Gengliang Zou, Tao Liu, Chunlan Wang, Chi Luo, Zihan Qin, Jiaying Ji and Zao Yi
{"title":"电偶极谐振驱动的广角动态可调谐太赫兹宽带吸收器","authors":"Gengliang Zou, Tao Liu, Chunlan Wang, Chi Luo, Zihan Qin, Jiaying Ji and Zao Yi","doi":"10.1039/D5DT01258A","DOIUrl":null,"url":null,"abstract":"<p >To address the challenges of limited bandwidth and structural complexity in terahertz absorbers, this study proposes a vanadium dioxide (VO<small><sub>2</sub></small>)-based broadband terahertz (THz) absorber driven by electric dipole resonance. The device achieves broadband absorption exceeding 90% within 3.55–9.95 THz, an absorption bandwidth of 6.4 THz and a fractional bandwidth reaching 94.81%. Through comprehensive analyses including impedance matching theory, multiple reflection interference theory, multipole decomposition, and electric field distribution, we confirm that the broadband absorption mechanism originates from electric dipole resonances excited at the structural edges of VO<small><sub>2</sub></small>. Furthermore, the temperature-controlled phase transition properties of VO<small><sub>2</sub></small> enable dynamic tuning capability. The devices exhibit excellent polarization insensitivity and wide-angle stability with a synergistic effect of structural symmetry and slit design, and maintain efficient broad absorption at 40° incidence. Finally, the devices were found to have good process tolerance by varying different structural parameters. This work provides a high-performance and integration-friendly solution for THz metamaterial absorbers, showing significant application potential in electromagnetic shielding, smart switching, and wavefront modulation.</p>","PeriodicalId":71,"journal":{"name":"Dalton Transactions","volume":" 28","pages":" 10898-10906"},"PeriodicalIF":3.3000,"publicationDate":"2025-06-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Electric dipole resonance-driven terahertz broadband absorber with wide-angle and dynamic tunability\",\"authors\":\"Gengliang Zou, Tao Liu, Chunlan Wang, Chi Luo, Zihan Qin, Jiaying Ji and Zao Yi\",\"doi\":\"10.1039/D5DT01258A\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p >To address the challenges of limited bandwidth and structural complexity in terahertz absorbers, this study proposes a vanadium dioxide (VO<small><sub>2</sub></small>)-based broadband terahertz (THz) absorber driven by electric dipole resonance. The device achieves broadband absorption exceeding 90% within 3.55–9.95 THz, an absorption bandwidth of 6.4 THz and a fractional bandwidth reaching 94.81%. Through comprehensive analyses including impedance matching theory, multiple reflection interference theory, multipole decomposition, and electric field distribution, we confirm that the broadband absorption mechanism originates from electric dipole resonances excited at the structural edges of VO<small><sub>2</sub></small>. Furthermore, the temperature-controlled phase transition properties of VO<small><sub>2</sub></small> enable dynamic tuning capability. The devices exhibit excellent polarization insensitivity and wide-angle stability with a synergistic effect of structural symmetry and slit design, and maintain efficient broad absorption at 40° incidence. Finally, the devices were found to have good process tolerance by varying different structural parameters. This work provides a high-performance and integration-friendly solution for THz metamaterial absorbers, showing significant application potential in electromagnetic shielding, smart switching, and wavefront modulation.</p>\",\"PeriodicalId\":71,\"journal\":{\"name\":\"Dalton Transactions\",\"volume\":\" 28\",\"pages\":\" 10898-10906\"},\"PeriodicalIF\":3.3000,\"publicationDate\":\"2025-06-23\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Dalton Transactions\",\"FirstCategoryId\":\"92\",\"ListUrlMain\":\"https://pubs.rsc.org/en/content/articlelanding/2025/dt/d5dt01258a\",\"RegionNum\":3,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"CHEMISTRY, INORGANIC & NUCLEAR\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Dalton Transactions","FirstCategoryId":"92","ListUrlMain":"https://pubs.rsc.org/en/content/articlelanding/2025/dt/d5dt01258a","RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"CHEMISTRY, INORGANIC & NUCLEAR","Score":null,"Total":0}
Electric dipole resonance-driven terahertz broadband absorber with wide-angle and dynamic tunability
To address the challenges of limited bandwidth and structural complexity in terahertz absorbers, this study proposes a vanadium dioxide (VO2)-based broadband terahertz (THz) absorber driven by electric dipole resonance. The device achieves broadband absorption exceeding 90% within 3.55–9.95 THz, an absorption bandwidth of 6.4 THz and a fractional bandwidth reaching 94.81%. Through comprehensive analyses including impedance matching theory, multiple reflection interference theory, multipole decomposition, and electric field distribution, we confirm that the broadband absorption mechanism originates from electric dipole resonances excited at the structural edges of VO2. Furthermore, the temperature-controlled phase transition properties of VO2 enable dynamic tuning capability. The devices exhibit excellent polarization insensitivity and wide-angle stability with a synergistic effect of structural symmetry and slit design, and maintain efficient broad absorption at 40° incidence. Finally, the devices were found to have good process tolerance by varying different structural parameters. This work provides a high-performance and integration-friendly solution for THz metamaterial absorbers, showing significant application potential in electromagnetic shielding, smart switching, and wavefront modulation.
期刊介绍:
Dalton Transactions is a journal for all areas of inorganic chemistry, which encompasses the organometallic, bioinorganic and materials chemistry of the elements, with applications including synthesis, catalysis, energy conversion/storage, electrical devices and medicine. Dalton Transactions welcomes high-quality, original submissions in all of these areas and more, where the advancement of knowledge in inorganic chemistry is significant.