掺hf异质层结构in - zn - o tft中交流漏偏置稳定性的改善。

IF 8.2 2区 材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY
Hyunjeong Doh, Hyeokjun You, Hwijoong Kim, Minki Son, Sejoong Kim, Dongil Ho*, Sihyun Kim* and Choongik Kim*, 
{"title":"掺hf异质层结构in - zn - o tft中交流漏偏置稳定性的改善。","authors":"Hyunjeong Doh,&nbsp;Hyeokjun You,&nbsp;Hwijoong Kim,&nbsp;Minki Son,&nbsp;Sejoong Kim,&nbsp;Dongil Ho*,&nbsp;Sihyun Kim* and Choongik Kim*,&nbsp;","doi":"10.1021/acsami.5c05480","DOIUrl":null,"url":null,"abstract":"<p >Metal oxide semiconductors are widely used in display technologies due to their high electron mobility, low leakage current, and robust switching characteristics. However, ensuring stability under AC bias stress, which is an inherent condition for practical device operation, remains a critical challenge. In particular, hot carrier effects (HCE) have been identified as a key mechanism for device instability under AC bias stress, as they induce oxygen vacancies (V<sub>O</sub>) and acceptor-like defect states. In this study, we selected IZO, a material with excellent properties but weak M–O bonds, to improve AC stability. To address this challenge, we propose a heterobilayer channel thin-film transistor (TFT) consisting of an indium–zinc oxide (IZO) bottom layer and a Hf-doped IZO top layer as a solution to enhance AC bias stability as well as electron mobility. The Hf-doped IZO top layer forms strong bonds with oxygen, effectively reducing oxygen vacancies and V<sub>O</sub>-related defect states, while inhibiting excessive hot carrier accumulation near the drain electrode. Meanwhile, the IZO bottom layer provides an abundance of oxygen vacancies, contributing to enhanced mobility. The fabricated TFT with the IZO:Hf/IZO bilayer channel exhibits a mobility of 7.3 cm<sup>2</sup>/(V s) and an <i>I</i><sub>on</sub> degradation rate of only 4% after 1000 s, demonstrating excellent device stability under AC drain bias stress. In addition, negligible hysteresis and excellent reproducibility were also achieved even under AC bias conditions. After stress, the threshold voltage shift was only 0.11 V, with a current on/off ratio of 1.8 × 10<sup>6</sup> and a subthreshold swing of 512 mV/dec. TCAD simulations further validated the heterobilayer structure in improving stability under AC drain bias stress by demonstrating its effectiveness in suppressing defect generation.</p>","PeriodicalId":5,"journal":{"name":"ACS Applied Materials & Interfaces","volume":"17 28","pages":"40662–40672"},"PeriodicalIF":8.2000,"publicationDate":"2025-07-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Improved AC Drain Bias Stability in In–Zn–O TFTs with an Hf-Doped Heterobilayer Structure\",\"authors\":\"Hyunjeong Doh,&nbsp;Hyeokjun You,&nbsp;Hwijoong Kim,&nbsp;Minki Son,&nbsp;Sejoong Kim,&nbsp;Dongil Ho*,&nbsp;Sihyun Kim* and Choongik Kim*,&nbsp;\",\"doi\":\"10.1021/acsami.5c05480\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p >Metal oxide semiconductors are widely used in display technologies due to their high electron mobility, low leakage current, and robust switching characteristics. However, ensuring stability under AC bias stress, which is an inherent condition for practical device operation, remains a critical challenge. In particular, hot carrier effects (HCE) have been identified as a key mechanism for device instability under AC bias stress, as they induce oxygen vacancies (V<sub>O</sub>) and acceptor-like defect states. In this study, we selected IZO, a material with excellent properties but weak M–O bonds, to improve AC stability. To address this challenge, we propose a heterobilayer channel thin-film transistor (TFT) consisting of an indium–zinc oxide (IZO) bottom layer and a Hf-doped IZO top layer as a solution to enhance AC bias stability as well as electron mobility. The Hf-doped IZO top layer forms strong bonds with oxygen, effectively reducing oxygen vacancies and V<sub>O</sub>-related defect states, while inhibiting excessive hot carrier accumulation near the drain electrode. Meanwhile, the IZO bottom layer provides an abundance of oxygen vacancies, contributing to enhanced mobility. The fabricated TFT with the IZO:Hf/IZO bilayer channel exhibits a mobility of 7.3 cm<sup>2</sup>/(V s) and an <i>I</i><sub>on</sub> degradation rate of only 4% after 1000 s, demonstrating excellent device stability under AC drain bias stress. In addition, negligible hysteresis and excellent reproducibility were also achieved even under AC bias conditions. After stress, the threshold voltage shift was only 0.11 V, with a current on/off ratio of 1.8 × 10<sup>6</sup> and a subthreshold swing of 512 mV/dec. TCAD simulations further validated the heterobilayer structure in improving stability under AC drain bias stress by demonstrating its effectiveness in suppressing defect generation.</p>\",\"PeriodicalId\":5,\"journal\":{\"name\":\"ACS Applied Materials & Interfaces\",\"volume\":\"17 28\",\"pages\":\"40662–40672\"},\"PeriodicalIF\":8.2000,\"publicationDate\":\"2025-07-03\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"ACS Applied Materials & Interfaces\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://pubs.acs.org/doi/10.1021/acsami.5c05480\",\"RegionNum\":2,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"MATERIALS SCIENCE, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"ACS Applied Materials & Interfaces","FirstCategoryId":"88","ListUrlMain":"https://pubs.acs.org/doi/10.1021/acsami.5c05480","RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"MATERIALS SCIENCE, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0

摘要

金属氧化物半导体由于其高电子迁移率、低漏电流和强大的开关特性而广泛应用于显示技术中。然而,确保在交流偏置应力下的稳定性,这是实际设备运行的固有条件,仍然是一个关键的挑战。特别是,热载子效应(HCE)已被确定为交流偏压下器件不稳定的关键机制,因为它们诱导氧空位(VO)和受体样缺陷态。在本研究中,我们选择了一种性能优异但M-O键较弱的材料IZO来提高交流稳定性。为了解决这一挑战,我们提出了一种由铟氧化锌(IZO)底层和hf掺杂IZO顶层组成的异质层通道薄膜晶体管(TFT),作为提高交流偏置稳定性和电子迁移率的解决方案。掺hf的IZO顶层与氧形成强键,有效地减少了氧空位和vo相关的缺陷状态,同时抑制了漏极附近过多的热载子积累。同时,IZO底层提供了丰富的氧空位,有助于增强流动性。具有IZO:Hf/IZO双层通道的TFT在1000 s后的迁移率为7.3 cm2/(V s),离子降解率仅为4%,在交流漏极偏置应力下表现出优异的器件稳定性。此外,即使在交流偏压条件下,也可以实现可忽略的滞后和良好的再现性。应力后的阈值电压位移仅为0.11 V,电流开/关比为1.8 × 106,亚阈值摆幅为512 mV/dec。TCAD仿真进一步验证了异质层结构在抑制缺陷产生方面的有效性,从而提高了交流漏极偏置应力下的稳定性。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Improved AC Drain Bias Stability in In–Zn–O TFTs with an Hf-Doped Heterobilayer Structure

Improved AC Drain Bias Stability in In–Zn–O TFTs with an Hf-Doped Heterobilayer Structure

Metal oxide semiconductors are widely used in display technologies due to their high electron mobility, low leakage current, and robust switching characteristics. However, ensuring stability under AC bias stress, which is an inherent condition for practical device operation, remains a critical challenge. In particular, hot carrier effects (HCE) have been identified as a key mechanism for device instability under AC bias stress, as they induce oxygen vacancies (VO) and acceptor-like defect states. In this study, we selected IZO, a material with excellent properties but weak M–O bonds, to improve AC stability. To address this challenge, we propose a heterobilayer channel thin-film transistor (TFT) consisting of an indium–zinc oxide (IZO) bottom layer and a Hf-doped IZO top layer as a solution to enhance AC bias stability as well as electron mobility. The Hf-doped IZO top layer forms strong bonds with oxygen, effectively reducing oxygen vacancies and VO-related defect states, while inhibiting excessive hot carrier accumulation near the drain electrode. Meanwhile, the IZO bottom layer provides an abundance of oxygen vacancies, contributing to enhanced mobility. The fabricated TFT with the IZO:Hf/IZO bilayer channel exhibits a mobility of 7.3 cm2/(V s) and an Ion degradation rate of only 4% after 1000 s, demonstrating excellent device stability under AC drain bias stress. In addition, negligible hysteresis and excellent reproducibility were also achieved even under AC bias conditions. After stress, the threshold voltage shift was only 0.11 V, with a current on/off ratio of 1.8 × 106 and a subthreshold swing of 512 mV/dec. TCAD simulations further validated the heterobilayer structure in improving stability under AC drain bias stress by demonstrating its effectiveness in suppressing defect generation.

求助全文
通过发布文献求助,成功后即可免费获取论文全文。 去求助
来源期刊
ACS Applied Materials & Interfaces
ACS Applied Materials & Interfaces 工程技术-材料科学:综合
CiteScore
16.00
自引率
6.30%
发文量
4978
审稿时长
1.8 months
期刊介绍: ACS Applied Materials & Interfaces is a leading interdisciplinary journal that brings together chemists, engineers, physicists, and biologists to explore the development and utilization of newly-discovered materials and interfacial processes for specific applications. Our journal has experienced remarkable growth since its establishment in 2009, both in terms of the number of articles published and the impact of the research showcased. We are proud to foster a truly global community, with the majority of published articles originating from outside the United States, reflecting the rapid growth of applied research worldwide.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
确定
请完成安全验证×
copy
已复制链接
快去分享给好友吧!
我知道了
右上角分享
点击右上角分享
0
联系我们:info@booksci.cn Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。 Copyright © 2023 布克学术 All rights reserved.
京ICP备2023020795号-1
ghs 京公网安备 11010802042870号
Book学术文献互助
Book学术文献互助群
群 号:604180095
Book学术官方微信