增强协同Dion-Jacobson 2D-3D钙钛矿- cigs串联太阳能电池的滤波光谱和电流匹配分析：达到32.56%的效率

IF 3.9 3区材料科学 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY

Materials Science and Engineering: B Pub Date : 2025-07-10 DOI:10.1016/j.mseb.2025.118599

Gauri Pathak , Yashwant Kumar Singh , D.K. Dwivedi , Pooja Lohia , Rahul Pandey , Upendra Kulshrestha , Manish Kumar

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引用次数: 0

摘要

串联太阳能电池具有比传统太阳能电池更高的功率转换效率（PCE）的潜力。目前的工作是基于两个电池的模拟-顶部电池（TCELL）和底部电池（BCELL），依赖于每个电池的吸收层带隙。TCELL拥有Dion-Jacobson (DJ) 2D-3D金属卤化物钙钛矿材料，在实现高性能方面发挥了主要作用。TCELL二维材料PeDAMA2Pb3I10（带隙= 1.83 eV）添加在三维层材料CH3NH3SnI3（带隙= 1.3 eV）之上，制成二维/三维混合钙钛矿太阳能电池，三维层钙钛矿对环境友好，具有更高的理论效率值。BCELL采用带隙值为1.27 eV的CIGS（铜铟硒化镓）材料，用于吸收阳光，特别是在冬季，而且它比碲化镉（CdTe）电池毒性更小。本研究利用一维太阳能电池电容模拟器（SCAPS-1D）程序对开路电压（VOC）等重要参数进行分析；短路电流密度；填充系数（FF）和功率转换效率（PCE）。在独立情况下，（TCELL， BCELL）的功率转换效率百分比：（23.72,26.32），（TCELL， BCELL）的开路电压百分比：（1.0,0.89），（TCELL， BCELL）的填充因子百分比：（78.48,86.72）和（TCELL， BCELL）的短路电压百分比（27.7,33.95）在空气质量1.5光谱下测量，辐照度为100 mW/cm2, 300 K。优化后，得到了2D-3D缺陷密度（cm−3）的顶层和底层电池活性层厚度变化的各种模拟结果。TCELL和BCELL利用广谱光，从而产生多余的电子和空穴，从而有助于更多的PCE，因此提供卓越的性能。利用滤波后的光谱和匹配的电流，得到了钙钛矿- cigs串联太阳能电池（PCTSC），该电池具有优异的光伏（PV）参数，PCE = 32.56%, VOC = 1.77 V, JSC = 22.14 mA/cm2, FF = 83.11%。这一全面的讨论有助于PCTSC的未来发展。清洁能源。

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Augmenting the filtered spectrum and current matching analysis of synergistic Dion-Jacobson 2D-3D Perovskite-CIGS tandem solar Cell: Achieving 32.56% efficiency

Tandem solar cell has potential for higher PCE (power conversion efficiency) value than traditional solar cells. Present work is based on simulation of two cells- top cell (T_CELL) and bottom cell (B_CELL) which relies on absorber layer’s bandgap of each cell. T_CELL has Dion-Jacobson (DJ) 2D-3D metal halide perovskite material which play main role to achieve high performance. T_CELL 2D material PeDAMA₂Pb₃I₁₀ (bandgap = 1.83 eV) added on top of the 3D layer material CH₃NH₃SnI₃ (bandgap = 1.3 eV) to create a 2D/3D hybrid perovskite solar cell in which 3D layer perovskite is environment friendly, having higher theoretical efficiency value. B_CELL has CIGS (Copper Indium Gallium Selenide) material with bandgap value 1.27 eV used to absorb sunlight specially in winter seasons also it is less toxic than Cadmium telluride (CdTe) cell. In present work, the one-dimensional solar cell capacitance simulator (SCAPS-1D) program is utilized to analyze important parameter like open-circuit voltage (V_OC); short- circuit current density (J_SC); fill factor (FF) and power conversion efficiency (PCE). In case of standalone, power conversion efficiency in percentage for (T_CELL, B_CELL): (23.72, 26.32), open circuit voltage in volts for (T_CELL, B_CELL): (1.0, 0.89), fill factor in percentage for (T_CELL, B_CELL): (78.48, 86.72) and short circuit voltage in mA/cm² for (T_CELL, B_CELL): (27.7, 33.95) measured under Air-Mass1.5 spectrum with irradiance of 100 mW/cm² at 300 K. After optimization, the various simulation work related to thickness variation for 2D-3D top layer with defect density (cm⁻³) as well as for bottom cell active layer has been obtained. T_CELL and B_CELL utilizes a broad spectrum of light thus generating excess electrons and holes which contribute towards more PCE, therefore delivering superior performance. Consequently, a perovskite-CIGS tandem solar cell (PCTSC) has been obtained using filtered spectrum along with matching its current that displays outstanding photovoltaic (PV) parameter with high PCE = 32.56 %, V_OC = 1.77 V, J_SC = 22.14 mA/cm² and FF = 83.11 %. This comprehensive discussion helps in future development of PCTSC for Affordable & Clean Energy.

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来源期刊

Materials Science and Engineering: B 工程技术-材料科学：综合

CiteScore

5.60

自引率

2.80%

发文量

481

审稿时长

3.5 months

期刊介绍： The journal provides an international medium for the publication of theoretical and experimental studies and reviews related to the electronic, electrochemical, ionic, magnetic, optical, and biosensing properties of solid state materials in bulk, thin film and particulate forms. Papers dealing with synthesis, processing, characterization, structure, physical properties and computational aspects of nano-crystalline, crystalline, amorphous and glassy forms of ceramics, semiconductors, layered insertion compounds, low-dimensional compounds and systems, fast-ion conductors, polymers and dielectrics are viewed as suitable for publication. Articles focused on nano-structured aspects of these advanced solid-state materials will also be considered suitable.