在热解过程中做出明智的决策:扭转塑料回收潮流的关键

IF 7.3 1区 化学 Q1 CHEMISTRY, MULTIDISCIPLINARY
Patritsia Maria Stathatou*, Elisavet Anglou, Yuchen Chang, Jacob Sweet, Arvind Ganesan, Natechanok Yutthasaksunthorn, Erin V. Phillips, Nikhita S. Ragam, Omar Isaac Asensio, Sankar Nair, Fani Boukouvala* and Carsten Sievers*, 
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引用次数: 0

摘要

塑料工业的迅速扩张带来了重大的环境挑战,促使人们探索替代回收方法。虽然机械回收有局限性,但化学回收,特别是热解,是一个很有前途的解决方案。然而,它在环境影响和经济可行性方面面临争议。从这个角度来看,我们分析了支持和反对塑料热解的观点,强调了对热解系统进行透明、全面和基于测量的生命周期评估(lca)的必要性,以为决策提供信息。我们还提出了一个关于美国热解衍生超低硫柴油(ULSD)温室气体(GHG)排放的文献报告案例研究,表明根据工厂产能和副产品分配方法,排放量可能比化石衍生超低硫柴油低28%至高30%。同样,当被视为一种废物管理策略时,塑料热解的温室气体净排放量可以比目前美国塑料废物管理实践低220%到高60%,具体取决于系统条件。这些发现强调了结果的可变性,以及对目前缺失的、健全的和情境化的lca的需求。最后,我们讨论了更广泛采用化学回收的监管和社会挑战与机遇,强调了公众支持在实现热解循环经济潜力方面的关键作用。需要对塑料热解的潜力和挑战进行全面的生命周期评估和利益相关者的参与。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Enabling Informed Decisions on Pyrolysis: A Key to Turn the Tide on Plastics Recycling

The rapid expansion of the plastic industry has led to significant environmental challenges, prompting the exploration of alternative recycling methods. While mechanical recycling has limitations, chemical recycling, particularly pyrolysis, presents a promising solution. However, it faces contention regarding its environmental impacts and economic feasibility. In this perspective, we analyze both supporting and opposing viewpoints of plastic pyrolysis, highlighting the need for transparent, comprehensive, and measurement-informed life cycle assessments (LCAs) of pyrolysis systems to inform decisions. We also present a case study of literature-reported greenhouse gas (GHG) emissions from pyrolysis-derived ultralow sulfur diesel (ULSD) in the United States, showing that depending on plant capacity and co-product allocation methods, emissions can range from 28% lower to 30% higher than fossil-derived ULSD. Similarly, when viewed as a waste management strategy, net GHG emissions from plastic pyrolysis can range from 220% lower to 60% higher than those from current U.S. plastic waste management practices, depending on system conditions. These findings underscore the variability of results and the need for currently missing, robust, and contextualized LCAs. Finally, we discuss regulatory and social challenges and opportunities for the wider adoption of chemical recycling, emphasizing the critical role of public support in realizing the potential of pyrolysis for a circular economy.

Thorough life cycle assessments and stakeholder engagement are needed for informed discussions of the potential and challenges of plastic pyrolysis.

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来源期刊
ACS Sustainable Chemistry & Engineering
ACS Sustainable Chemistry & Engineering CHEMISTRY, MULTIDISCIPLINARY-ENGINEERING, CHEMICAL
CiteScore
13.80
自引率
4.80%
发文量
1470
审稿时长
1.7 months
期刊介绍: ACS Sustainable Chemistry & Engineering is a prestigious weekly peer-reviewed scientific journal published by the American Chemical Society. Dedicated to advancing the principles of green chemistry and green engineering, it covers a wide array of research topics including green chemistry, green engineering, biomass, alternative energy, and life cycle assessment. The journal welcomes submissions in various formats, including Letters, Articles, Features, and Perspectives (Reviews), that address the challenges of sustainability in the chemical enterprise and contribute to the advancement of sustainable practices. Join us in shaping the future of sustainable chemistry and engineering.
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