{"title":"日本农业土壤中放射性铯的土壤-土壤溶液分配系数的温度依赖性","authors":"Keiko Tagami, Shigeo Uchida","doi":"10.1016/j.jenvrad.2025.107743","DOIUrl":null,"url":null,"abstract":"<div><div>Radiocaesium mobility in 40 agricultural soil samples at different temperature conditions (4–30 °C) was studied by measuring the soil-soil solution distribution coefficient, <em>K</em><sub>d</sub> (L/kg). Comparison of <em>K</em><sub>d</sub> values obtained at 10 °C and at 30 °C indicated significant differences for 36 soil samples by the one-way ANOVA test (p < 0.05) with decreases in <em>K</em><sub>d</sub> values under the higher temperature condition. The <em>K</em><sub>d</sub> measurement at 4 °C was intended to minimize the soil microbial activity effect; the results were almost the same as those observed at 10 °C. From this result, it was difficult to identify the effect of microbial activity on the radiocaesium absorbability to the soil solid phase. The obtained data imply a possible seasonal change of <em>K</em><sub>d</sub> values in many types of soils, and the <em>K</em><sub>d</sub> change likely affects the radiocaesium release rate change from soil to river water during a year.</div></div>","PeriodicalId":15667,"journal":{"name":"Journal of environmental radioactivity","volume":"288 ","pages":"Article 107743"},"PeriodicalIF":2.1000,"publicationDate":"2025-06-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Temperature dependence on soil-soil solution distribution coefficient of radiocaesium in Japanese agricultural soils\",\"authors\":\"Keiko Tagami, Shigeo Uchida\",\"doi\":\"10.1016/j.jenvrad.2025.107743\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><div>Radiocaesium mobility in 40 agricultural soil samples at different temperature conditions (4–30 °C) was studied by measuring the soil-soil solution distribution coefficient, <em>K</em><sub>d</sub> (L/kg). Comparison of <em>K</em><sub>d</sub> values obtained at 10 °C and at 30 °C indicated significant differences for 36 soil samples by the one-way ANOVA test (p < 0.05) with decreases in <em>K</em><sub>d</sub> values under the higher temperature condition. The <em>K</em><sub>d</sub> measurement at 4 °C was intended to minimize the soil microbial activity effect; the results were almost the same as those observed at 10 °C. From this result, it was difficult to identify the effect of microbial activity on the radiocaesium absorbability to the soil solid phase. The obtained data imply a possible seasonal change of <em>K</em><sub>d</sub> values in many types of soils, and the <em>K</em><sub>d</sub> change likely affects the radiocaesium release rate change from soil to river water during a year.</div></div>\",\"PeriodicalId\":15667,\"journal\":{\"name\":\"Journal of environmental radioactivity\",\"volume\":\"288 \",\"pages\":\"Article 107743\"},\"PeriodicalIF\":2.1000,\"publicationDate\":\"2025-06-23\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Journal of environmental radioactivity\",\"FirstCategoryId\":\"93\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S0265931X25001304\",\"RegionNum\":3,\"RegionCategory\":\"环境科学与生态学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q3\",\"JCRName\":\"ENVIRONMENTAL SCIENCES\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Journal of environmental radioactivity","FirstCategoryId":"93","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S0265931X25001304","RegionNum":3,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"ENVIRONMENTAL SCIENCES","Score":null,"Total":0}
Temperature dependence on soil-soil solution distribution coefficient of radiocaesium in Japanese agricultural soils
Radiocaesium mobility in 40 agricultural soil samples at different temperature conditions (4–30 °C) was studied by measuring the soil-soil solution distribution coefficient, Kd (L/kg). Comparison of Kd values obtained at 10 °C and at 30 °C indicated significant differences for 36 soil samples by the one-way ANOVA test (p < 0.05) with decreases in Kd values under the higher temperature condition. The Kd measurement at 4 °C was intended to minimize the soil microbial activity effect; the results were almost the same as those observed at 10 °C. From this result, it was difficult to identify the effect of microbial activity on the radiocaesium absorbability to the soil solid phase. The obtained data imply a possible seasonal change of Kd values in many types of soils, and the Kd change likely affects the radiocaesium release rate change from soil to river water during a year.
期刊介绍:
The Journal of Environmental Radioactivity provides a coherent international forum for publication of original research or review papers on any aspect of the occurrence of radioactivity in natural systems.
Relevant subject areas range from applications of environmental radionuclides as mechanistic or timescale tracers of natural processes to assessments of the radioecological or radiological effects of ambient radioactivity. Papers deal with naturally occurring nuclides or with those created and released by man through nuclear weapons manufacture and testing, energy production, fuel-cycle technology, etc. Reports on radioactivity in the oceans, sediments, rivers, lakes, groundwaters, soils, atmosphere and all divisions of the biosphere are welcomed, but these should not simply be of a monitoring nature unless the data are particularly innovative.