石油污染钻井岩屑作为油井固井添加剂的可持续回收利用

IF 7.3 1区 化学 Q1 CHEMISTRY, MULTIDISCIPLINARY
Chengwen Wang*, Wenjian Yue, Aipu Shi and Junyi Liu, 
{"title":"石油污染钻井岩屑作为油井固井添加剂的可持续回收利用","authors":"Chengwen Wang*,&nbsp;Wenjian Yue,&nbsp;Aipu Shi and Junyi Liu,&nbsp;","doi":"10.1021/acssuschemeng.5c03365","DOIUrl":null,"url":null,"abstract":"<p >With the increasing exploitation of conventional oil/gas and large-scale shale gas development, the effective management of oil-contaminated solid waste from formations has become a major challenge. Conventional treatment methods for oil-contaminated drill cuttings (OCDCs) have several limitations, including high equipment costs, substantial energy consumption, and difficulties in controlling secondary pollution. This study proposes an innovative in situ recycling approach that repurposes the OCDC as a cement-based oil-contaminated cutting additive (OCCA), enabling low-energy consumption treatment at the contamination source and achieving waste valorization within a green closed loop system. Although unprocessed OCDC degrades cement integrity, amphiphilic surface modification of OCCA prevents agglomeration and enhances both dispersion and interfacial bonding, thereby improving the mechanical performance of the cement. Moreover, the use of OCCA significantly reduces the free heavy metal ion content in the set cement, effectively mitigating potential long-term environmental risks such as groundwater contamination from the cement sheath. The developed OCCA demonstrates excellent compatibility with cementing operations, fulfilling both mechanical and environmental requirements, and shows great potential in practical engineering applications.</p>","PeriodicalId":25,"journal":{"name":"ACS Sustainable Chemistry & Engineering","volume":"13 25","pages":"9819–9827"},"PeriodicalIF":7.3000,"publicationDate":"2025-06-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Sustainable Recycling of Oil-Contaminated Drilling Cuttings as Oil Well Cementing Additive\",\"authors\":\"Chengwen Wang*,&nbsp;Wenjian Yue,&nbsp;Aipu Shi and Junyi Liu,&nbsp;\",\"doi\":\"10.1021/acssuschemeng.5c03365\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p >With the increasing exploitation of conventional oil/gas and large-scale shale gas development, the effective management of oil-contaminated solid waste from formations has become a major challenge. Conventional treatment methods for oil-contaminated drill cuttings (OCDCs) have several limitations, including high equipment costs, substantial energy consumption, and difficulties in controlling secondary pollution. This study proposes an innovative in situ recycling approach that repurposes the OCDC as a cement-based oil-contaminated cutting additive (OCCA), enabling low-energy consumption treatment at the contamination source and achieving waste valorization within a green closed loop system. Although unprocessed OCDC degrades cement integrity, amphiphilic surface modification of OCCA prevents agglomeration and enhances both dispersion and interfacial bonding, thereby improving the mechanical performance of the cement. Moreover, the use of OCCA significantly reduces the free heavy metal ion content in the set cement, effectively mitigating potential long-term environmental risks such as groundwater contamination from the cement sheath. The developed OCCA demonstrates excellent compatibility with cementing operations, fulfilling both mechanical and environmental requirements, and shows great potential in practical engineering applications.</p>\",\"PeriodicalId\":25,\"journal\":{\"name\":\"ACS Sustainable Chemistry & Engineering\",\"volume\":\"13 25\",\"pages\":\"9819–9827\"},\"PeriodicalIF\":7.3000,\"publicationDate\":\"2025-06-15\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"ACS Sustainable Chemistry & Engineering\",\"FirstCategoryId\":\"92\",\"ListUrlMain\":\"https://pubs.acs.org/doi/10.1021/acssuschemeng.5c03365\",\"RegionNum\":1,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"CHEMISTRY, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"ACS Sustainable Chemistry & Engineering","FirstCategoryId":"92","ListUrlMain":"https://pubs.acs.org/doi/10.1021/acssuschemeng.5c03365","RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0

摘要

随着常规油气和页岩气开发规模的不断扩大,地层中含油固体废弃物的有效管理已成为一项重大挑战。常规的钻屑油污染处理方法存在设备成本高、能耗大、二次污染控制困难等诸多局限性。本研究提出了一种创新的原位回收方法,将OCDC重新用作水泥基油污染切削添加剂(OCCA),实现污染源的低能耗处理,并在绿色闭环系统中实现废物增值。虽然未经处理的OCDC会降低水泥的完整性,但OCCA的两亲性表面改性可以防止团聚,增强分散和界面结合,从而改善水泥的力学性能。此外,OCCA的使用显著降低了水泥凝块中的游离重金属离子含量,有效降低了水泥环对地下水污染等潜在的长期环境风险。开发的OCCA与固井作业具有良好的相容性,满足了机械和环境要求,在实际工程应用中具有很大的潜力。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Sustainable Recycling of Oil-Contaminated Drilling Cuttings as Oil Well Cementing Additive

Sustainable Recycling of Oil-Contaminated Drilling Cuttings as Oil Well Cementing Additive

Sustainable Recycling of Oil-Contaminated Drilling Cuttings as Oil Well Cementing Additive

With the increasing exploitation of conventional oil/gas and large-scale shale gas development, the effective management of oil-contaminated solid waste from formations has become a major challenge. Conventional treatment methods for oil-contaminated drill cuttings (OCDCs) have several limitations, including high equipment costs, substantial energy consumption, and difficulties in controlling secondary pollution. This study proposes an innovative in situ recycling approach that repurposes the OCDC as a cement-based oil-contaminated cutting additive (OCCA), enabling low-energy consumption treatment at the contamination source and achieving waste valorization within a green closed loop system. Although unprocessed OCDC degrades cement integrity, amphiphilic surface modification of OCCA prevents agglomeration and enhances both dispersion and interfacial bonding, thereby improving the mechanical performance of the cement. Moreover, the use of OCCA significantly reduces the free heavy metal ion content in the set cement, effectively mitigating potential long-term environmental risks such as groundwater contamination from the cement sheath. The developed OCCA demonstrates excellent compatibility with cementing operations, fulfilling both mechanical and environmental requirements, and shows great potential in practical engineering applications.

求助全文
通过发布文献求助,成功后即可免费获取论文全文。 去求助
来源期刊
ACS Sustainable Chemistry & Engineering
ACS Sustainable Chemistry & Engineering CHEMISTRY, MULTIDISCIPLINARY-ENGINEERING, CHEMICAL
CiteScore
13.80
自引率
4.80%
发文量
1470
审稿时长
1.7 months
期刊介绍: ACS Sustainable Chemistry & Engineering is a prestigious weekly peer-reviewed scientific journal published by the American Chemical Society. Dedicated to advancing the principles of green chemistry and green engineering, it covers a wide array of research topics including green chemistry, green engineering, biomass, alternative energy, and life cycle assessment. The journal welcomes submissions in various formats, including Letters, Articles, Features, and Perspectives (Reviews), that address the challenges of sustainability in the chemical enterprise and contribute to the advancement of sustainable practices. Join us in shaping the future of sustainable chemistry and engineering.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
确定
请完成安全验证×
copy
已复制链接
快去分享给好友吧!
我知道了
右上角分享
点击右上角分享
0
联系我们:info@booksci.cn Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。 Copyright © 2023 布克学术 All rights reserved.
京ICP备2023020795号-1
ghs 京公网安备 11010802042870号
Book学术文献互助
Book学术文献互助群
群 号:604180095
Book学术官方微信