Chengfeng Shen, Xiangyue Wei, Qiang Zhang, Pengbo Ye, Xuehui Liu, Shimei Xu, Yu-Zhong Wang
{"title":"将聚乙烯氧化升级回收成可降解、可回收和高性能的材料。","authors":"Chengfeng Shen, Xiangyue Wei, Qiang Zhang, Pengbo Ye, Xuehui Liu, Shimei Xu, Yu-Zhong Wang","doi":"10.1039/d5mh00967g","DOIUrl":null,"url":null,"abstract":"<p><p>Polyethylene waste was oxidatively converted into hydroxyl-terminated telechelic macromolecules with controlled molecular weights, which were further reconstructed into sustainable materials with enhanced strength, processability, degradability/recyclability, and filler compatibility through dynamic cross-linking. This strategy enables efficient upcycling of PE into sustainable, high-performance polymers, addressing plastic pollution and advancing circular materials.</p>","PeriodicalId":87,"journal":{"name":"Materials Horizons","volume":" ","pages":""},"PeriodicalIF":12.2000,"publicationDate":"2025-07-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Oxidation upcycling of polyethylene into degradable, recyclable and high-performance materials.\",\"authors\":\"Chengfeng Shen, Xiangyue Wei, Qiang Zhang, Pengbo Ye, Xuehui Liu, Shimei Xu, Yu-Zhong Wang\",\"doi\":\"10.1039/d5mh00967g\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p><p>Polyethylene waste was oxidatively converted into hydroxyl-terminated telechelic macromolecules with controlled molecular weights, which were further reconstructed into sustainable materials with enhanced strength, processability, degradability/recyclability, and filler compatibility through dynamic cross-linking. This strategy enables efficient upcycling of PE into sustainable, high-performance polymers, addressing plastic pollution and advancing circular materials.</p>\",\"PeriodicalId\":87,\"journal\":{\"name\":\"Materials Horizons\",\"volume\":\" \",\"pages\":\"\"},\"PeriodicalIF\":12.2000,\"publicationDate\":\"2025-07-08\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Materials Horizons\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://doi.org/10.1039/d5mh00967g\",\"RegionNum\":2,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"CHEMISTRY, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Materials Horizons","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1039/d5mh00967g","RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
Oxidation upcycling of polyethylene into degradable, recyclable and high-performance materials.
Polyethylene waste was oxidatively converted into hydroxyl-terminated telechelic macromolecules with controlled molecular weights, which were further reconstructed into sustainable materials with enhanced strength, processability, degradability/recyclability, and filler compatibility through dynamic cross-linking. This strategy enables efficient upcycling of PE into sustainable, high-performance polymers, addressing plastic pollution and advancing circular materials.