基于氧化石墨烯涂层长周期光纤光栅的高灵敏度CO2传感器。

IF 4.3 3区 化学 Q2 CHEMISTRY, MULTIDISCIPLINARY
ACS Omega Pub Date : 2025-05-28 eCollection Date: 2025-06-10 DOI:10.1021/acsomega.5c00184
Anne C P Fernandes, Nayton C Vicentini, Matheus S Couto, Giovanni R Carvalho, Benjamin Fragneaud, Cristiano Legnani, Indhira O Maciel, Renato Luiz Faraco Filho, João Victor de Castro Nascimento, João Pedro Emanuel Ferreira, Felipe Barino, Diogo Coelho, Alexandre Bessa Dos Santos, Welber G Quirino
{"title":"基于氧化石墨烯涂层长周期光纤光栅的高灵敏度CO2传感器。","authors":"Anne C P Fernandes, Nayton C Vicentini, Matheus S Couto, Giovanni R Carvalho, Benjamin Fragneaud, Cristiano Legnani, Indhira O Maciel, Renato Luiz Faraco Filho, João Victor de Castro Nascimento, João Pedro Emanuel Ferreira, Felipe Barino, Diogo Coelho, Alexandre Bessa Dos Santos, Welber G Quirino","doi":"10.1021/acsomega.5c00184","DOIUrl":null,"url":null,"abstract":"<p><p>This study presents the development and characterization of a novel carbon dioxide (CO<sub>2</sub>) sensor based on graphene oxide (GO)-coated long-period fiber grating (LPFG). The structural and chemical properties of GO were analyzed using Raman spectroscopy and scanning electron microscopy (SEM), revealing a defective structure with a high degree of oxidation and significant surface roughness, which enhances gas adsorption capabilities, making it highly suitable for CO<sub>2</sub> detection. The sensor's performance was evaluated across CO<sub>2</sub> concentrations ranging from 5 to 65%. The operational principle of the sensor is based on changes in the resonance wavelength induced by variations in the refractive index of the GO coating as it interacts with CO<sub>2</sub> molecules. Results indicate a notable sensitivity of 0.0643 nm/% and low hysteresis during adsorption and desorption processes, affirming its stability and reliability. Additionally, the sensor demonstrated a strong linear fit of approximately 96% in adsorption and desorption cycles (5-65 and 65-5%). These findings underscore the significant potential of the GO-coated LPFG sensor for practical CO<sub>2</sub> sensing applications, offering advantages such as immunity to electromagnetic interference and ease of integration into remote sensing technologies.</p>","PeriodicalId":22,"journal":{"name":"ACS Omega","volume":"10 22","pages":"22874-22883"},"PeriodicalIF":4.3000,"publicationDate":"2025-05-28","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC12163766/pdf/","citationCount":"0","resultStr":"{\"title\":\"High-Sensitivity CO<sub>2</sub> Sensor Based on a Graphene Oxide Coated Long-Period Fiber Grating.\",\"authors\":\"Anne C P Fernandes, Nayton C Vicentini, Matheus S Couto, Giovanni R Carvalho, Benjamin Fragneaud, Cristiano Legnani, Indhira O Maciel, Renato Luiz Faraco Filho, João Victor de Castro Nascimento, João Pedro Emanuel Ferreira, Felipe Barino, Diogo Coelho, Alexandre Bessa Dos Santos, Welber G Quirino\",\"doi\":\"10.1021/acsomega.5c00184\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p><p>This study presents the development and characterization of a novel carbon dioxide (CO<sub>2</sub>) sensor based on graphene oxide (GO)-coated long-period fiber grating (LPFG). The structural and chemical properties of GO were analyzed using Raman spectroscopy and scanning electron microscopy (SEM), revealing a defective structure with a high degree of oxidation and significant surface roughness, which enhances gas adsorption capabilities, making it highly suitable for CO<sub>2</sub> detection. The sensor's performance was evaluated across CO<sub>2</sub> concentrations ranging from 5 to 65%. The operational principle of the sensor is based on changes in the resonance wavelength induced by variations in the refractive index of the GO coating as it interacts with CO<sub>2</sub> molecules. Results indicate a notable sensitivity of 0.0643 nm/% and low hysteresis during adsorption and desorption processes, affirming its stability and reliability. Additionally, the sensor demonstrated a strong linear fit of approximately 96% in adsorption and desorption cycles (5-65 and 65-5%). These findings underscore the significant potential of the GO-coated LPFG sensor for practical CO<sub>2</sub> sensing applications, offering advantages such as immunity to electromagnetic interference and ease of integration into remote sensing technologies.</p>\",\"PeriodicalId\":22,\"journal\":{\"name\":\"ACS Omega\",\"volume\":\"10 22\",\"pages\":\"22874-22883\"},\"PeriodicalIF\":4.3000,\"publicationDate\":\"2025-05-28\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC12163766/pdf/\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"ACS Omega\",\"FirstCategoryId\":\"92\",\"ListUrlMain\":\"https://doi.org/10.1021/acsomega.5c00184\",\"RegionNum\":3,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"2025/6/10 0:00:00\",\"PubModel\":\"eCollection\",\"JCR\":\"Q2\",\"JCRName\":\"CHEMISTRY, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"ACS Omega","FirstCategoryId":"92","ListUrlMain":"https://doi.org/10.1021/acsomega.5c00184","RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"2025/6/10 0:00:00","PubModel":"eCollection","JCR":"Q2","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0

摘要

本研究提出了一种基于氧化石墨烯(GO)涂层长周期光纤光栅(LPFG)的新型二氧化碳(CO2)传感器的开发和表征。利用拉曼光谱和扫描电子显微镜(SEM)对氧化石墨烯的结构和化学性质进行了分析,发现氧化石墨烯具有高度氧化和显著表面粗糙度的缺陷结构,增强了气体吸附能力,使其非常适合用于CO2检测。传感器的性能在二氧化碳浓度从5%到65%的范围内进行了评估。传感器的工作原理是基于氧化石墨烯涂层与二氧化碳分子相互作用时折射率的变化引起的共振波长的变化。结果表明,该方法的灵敏度为0.0643 nm/%,在吸附和解吸过程中具有较低的滞后,具有较好的稳定性和可靠性。此外,该传感器在吸附和解吸循环中表现出约96%的强线性拟合(5- 65%和65-5%)。这些发现强调了氧化石墨烯涂层LPFG传感器在实际二氧化碳传感应用中的巨大潜力,它具有抗电磁干扰和易于集成到遥感技术中的优势。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
High-Sensitivity CO2 Sensor Based on a Graphene Oxide Coated Long-Period Fiber Grating.

This study presents the development and characterization of a novel carbon dioxide (CO2) sensor based on graphene oxide (GO)-coated long-period fiber grating (LPFG). The structural and chemical properties of GO were analyzed using Raman spectroscopy and scanning electron microscopy (SEM), revealing a defective structure with a high degree of oxidation and significant surface roughness, which enhances gas adsorption capabilities, making it highly suitable for CO2 detection. The sensor's performance was evaluated across CO2 concentrations ranging from 5 to 65%. The operational principle of the sensor is based on changes in the resonance wavelength induced by variations in the refractive index of the GO coating as it interacts with CO2 molecules. Results indicate a notable sensitivity of 0.0643 nm/% and low hysteresis during adsorption and desorption processes, affirming its stability and reliability. Additionally, the sensor demonstrated a strong linear fit of approximately 96% in adsorption and desorption cycles (5-65 and 65-5%). These findings underscore the significant potential of the GO-coated LPFG sensor for practical CO2 sensing applications, offering advantages such as immunity to electromagnetic interference and ease of integration into remote sensing technologies.

求助全文
通过发布文献求助,成功后即可免费获取论文全文。 去求助
来源期刊
ACS Omega
ACS Omega Chemical Engineering-General Chemical Engineering
CiteScore
6.60
自引率
4.90%
发文量
3945
审稿时长
2.4 months
期刊介绍: ACS Omega is an open-access global publication for scientific articles that describe new findings in chemistry and interfacing areas of science, without any perceived evaluation of immediate impact.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
确定
请完成安全验证×
copy
已复制链接
快去分享给好友吧!
我知道了
右上角分享
点击右上角分享
0
联系我们:info@booksci.cn Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。 Copyright © 2023 布克学术 All rights reserved.
京ICP备2023020795号-1
ghs 京公网安备 11010802042870号
Book学术文献互助
Book学术文献互助群
群 号:604180095
Book学术官方微信