{"title":"3he粒子在27mev的天然银上诱导核反应的激活截面","authors":"B.M. Ali , A. Elbinawi , F. Ditrói , M. Al-Abyad","doi":"10.1016/j.apradiso.2025.112011","DOIUrl":null,"url":null,"abstract":"<div><div>This study presents new experimental cross-section data for the production of radionuclides <sup>104</sup>ᵐ, <sup>104g</sup>, <sup>105</sup>ᵐ, <sup>106</sup>ᵐ, <sup>110</sup>ᵐAg, <sup>107g</sup>, <sup>108</sup>ᵐ, <sup>108g</sup>, <sup>109</sup>, <sup>110</sup>ᵐ, <sup>110g</sup>, <sup>111</sup>In, and <sup>107</sup>, <sup>109</sup>Cd produced via <sup>3</sup>He-particle irradiation of natural silver using the stacked-foil activation technique. The results were validated by comparison with previous studies, corrected for updated γ-ray emissions, if possible. Beam energy and current were verified using the monitor reactions, which improved data reliability. The experimental excitation functions were further compared with theoretical predictions from the EMPIRE code and the TENDL-2023 library, revealing notable discrepancies that underscore the need for refinement in nuclear reaction models for ³He projectiles. Thick target yields were also calculated, with ¹⁰⁷ᵍIn and ¹⁰⁸ᵐIn showing the highest production rates. The yields are generally insufficient for large-scale radionuclide production. These results anyhow extend the existing experimental database for <sup>3</sup>He-induced nuclear reactions, contribute new material for the advancement of nuclear reaction modeling, as well as for applications in activation analysis and astrophysics.</div></div>","PeriodicalId":8096,"journal":{"name":"Applied Radiation and Isotopes","volume":"225 ","pages":"Article 112011"},"PeriodicalIF":1.8000,"publicationDate":"2025-06-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Activation cross-sections of 3He-particle induced nuclear reactions on natural silver up to 27 MeV\",\"authors\":\"B.M. Ali , A. Elbinawi , F. Ditrói , M. Al-Abyad\",\"doi\":\"10.1016/j.apradiso.2025.112011\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><div>This study presents new experimental cross-section data for the production of radionuclides <sup>104</sup>ᵐ, <sup>104g</sup>, <sup>105</sup>ᵐ, <sup>106</sup>ᵐ, <sup>110</sup>ᵐAg, <sup>107g</sup>, <sup>108</sup>ᵐ, <sup>108g</sup>, <sup>109</sup>, <sup>110</sup>ᵐ, <sup>110g</sup>, <sup>111</sup>In, and <sup>107</sup>, <sup>109</sup>Cd produced via <sup>3</sup>He-particle irradiation of natural silver using the stacked-foil activation technique. The results were validated by comparison with previous studies, corrected for updated γ-ray emissions, if possible. Beam energy and current were verified using the monitor reactions, which improved data reliability. The experimental excitation functions were further compared with theoretical predictions from the EMPIRE code and the TENDL-2023 library, revealing notable discrepancies that underscore the need for refinement in nuclear reaction models for ³He projectiles. Thick target yields were also calculated, with ¹⁰⁷ᵍIn and ¹⁰⁸ᵐIn showing the highest production rates. The yields are generally insufficient for large-scale radionuclide production. These results anyhow extend the existing experimental database for <sup>3</sup>He-induced nuclear reactions, contribute new material for the advancement of nuclear reaction modeling, as well as for applications in activation analysis and astrophysics.</div></div>\",\"PeriodicalId\":8096,\"journal\":{\"name\":\"Applied Radiation and Isotopes\",\"volume\":\"225 \",\"pages\":\"Article 112011\"},\"PeriodicalIF\":1.8000,\"publicationDate\":\"2025-06-24\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Applied Radiation and Isotopes\",\"FirstCategoryId\":\"5\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S0969804325003562\",\"RegionNum\":3,\"RegionCategory\":\"工程技术\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q3\",\"JCRName\":\"CHEMISTRY, INORGANIC & NUCLEAR\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Applied Radiation and Isotopes","FirstCategoryId":"5","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S0969804325003562","RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"CHEMISTRY, INORGANIC & NUCLEAR","Score":null,"Total":0}
Activation cross-sections of 3He-particle induced nuclear reactions on natural silver up to 27 MeV
This study presents new experimental cross-section data for the production of radionuclides 104ᵐ, 104g, 105ᵐ, 106ᵐ, 110ᵐAg, 107g, 108ᵐ, 108g, 109, 110ᵐ, 110g, 111In, and 107, 109Cd produced via 3He-particle irradiation of natural silver using the stacked-foil activation technique. The results were validated by comparison with previous studies, corrected for updated γ-ray emissions, if possible. Beam energy and current were verified using the monitor reactions, which improved data reliability. The experimental excitation functions were further compared with theoretical predictions from the EMPIRE code and the TENDL-2023 library, revealing notable discrepancies that underscore the need for refinement in nuclear reaction models for ³He projectiles. Thick target yields were also calculated, with ¹⁰⁷ᵍIn and ¹⁰⁸ᵐIn showing the highest production rates. The yields are generally insufficient for large-scale radionuclide production. These results anyhow extend the existing experimental database for 3He-induced nuclear reactions, contribute new material for the advancement of nuclear reaction modeling, as well as for applications in activation analysis and astrophysics.
期刊介绍:
Applied Radiation and Isotopes provides a high quality medium for the publication of substantial, original and scientific and technological papers on the development and peaceful application of nuclear, radiation and radionuclide techniques in chemistry, physics, biochemistry, biology, medicine, security, engineering and in the earth, planetary and environmental sciences, all including dosimetry. Nuclear techniques are defined in the broadest sense and both experimental and theoretical papers are welcome. They include the development and use of α- and β-particles, X-rays and γ-rays, neutrons and other nuclear particles and radiations from all sources, including radionuclides, synchrotron sources, cyclotrons and reactors and from the natural environment.
The journal aims to publish papers with significance to an international audience, containing substantial novelty and scientific impact. The Editors reserve the rights to reject, with or without external review, papers that do not meet these criteria.
Papers dealing with radiation processing, i.e., where radiation is used to bring about a biological, chemical or physical change in a material, should be directed to our sister journal Radiation Physics and Chemistry.