{"title":"松辽盆地青山口组页岩含油量与孔隙结构耦合演化——基于热模拟实验的启示","authors":"Xuening Qi, Lianjie Tian, Kun He, Zhichao Yu, Minghao Wu, Jing Zhao","doi":"10.1021/acsomega.5c00238","DOIUrl":null,"url":null,"abstract":"<p><p>Oil content estimation and pore characterization of shale are crucial for identifying sweet spots in shale plays. Despite extensive research, the correlation between retained hydrocarbon characteristics and pore evolution in shale with thermal maturity remains controversial. This study employs an integrated approach, combining thermal simulation experiments with multiple analytical techniques, to investigate organic geochemical characteristics and pore structure evolution across different maturity stages. The results demonstrate that thermal maturity plays a significant role in evolution and synergistic changes in oil content and pore characteristics. Within the optimal maturity of 1.20%-1.60%, shale has three key favorable characteristics: (1) elevated gas-to-oil ratios, (2) enhanced fluidity of retained hydrocarbons, and (3) well-developed pore networks that facilitate efficient hydrocarbon. Combined with the geological conditions of the Songliao Basin, we identify that the shale oil in the Gulong Depression with an optimal maturity range of 1.20%-1.60% is the most promising exploration target.</p>","PeriodicalId":22,"journal":{"name":"ACS Omega","volume":"10 22","pages":"22930-22943"},"PeriodicalIF":4.3000,"publicationDate":"2025-05-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC12163820/pdf/","citationCount":"0","resultStr":"{\"title\":\"Coupled Evolution of Oil Content and Pore Structure of the Qingshankou Formation Shale, Songliao Basin, Northeastern China: Insights from Thermal Simulation Experiments.\",\"authors\":\"Xuening Qi, Lianjie Tian, Kun He, Zhichao Yu, Minghao Wu, Jing Zhao\",\"doi\":\"10.1021/acsomega.5c00238\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p><p>Oil content estimation and pore characterization of shale are crucial for identifying sweet spots in shale plays. Despite extensive research, the correlation between retained hydrocarbon characteristics and pore evolution in shale with thermal maturity remains controversial. This study employs an integrated approach, combining thermal simulation experiments with multiple analytical techniques, to investigate organic geochemical characteristics and pore structure evolution across different maturity stages. The results demonstrate that thermal maturity plays a significant role in evolution and synergistic changes in oil content and pore characteristics. Within the optimal maturity of 1.20%-1.60%, shale has three key favorable characteristics: (1) elevated gas-to-oil ratios, (2) enhanced fluidity of retained hydrocarbons, and (3) well-developed pore networks that facilitate efficient hydrocarbon. Combined with the geological conditions of the Songliao Basin, we identify that the shale oil in the Gulong Depression with an optimal maturity range of 1.20%-1.60% is the most promising exploration target.</p>\",\"PeriodicalId\":22,\"journal\":{\"name\":\"ACS Omega\",\"volume\":\"10 22\",\"pages\":\"22930-22943\"},\"PeriodicalIF\":4.3000,\"publicationDate\":\"2025-05-29\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC12163820/pdf/\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"ACS Omega\",\"FirstCategoryId\":\"92\",\"ListUrlMain\":\"https://doi.org/10.1021/acsomega.5c00238\",\"RegionNum\":3,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"2025/6/10 0:00:00\",\"PubModel\":\"eCollection\",\"JCR\":\"Q2\",\"JCRName\":\"CHEMISTRY, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"ACS Omega","FirstCategoryId":"92","ListUrlMain":"https://doi.org/10.1021/acsomega.5c00238","RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"2025/6/10 0:00:00","PubModel":"eCollection","JCR":"Q2","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
Coupled Evolution of Oil Content and Pore Structure of the Qingshankou Formation Shale, Songliao Basin, Northeastern China: Insights from Thermal Simulation Experiments.
Oil content estimation and pore characterization of shale are crucial for identifying sweet spots in shale plays. Despite extensive research, the correlation between retained hydrocarbon characteristics and pore evolution in shale with thermal maturity remains controversial. This study employs an integrated approach, combining thermal simulation experiments with multiple analytical techniques, to investigate organic geochemical characteristics and pore structure evolution across different maturity stages. The results demonstrate that thermal maturity plays a significant role in evolution and synergistic changes in oil content and pore characteristics. Within the optimal maturity of 1.20%-1.60%, shale has three key favorable characteristics: (1) elevated gas-to-oil ratios, (2) enhanced fluidity of retained hydrocarbons, and (3) well-developed pore networks that facilitate efficient hydrocarbon. Combined with the geological conditions of the Songliao Basin, we identify that the shale oil in the Gulong Depression with an optimal maturity range of 1.20%-1.60% is the most promising exploration target.
ACS OmegaChemical Engineering-General Chemical Engineering
CiteScore
6.60
自引率
4.90%
发文量
3945
审稿时长
2.4 months
期刊介绍:
ACS Omega is an open-access global publication for scientific articles that describe new findings in chemistry and interfacing areas of science, without any perceived evaluation of immediate impact.