微生物电化学制氢过渡金属基电催化剂的15年进展：从纳米设计到宏观应用

IF 36.3 1区材料科学 Q1 Engineering

Nano-Micro Letters Pub Date : 2025-06-18 DOI:10.1007/s40820-025-01781-6

Seyed Masoud Parsa, Zhijie Chen, Huu Hao Ngo, Wei Wei, Xinbo Zhang, Ying Liu, Bing-Jie Ni, Wenshan Guo

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引用次数: 0

摘要

设计高性能电催化剂是微生物电化学制氢技术发展的关键挑战之一。过渡金属基（TM-based）电催化剂分别解决了贵金属和无金属电催化剂的高成本和低性能等缺点，成为未来催化剂的一个令人惊讶的替代方案。在这篇批判性的综述中，从微生物电解电池的发展开始，全面分析了过去15年来所有家族的tm基催化剂的主要发展。重要的是，重点突出和比较了关键的设计参数，如根据材料类型选择有效的合成方法，每种合成方法的主要标准，以及各种程序的优缺点。此外，还提出了调整和裁剪结构的方法、促进活性位点的先进策略以及实现新型未开发的基于tm的混合结构的潜力。此外，还重点讨论了未来大规模生产中基于tm的催化剂的大规模应用，包括生命周期评估、成本评估、经济分析以及最近的中试研究。重要的是，利用人工智能和先进的计算方法，如主动学习、微动力学建模和物理信息机器学习，在设计高性能电极的成功实践中具有潜力。最后，提出了未来研究的概念框架和微生物电解电池中基于tm的电催化剂的不同方面的挑战。

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15 Years of Progress on Transition Metal-Based Electrocatalysts for Microbial Electrochemical Hydrogen Production: From Nanoscale Design to Macroscale Application

Highlights

Comprehensive overview of the evolution of transition metal-based catalysts in microbial electrolysis cells from their inception to the present.
Critical design parameters of catalysts evaluated from technical, economic, and sustainability perspectives.
A conceptual framework is proposed to address current challenges and guide future research based on literature best practices.

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来源期刊

Nano-Micro Letters NANOSCIENCE & NANOTECHNOLOGY-MATERIALS SCIENCE, MULTIDISCIPLINARY

CiteScore

32.60

自引率

4.90%

发文量

981

审稿时长

1.1 months

期刊介绍： Nano-Micro Letters is a peer-reviewed, international, interdisciplinary, and open-access journal published under the SpringerOpen brand. Nano-Micro Letters focuses on the science, experiments, engineering, technologies, and applications of nano- or microscale structures and systems in various fields such as physics, chemistry, biology, material science, and pharmacy.It also explores the expanding interfaces between these fields. Nano-Micro Letters particularly emphasizes the bottom-up approach in the length scale from nano to micro. This approach is crucial for achieving industrial applications in nanotechnology, as it involves the assembly, modification, and control of nanostructures on a microscale.