Luca Carpentieri, Thomas Mikolajick, Stefan Slesazeck
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Moreover, investigation of the polarization decay observed at different delay times after the writing reveals the direct correlation between the depolarization field and thickness scaling. Retention studies further indicate that tunneling current decay induced greater vulnerability to the On state, primarily attributed to the asymmetry of the stack structure, which results in imperfect screening of polarization charges. Our investigation into the scaling of ferroelectric thickness emphasizes its critical importance by examining both ferroelectric properties and device performance. These findings indicate that the optimization of FTJ for low operation voltage, long data retention, and high on-current density necessitates a coordinated optimization of the layer stack structure, establishing a direct relationship crucial for the future development of hafnia-based FTJ devices.</p>","PeriodicalId":3,"journal":{"name":"ACS Applied Electronic Materials","volume":"7 11","pages":"5008-5017"},"PeriodicalIF":4.7000,"publicationDate":"2025-05-26","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC12160526/pdf/","citationCount":"0","resultStr":"{\"title\":\"Effect of HZO Thickness Scaling in the Bilayer Ferroelectric Tunnel Junction.\",\"authors\":\"Luca Carpentieri, Thomas Mikolajick, Stefan Slesazeck\",\"doi\":\"10.1021/acsaelm.5c00469\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p><p>This study investigates the effects of ferroelectric thickness scaling in a bilayer-structured ferroelectric tunnel junction. It was found that both the remnant polarization and the transport mechanisms exhibit a correlation with the thickness of the ferroelectric film. While variations in ferroelectric thickness influence the tunneling current in the Off state, the magnitude of the remnant polarization significantly affects the current during the On state. Considering that the On-Off ratio serves as an important figure of merit, an analysis of the optimal memory window is provided, accounting for the impact of reading voltage and cycling conditions. Moreover, investigation of the polarization decay observed at different delay times after the writing reveals the direct correlation between the depolarization field and thickness scaling. Retention studies further indicate that tunneling current decay induced greater vulnerability to the On state, primarily attributed to the asymmetry of the stack structure, which results in imperfect screening of polarization charges. Our investigation into the scaling of ferroelectric thickness emphasizes its critical importance by examining both ferroelectric properties and device performance. These findings indicate that the optimization of FTJ for low operation voltage, long data retention, and high on-current density necessitates a coordinated optimization of the layer stack structure, establishing a direct relationship crucial for the future development of hafnia-based FTJ devices.</p>\",\"PeriodicalId\":3,\"journal\":{\"name\":\"ACS Applied Electronic Materials\",\"volume\":\"7 11\",\"pages\":\"5008-5017\"},\"PeriodicalIF\":4.7000,\"publicationDate\":\"2025-05-26\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC12160526/pdf/\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"ACS Applied Electronic Materials\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://doi.org/10.1021/acsaelm.5c00469\",\"RegionNum\":3,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"2025/6/10 0:00:00\",\"PubModel\":\"eCollection\",\"JCR\":\"Q1\",\"JCRName\":\"ENGINEERING, ELECTRICAL & ELECTRONIC\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"ACS Applied Electronic Materials","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1021/acsaelm.5c00469","RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"2025/6/10 0:00:00","PubModel":"eCollection","JCR":"Q1","JCRName":"ENGINEERING, ELECTRICAL & ELECTRONIC","Score":null,"Total":0}
Effect of HZO Thickness Scaling in the Bilayer Ferroelectric Tunnel Junction.
This study investigates the effects of ferroelectric thickness scaling in a bilayer-structured ferroelectric tunnel junction. It was found that both the remnant polarization and the transport mechanisms exhibit a correlation with the thickness of the ferroelectric film. While variations in ferroelectric thickness influence the tunneling current in the Off state, the magnitude of the remnant polarization significantly affects the current during the On state. Considering that the On-Off ratio serves as an important figure of merit, an analysis of the optimal memory window is provided, accounting for the impact of reading voltage and cycling conditions. Moreover, investigation of the polarization decay observed at different delay times after the writing reveals the direct correlation between the depolarization field and thickness scaling. Retention studies further indicate that tunneling current decay induced greater vulnerability to the On state, primarily attributed to the asymmetry of the stack structure, which results in imperfect screening of polarization charges. Our investigation into the scaling of ferroelectric thickness emphasizes its critical importance by examining both ferroelectric properties and device performance. These findings indicate that the optimization of FTJ for low operation voltage, long data retention, and high on-current density necessitates a coordinated optimization of the layer stack structure, establishing a direct relationship crucial for the future development of hafnia-based FTJ devices.
期刊介绍:
ACS Applied Electronic Materials is an interdisciplinary journal publishing original research covering all aspects of electronic materials. The journal is devoted to reports of new and original experimental and theoretical research of an applied nature that integrate knowledge in the areas of materials science, engineering, optics, physics, and chemistry into important applications of electronic materials. Sample research topics that span the journal's scope are inorganic, organic, ionic and polymeric materials with properties that include conducting, semiconducting, superconducting, insulating, dielectric, magnetic, optoelectronic, piezoelectric, ferroelectric and thermoelectric.
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