{"title":"超高灵敏度PtNPs@CsCu2I3/AlGaN范德华异质结自供电光电探测器,实现精确的太阳盲紫外光度定量","authors":"Guokang Sun, Wenjie Li, Peng Wan, Tong Xu, Yalin Zhai, Chengyu Luan, Yuqi Zhou, Caixia Kan, Daning Shi, Mingming Jiang","doi":"10.1063/5.0276958","DOIUrl":null,"url":null,"abstract":"High-fidelity quantitative detection in the solar-blind ultraviolet regime is essential for radiation-hardened optical systems and secure communications. This study demonstrates a pioneering self-powered ultraviolet photodetector utilizing an engineered CsCu2I3/AlGaN van der Waals heterojunction (vdWh) architecture, enabling high-precision light irradiance measurement. Through strategic integration of size-controlled platinum nanoparticles (PtNPs) that induce localized surface plasmon resonances enhancement, the optimized device achieves remarkable performance metrics at zero bias: a photoresponsivity of 200 mA/W, a specific detectivity of 1.65 × 1012 Jones as well as ultrafast response speed with rise/fall times of 400/540 μs under 254 nm illumination, surpassing the majority of its competitors. The unencapsulated detector exhibits robust thermal-humidity stability under ambient conditions, demonstrating exceptional reliability. A prototype light-intensity monitoring system, integrating this PtNPs@CsCu2I3/AlGaN vdWh detector with customized signal processing circuitry, demonstrates exceptional measurement accuracy with absolute error < 5.0 μ W/cm2 and relative error < 5.0%, respectively. This work develops high-performance solar-blind ultraviolet photodetectors using eco-friendly lead-free perovskites with tailored interfaces, and establishes an integration framework bridging these devices to deep-ultraviolet photonics and radiation-resistant applications.","PeriodicalId":8094,"journal":{"name":"Applied Physics Letters","volume":"411 1","pages":""},"PeriodicalIF":3.6000,"publicationDate":"2025-07-07","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Ultrahigh-sensitivity PtNPs@CsCu2I3/AlGaN van der Waals heterojunction self-powered photodetector enabling precision solar-blind UV photometric quantification\",\"authors\":\"Guokang Sun, Wenjie Li, Peng Wan, Tong Xu, Yalin Zhai, Chengyu Luan, Yuqi Zhou, Caixia Kan, Daning Shi, Mingming Jiang\",\"doi\":\"10.1063/5.0276958\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"High-fidelity quantitative detection in the solar-blind ultraviolet regime is essential for radiation-hardened optical systems and secure communications. This study demonstrates a pioneering self-powered ultraviolet photodetector utilizing an engineered CsCu2I3/AlGaN van der Waals heterojunction (vdWh) architecture, enabling high-precision light irradiance measurement. Through strategic integration of size-controlled platinum nanoparticles (PtNPs) that induce localized surface plasmon resonances enhancement, the optimized device achieves remarkable performance metrics at zero bias: a photoresponsivity of 200 mA/W, a specific detectivity of 1.65 × 1012 Jones as well as ultrafast response speed with rise/fall times of 400/540 μs under 254 nm illumination, surpassing the majority of its competitors. The unencapsulated detector exhibits robust thermal-humidity stability under ambient conditions, demonstrating exceptional reliability. A prototype light-intensity monitoring system, integrating this PtNPs@CsCu2I3/AlGaN vdWh detector with customized signal processing circuitry, demonstrates exceptional measurement accuracy with absolute error < 5.0 μ W/cm2 and relative error < 5.0%, respectively. This work develops high-performance solar-blind ultraviolet photodetectors using eco-friendly lead-free perovskites with tailored interfaces, and establishes an integration framework bridging these devices to deep-ultraviolet photonics and radiation-resistant applications.\",\"PeriodicalId\":8094,\"journal\":{\"name\":\"Applied Physics Letters\",\"volume\":\"411 1\",\"pages\":\"\"},\"PeriodicalIF\":3.6000,\"publicationDate\":\"2025-07-07\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Applied Physics Letters\",\"FirstCategoryId\":\"101\",\"ListUrlMain\":\"https://doi.org/10.1063/5.0276958\",\"RegionNum\":2,\"RegionCategory\":\"物理与天体物理\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"PHYSICS, APPLIED\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Applied Physics Letters","FirstCategoryId":"101","ListUrlMain":"https://doi.org/10.1063/5.0276958","RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"PHYSICS, APPLIED","Score":null,"Total":0}
引用次数: 0
摘要
太阳盲紫外波段的高保真定量检测对于抗辐射光学系统和安全通信至关重要。本研究展示了一种开创性的自供电紫外光电探测器,利用工程CsCu2I3/AlGaN van der Waals异质结(vdWh)结构,实现高精度光辐照度测量。通过整合尺寸可控铂纳米粒子(PtNPs)诱导局部表面等离子体共振增强,优化后的器件在零偏置下实现了卓越的性能指标:光响应率为200 mA/W,比探测率为1.65 × 1012 Jones,以及在254 nm照明下上升/下降时间为400/540 μs的超快响应速度,超过了大多数竞争对手。未封装的探测器在环境条件下表现出强大的热湿稳定性,表现出卓越的可靠性。一个原型光强监测系统,集成了PtNPs@CsCu2I3/AlGaN vdWh探测器和定制的信号处理电路,在绝对误差下展示了卓越的测量精度&;lt;5.0 μ W/cm2,相对误差&;lt;5.0%,分别。这项工作开发了高性能的太阳盲紫外光电探测器,使用具有定制接口的环保无铅钙钛矿,并建立了一个集成框架,将这些设备连接到深紫外光子学和抗辐射应用中。
Ultrahigh-sensitivity PtNPs@CsCu2I3/AlGaN van der Waals heterojunction self-powered photodetector enabling precision solar-blind UV photometric quantification
High-fidelity quantitative detection in the solar-blind ultraviolet regime is essential for radiation-hardened optical systems and secure communications. This study demonstrates a pioneering self-powered ultraviolet photodetector utilizing an engineered CsCu2I3/AlGaN van der Waals heterojunction (vdWh) architecture, enabling high-precision light irradiance measurement. Through strategic integration of size-controlled platinum nanoparticles (PtNPs) that induce localized surface plasmon resonances enhancement, the optimized device achieves remarkable performance metrics at zero bias: a photoresponsivity of 200 mA/W, a specific detectivity of 1.65 × 1012 Jones as well as ultrafast response speed with rise/fall times of 400/540 μs under 254 nm illumination, surpassing the majority of its competitors. The unencapsulated detector exhibits robust thermal-humidity stability under ambient conditions, demonstrating exceptional reliability. A prototype light-intensity monitoring system, integrating this PtNPs@CsCu2I3/AlGaN vdWh detector with customized signal processing circuitry, demonstrates exceptional measurement accuracy with absolute error < 5.0 μ W/cm2 and relative error < 5.0%, respectively. This work develops high-performance solar-blind ultraviolet photodetectors using eco-friendly lead-free perovskites with tailored interfaces, and establishes an integration framework bridging these devices to deep-ultraviolet photonics and radiation-resistant applications.
期刊介绍:
Applied Physics Letters (APL) features concise, up-to-date reports on significant new findings in applied physics. Emphasizing rapid dissemination of key data and new physical insights, APL offers prompt publication of new experimental and theoretical papers reporting applications of physics phenomena to all branches of science, engineering, and modern technology.
In addition to regular articles, the journal also publishes invited Fast Track, Perspectives, and in-depth Editorials which report on cutting-edge areas in applied physics.
APL Perspectives are forward-looking invited letters which highlight recent developments or discoveries. Emphasis is placed on very recent developments, potentially disruptive technologies, open questions and possible solutions. They also include a mini-roadmap detailing where the community should direct efforts in order for the phenomena to be viable for application and the challenges associated with meeting that performance threshold. Perspectives are characterized by personal viewpoints and opinions of recognized experts in the field.
Fast Track articles are invited original research articles that report results that are particularly novel and important or provide a significant advancement in an emerging field. Because of the urgency and scientific importance of the work, the peer review process is accelerated. If, during the review process, it becomes apparent that the paper does not meet the Fast Track criterion, it is returned to a normal track.