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Extensive experiments reveal that incorporation of an N-terminal His-tag notably affects eAPN's aminopeptidase activity. This cost-effective recombinant eAPN exhibits favorable thermostability and optimal activity at pH 7.5. Kinetic analysis toward peptidase substrates reveals that eAPN preferentially cleaves peptides following amino acid residues in the order of Ala > Arg >> Met, Gly > Leu > Pro, indicating a preference for small or basic amino acid residues as substrates. Computational and experimental studies have, for the first time, discovered that eAPN is capable of catalyzing the hydrolysis of heroin and 6-MAM, which has shed light on its functional versatility and potential applications. 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引用次数: 0
摘要
6-单乙酰吗啡(6-MAM)是海洛因到达人脑的主要活性代谢物,在产生与海洛因相关的生理和致死效应方面起着至关重要的作用。因此,6-MAM已成为减轻海洛因滥用不良后果的关键目标。本研究重组制备了6-MAM水解酶大肠杆菌氨基肽酶N (E. coli aminopeptidase N, eAPN),并对其进行了生化和功能分析。研究了eAPN在pH、金属离子和温度方面的生化特性,以及对肽酶底物和6-MAM的催化功能。大量实验表明,n端His-tag的掺入显著影响eAPN的氨基肽酶活性。该重组eAPN在pH 7.5下具有良好的热稳定性和最佳活性。对肽酶底物的动力学分析表明,eAPN优先切割氨基酸残基顺序为Ala > Arg >> Met, Gly > Leu > Pro的肽,表明eAPN优先选择小氨基酸或碱性氨基酸残基作为底物。计算和实验研究首次发现eAPN能够催化海洛因和6-MAM的水解,揭示了其功能的通用性和潜在的应用前景。本研究阐明了eAPN的生化特性,拓展了其催化功能,为进一步深入了解和重组eAPN以增强其对6-MAM的脱毒活性奠定了基础。
Biochemical and Functional Characterization of E. coli Aminopeptidase N: A New Role as a 6-Monoacetylmorphine Hydrolase.
6-monoacetylmorphine (6-MAM), a primary active metabolite of heroin that reaches the human brain, plays a crucial role in producing heroin-associated physiological and lethal effects. Therefore, 6-MAM has emerged as a key target for alleviating the adverse consequences of heroin abuse. In this study, the proposed 6-MAM hydrolase E. coli aminopeptidase N (eAPN) was recombinantly produced, and its biochemical and functional profiles were investigated. eAPN's biochemical properties, with respect to pH, metal ions, and temperature, and catalytic functions toward peptidase substrates and 6-MAM were thoroughly examined. Extensive experiments reveal that incorporation of an N-terminal His-tag notably affects eAPN's aminopeptidase activity. This cost-effective recombinant eAPN exhibits favorable thermostability and optimal activity at pH 7.5. Kinetic analysis toward peptidase substrates reveals that eAPN preferentially cleaves peptides following amino acid residues in the order of Ala > Arg >> Met, Gly > Leu > Pro, indicating a preference for small or basic amino acid residues as substrates. Computational and experimental studies have, for the first time, discovered that eAPN is capable of catalyzing the hydrolysis of heroin and 6-MAM, which has shed light on its functional versatility and potential applications. This work elucidates the biochemical properties of eAPN and expands its catalytic functions, thereby laying the groundwork for a deep understanding and further reengineering of eAPN to enhance its activity toward 6-MAM for heroin detoxification.
BiomoleculesBiochemistry, Genetics and Molecular Biology-Molecular Biology
CiteScore
9.40
自引率
3.60%
发文量
1640
审稿时长
18.28 days
期刊介绍:
Biomolecules (ISSN 2218-273X) is an international, peer-reviewed open access journal focusing on biogenic substances and their biological functions, structures, interactions with other molecules, and their microenvironment as well as biological systems. Biomolecules publishes reviews, regular research papers and short communications. Our aim is to encourage scientists to publish their experimental and theoretical results in as much detail as possible. There is no restriction on the length of the papers. The full experimental details must be provided so that the results can be reproduced.