用于高性能自供电硅基异质结光电探测器的CdS和au修饰CdS纳米颗粒的强脉冲光退火

IF 4.6 3区 化学 Q2 CHEMISTRY, MULTIDISCIPLINARY
RSC Advances Pub Date : 2025-07-04 DOI:10.1039/D5RA04075B
Hadeel F. Abbas, Raid A. Ismail, Walid K. Hamoudi and Mayyadah H. Mohsin
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引用次数: 0

摘要

纳米结构异质结硅光电探测器可见光响应性的提高引起了广泛的研究兴趣。本文采用强脉冲光(IPL)退火技术提高了激光烧蚀制备的CdS/Si和au修饰CdS/Si光电探测器的性能。x射线衍射(XRD)证实,经过IPL退火后,CdS和au修饰的CdS的结晶度都有了很大的改善。经退火后,CdS的粒径从78 nm增加到100 nm, au修饰CdS的粒径从10 nm增加到15 nm。退火后cd和au修饰cd的迁移率提高。退火后CdS的光能隙由2.55 eV增大到2.68 eV。退火后的CdS纳米粒子的光致发光研究表明,在450nm处存在一个强烈的单峰。结构和光学分析表明,IPL退火减少了缺陷并扩大了耗尽层宽度,使得CdS/Si在520 nm处的响应率从0.19增加到0.36 a W−1,而au修饰的CdS/Si在460 nm处的响应率从0.23增加到0.42 a W−1。结果表明,IPL退火是快速优化的异质结光电探测器。在光照下构造了au修饰的CdS/Si退火后的能带图。研究了老化时间对光电探测器性能的影响。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Intense pulsed light annealing of CdS and Au-decorated CdS nanoparticles for high-performance, self-powered silicon-based heterojunction photodetectors

Intense pulsed light annealing of CdS and Au-decorated CdS nanoparticles for high-performance, self-powered silicon-based heterojunction photodetectors

The enhancement of visible light responsivity in nanostructured heterojunction silicon photodetectors has attracted significant research interest. In this work, intense pulsed light (IPL) annealing was employed to improve the performance of CdS/Si and Au-decorated CdS/Si photodetectors fabricated via laser ablation. X-ray diffraction (XRD) confirms a substantial improvement in crystallinity of both CdS and Au-decorated CdS after IPL annealing. The particle size of the CdS increased from 78 to 100 nm and from 10 to 15 nm for Au-decorated CdS after annealing. The mobility of the CdS and Au-decorated CdS increases after annealing. The optical energy gap of CdS increases from 2.55 to 2.68 eV after annealing. Photoluminescence studies of CdS nanoparticles after annealing show the presence of an intense single peak at 450 nm. Structural and optical analyses reveal that IPL annealing reduced defects and enlarged the depletion layer width, giving a twofold responsivity increase from 0.19 to 0.36 A W−1 at 520 nm for CdS/Si and 0.23 to 0.42 A W−1 at 460 nm for Au-decorated CdS/Si. The obtained results indicated that IPL annealing was rapid and optimized heterojunction photodetectors. The energy band diagram of Au-decorated CdS/Si after annealing was constructed under illumination. The effect of aging time on the performance of the fabricated photodetectors was investigated.

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来源期刊
RSC Advances
RSC Advances chemical sciences-
CiteScore
7.50
自引率
2.60%
发文量
3116
审稿时长
1.6 months
期刊介绍: An international, peer-reviewed journal covering all of the chemical sciences, including multidisciplinary and emerging areas. RSC Advances is a gold open access journal allowing researchers free access to research articles, and offering an affordable open access publishing option for authors around the world.
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