene composites is designed, wherein the application of a genetic algorithm-optimized back propagation neural network to compensate for humidity leads to a significantly enhanced detection accuracy. Notably, the use of a genetic algorithm-optimized back propagation neural network reduces the detection error from 8.06 % to 1.3 % in the presence of 50 ppm NH<sub>3</sub>. A wireless Bluetooth monitoring system is integrated to enable real-time data transmission and remote monitoring. This sensor detects ammonia within the range of 0.6–1000 ppm, demonstrating an excellent stability, selectivity, and flexibility, thereby confirming the synergistic effects between PEDOT:PSS and MXene. Importantly, in application tests, the developed system reliably assesses meat spoilage and farm ventilation levels, indicating its high applicability and reliability. Successful human breath tests also open new possibilities for the application of this sensor in respiratory health monitoring. Ultimately, this study offers a convenient and efficient approach for food quality assurance, disease diagnosis, and environmental monitoring.</div></div>\",\"PeriodicalId\":425,\"journal\":{\"name\":\"Sensors and Actuators B: Chemical\",\"volume\":\"444 \",\"pages\":\"Article 138326\"},\"PeriodicalIF\":8.0000,\"publicationDate\":\"2025-07-14\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Sensors and Actuators B: Chemical\",\"FirstCategoryId\":\"92\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S0925400525011025\",\"RegionNum\":1,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"CHEMISTRY, ANALYTICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Sensors and Actuators B: Chemical","FirstCategoryId":"92","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S0925400525011025","RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, ANALYTICAL","Score":null,"Total":0}
A GA-BP compensated PEDOT:PSS/MXene wearable NH3 detection device for food safety, environmental monitoring, and disease diagnosis
The real-time and accurate detection of ammonia is critical for food freshness testing, agricultural monitoring, and respiratory health diagnostics. Recently, flexible gas sensors have garnered attention owing to their potential for integration into smart wearable electronics and display devices. However, the development of high-performance, low-power, and stable devices remains challenging. In this study, a chemoresistive sensor based on poly(3,4-ethylenedioxythiophene):poly(styrenesulfonate) (PEDOT:PSS)/MXene composites is designed, wherein the application of a genetic algorithm-optimized back propagation neural network to compensate for humidity leads to a significantly enhanced detection accuracy. Notably, the use of a genetic algorithm-optimized back propagation neural network reduces the detection error from 8.06 % to 1.3 % in the presence of 50 ppm NH3. A wireless Bluetooth monitoring system is integrated to enable real-time data transmission and remote monitoring. This sensor detects ammonia within the range of 0.6–1000 ppm, demonstrating an excellent stability, selectivity, and flexibility, thereby confirming the synergistic effects between PEDOT:PSS and MXene. Importantly, in application tests, the developed system reliably assesses meat spoilage and farm ventilation levels, indicating its high applicability and reliability. Successful human breath tests also open new possibilities for the application of this sensor in respiratory health monitoring. Ultimately, this study offers a convenient and efficient approach for food quality assurance, disease diagnosis, and environmental monitoring.
期刊介绍:
Sensors & Actuators, B: Chemical is an international journal focused on the research and development of chemical transducers. It covers chemical sensors and biosensors, chemical actuators, and analytical microsystems. The journal is interdisciplinary, aiming to publish original works showcasing substantial advancements beyond the current state of the art in these fields, with practical applicability to solving meaningful analytical problems. Review articles are accepted by invitation from an Editor of the journal.