用于保形柔性和可穿戴x射线探测和成像的全无机超织物闪烁体

IF 12.5 1区 综合性期刊 Q1 MULTIDISCIPLINARY SCIENCES
Science Advances Pub Date : 2025-06-27
Li Xu, Peng Ran, Wenqian Zhou, Yu Jia, Jianyong Yu, Yang (Michael) Yang, Yang Si
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引用次数: 0

摘要

传统的闪烁体依赖于具有高z元素的刚性无机基质,其机械不灵活性限制了其在多种情况下的应用。开发一种结合无机特性和柔韧性的高效闪烁体是一个理想但极具挑战性的目标。我们开创了一种无机超织物闪烁体范例,通过自我维持的滑动系统工程,将脆性的全无机闪烁材料转化为延展性的纺织结构,产生本质上共形的柔性闪烁体,无缝地粘附在复杂的曲面上。最终的全无机闪烁体提供了接近统一的量子产率,闪烁输出比以前基于聚合物基质的柔性闪烁体高10倍以上。利用这些超纤维闪烁体,开发了一种多模态x射线交互式可穿戴平台(X-Wear),并成功演示了其在以身体为中心的柔性检测与成像、移动健康、视觉辐射监测和可呼吸辐射屏蔽等方面的应用。这项工作为闪烁体系统设计策略提供了一个以前未定义的范例,该策略保持了无机闪烁体的高性能,同时增加了织物的保形灵活性和可穿戴性。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

All-inorganic metafabric scintillators for conformally flexible and wearable x-ray detection and imaging

All-inorganic metafabric scintillators for conformally flexible and wearable x-ray detection and imaging
Traditional scintillators rely on rigid inorganic matrices with high-Z elements, whose mechanical inflexibility restricts applications in multiple scenarios. Developing an efficient scintillator that combines inorganic properties with flexibility is a desirable yet highly challenging goal. We pioneered an inorganic metafabric scintillator paradigm through self-sustained slip system engineering, transforming brittle all-inorganic scintillation materials into ductile textile architectures, yielding intrinsically conformally flexible scintillators that adhere seamlessly to complex, curved surfaces. The ultimate all-inorganic scintillator delivers near-unity quantum yield, with scintillation output more than 10 times higher than that of previous polymer matrix–based flexible scintillators. Using these metafabric scintillators, a multimodal x-ray interactive wearable platform (X-Wear) was developed, and their applications in body-centered flexible detection and imaging, mobile health, visual radiation monitoring, and breathable radiation shielding were successfully demonstrated. This work offers a previously undefined paradigm for a scintillator system design strategy that maintains the high performance of inorganic scintillators while adding the functionality of being conformally flexible and wearable of fabrics.
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来源期刊
Science Advances
Science Advances 综合性期刊-综合性期刊
CiteScore
21.40
自引率
1.50%
发文量
1937
审稿时长
29 weeks
期刊介绍: Science Advances, an open-access journal by AAAS, publishes impactful research in diverse scientific areas. It aims for fair, fast, and expert peer review, providing freely accessible research to readers. Led by distinguished scientists, the journal supports AAAS's mission by extending Science magazine's capacity to identify and promote significant advances. Evolving digital publishing technologies play a crucial role in advancing AAAS's global mission for science communication and benefitting humankind.
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