{"title":"烧结温度对凝胶铸造PMNT陶瓷电性能的影响","authors":"Kamonphan Thaenprom , Pornsuda Bomlai , Kowit Lertwittayanon , Pimpilai Wannasut , Methee Promsawat","doi":"10.1016/j.matlet.2025.138999","DOIUrl":null,"url":null,"abstract":"<div><div>This study investigates effects of sintering temperature and dispersant on properties of Pb(Mg<sub>1/3</sub>Nb<sub>2/3</sub>)<sub>0.65</sub>Ti<sub>0.35</sub>O<sub>3</sub> (PMNT) ceramics formed by agar gel-casting method. Poly(acrylic acid sodium salt) was found to be an effective dispersant for casting PMNT ceramics. Gelcast PMNT green bodies were sintered at 1180, 1200, 1220, 1240 and 1260 °C. Pure perovskite structure is observed in all ceramics. The PMNT ceramics sintered at 1200 °C exhibit the best ferroelectric and piezoelectric properties. An optimum sintering temperature was subsequently used for sintering concave-shaped PMNT ceramics. Concave-shaped ceramics were subjected to applied impact force and corresponding output voltages were recorded. An exponential relation between output voltage and input impact force is observed. We believe that the obtained findings will promote more convenience for fabricating complex-shaped piezoelectric materials.</div></div>","PeriodicalId":384,"journal":{"name":"Materials Letters","volume":"399 ","pages":"Article 138999"},"PeriodicalIF":2.7000,"publicationDate":"2025-06-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Effects of sintering temperature on electrical properties of PMNT ceramics formed by gel-casting\",\"authors\":\"Kamonphan Thaenprom , Pornsuda Bomlai , Kowit Lertwittayanon , Pimpilai Wannasut , Methee Promsawat\",\"doi\":\"10.1016/j.matlet.2025.138999\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><div>This study investigates effects of sintering temperature and dispersant on properties of Pb(Mg<sub>1/3</sub>Nb<sub>2/3</sub>)<sub>0.65</sub>Ti<sub>0.35</sub>O<sub>3</sub> (PMNT) ceramics formed by agar gel-casting method. Poly(acrylic acid sodium salt) was found to be an effective dispersant for casting PMNT ceramics. Gelcast PMNT green bodies were sintered at 1180, 1200, 1220, 1240 and 1260 °C. Pure perovskite structure is observed in all ceramics. The PMNT ceramics sintered at 1200 °C exhibit the best ferroelectric and piezoelectric properties. An optimum sintering temperature was subsequently used for sintering concave-shaped PMNT ceramics. Concave-shaped ceramics were subjected to applied impact force and corresponding output voltages were recorded. An exponential relation between output voltage and input impact force is observed. We believe that the obtained findings will promote more convenience for fabricating complex-shaped piezoelectric materials.</div></div>\",\"PeriodicalId\":384,\"journal\":{\"name\":\"Materials Letters\",\"volume\":\"399 \",\"pages\":\"Article 138999\"},\"PeriodicalIF\":2.7000,\"publicationDate\":\"2025-06-29\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Materials Letters\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S0167577X25010286\",\"RegionNum\":4,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q3\",\"JCRName\":\"MATERIALS SCIENCE, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Materials Letters","FirstCategoryId":"88","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S0167577X25010286","RegionNum":4,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"MATERIALS SCIENCE, MULTIDISCIPLINARY","Score":null,"Total":0}
Effects of sintering temperature on electrical properties of PMNT ceramics formed by gel-casting
This study investigates effects of sintering temperature and dispersant on properties of Pb(Mg1/3Nb2/3)0.65Ti0.35O3 (PMNT) ceramics formed by agar gel-casting method. Poly(acrylic acid sodium salt) was found to be an effective dispersant for casting PMNT ceramics. Gelcast PMNT green bodies were sintered at 1180, 1200, 1220, 1240 and 1260 °C. Pure perovskite structure is observed in all ceramics. The PMNT ceramics sintered at 1200 °C exhibit the best ferroelectric and piezoelectric properties. An optimum sintering temperature was subsequently used for sintering concave-shaped PMNT ceramics. Concave-shaped ceramics were subjected to applied impact force and corresponding output voltages were recorded. An exponential relation between output voltage and input impact force is observed. We believe that the obtained findings will promote more convenience for fabricating complex-shaped piezoelectric materials.
期刊介绍:
Materials Letters has an open access mirror journal Materials Letters: X, sharing the same aims and scope, editorial team, submission system and rigorous peer review.
Materials Letters is dedicated to publishing novel, cutting edge reports of broad interest to the materials community. The journal provides a forum for materials scientists and engineers, physicists, and chemists to rapidly communicate on the most important topics in the field of materials.
Contributions include, but are not limited to, a variety of topics such as:
• Materials - Metals and alloys, amorphous solids, ceramics, composites, polymers, semiconductors
• Applications - Structural, opto-electronic, magnetic, medical, MEMS, sensors, smart
• Characterization - Analytical, microscopy, scanning probes, nanoscopic, optical, electrical, magnetic, acoustic, spectroscopic, diffraction
• Novel Materials - Micro and nanostructures (nanowires, nanotubes, nanoparticles), nanocomposites, thin films, superlattices, quantum dots.
• Processing - Crystal growth, thin film processing, sol-gel processing, mechanical processing, assembly, nanocrystalline processing.
• Properties - Mechanical, magnetic, optical, electrical, ferroelectric, thermal, interfacial, transport, thermodynamic
• Synthesis - Quenching, solid state, solidification, solution synthesis, vapor deposition, high pressure, explosive