Asako Shimada, Ko Hemmi, Saki Ohira, Yoshihisa Iida
{"title":"alps处理水中氚和其他低水平放射性核素的分析和定量。","authors":"Asako Shimada, Ko Hemmi, Saki Ohira, Yoshihisa Iida","doi":"10.1007/s44211-025-00803-y","DOIUrl":null,"url":null,"abstract":"<p><p>Advanced liquid processing system (ALPS)-treated water was sampled from the K4-B tank group on March 24, 2022, in the presence of staff from the International Atomic Energy Agency (IAEA) and Tokyo Electric Power Company (TEPCO) Holdings, Inc. The Nuclear Safety Research Center (NSRC) of the Japan Atomic Energy Agency analyzed ten key radionuclides (<sup>3</sup>H, <sup>14</sup>C, <sup>60</sup>Co, <sup>90</sup>Sr, <sup>99</sup>Tc, <sup>106</sup>Ru, <sup>125</sup>Sb, <sup>129</sup>I, <sup>134</sup>Cs, and <sup>137</sup>Cs) and three additional nuclides (<sup>36</sup>Cl, <sup>55</sup>Fe, and <sup>79</sup>Se) in the ALPS-treated water as part of independent monitoring for the regulatory body. According to the obtained results, all radionuclide concentrations, except that for the <sup>3</sup>H concentration, were ultralow and less than the standard values permitted for discharge. TEPCO's analytical results were evaluated using the En number, which indicated satisfactory performance. In addition, reference values and ζ scores obtained via the IAEA's interlaboratory comparisons were recalculated incorporating the NSRC's results. All ζ scores for NSRC, IAEA, and TEPCO fell between - 2 and 2, demonstrating that the results are acceptable at a 95.4% confidence level.</p>","PeriodicalId":7802,"journal":{"name":"Analytical Sciences","volume":" ","pages":""},"PeriodicalIF":1.8000,"publicationDate":"2025-06-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Analysis and quantification of tritium and other low-level radionuclides present in ALPS-treated water.\",\"authors\":\"Asako Shimada, Ko Hemmi, Saki Ohira, Yoshihisa Iida\",\"doi\":\"10.1007/s44211-025-00803-y\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p><p>Advanced liquid processing system (ALPS)-treated water was sampled from the K4-B tank group on March 24, 2022, in the presence of staff from the International Atomic Energy Agency (IAEA) and Tokyo Electric Power Company (TEPCO) Holdings, Inc. The Nuclear Safety Research Center (NSRC) of the Japan Atomic Energy Agency analyzed ten key radionuclides (<sup>3</sup>H, <sup>14</sup>C, <sup>60</sup>Co, <sup>90</sup>Sr, <sup>99</sup>Tc, <sup>106</sup>Ru, <sup>125</sup>Sb, <sup>129</sup>I, <sup>134</sup>Cs, and <sup>137</sup>Cs) and three additional nuclides (<sup>36</sup>Cl, <sup>55</sup>Fe, and <sup>79</sup>Se) in the ALPS-treated water as part of independent monitoring for the regulatory body. According to the obtained results, all radionuclide concentrations, except that for the <sup>3</sup>H concentration, were ultralow and less than the standard values permitted for discharge. TEPCO's analytical results were evaluated using the En number, which indicated satisfactory performance. In addition, reference values and ζ scores obtained via the IAEA's interlaboratory comparisons were recalculated incorporating the NSRC's results. All ζ scores for NSRC, IAEA, and TEPCO fell between - 2 and 2, demonstrating that the results are acceptable at a 95.4% confidence level.</p>\",\"PeriodicalId\":7802,\"journal\":{\"name\":\"Analytical Sciences\",\"volume\":\" \",\"pages\":\"\"},\"PeriodicalIF\":1.8000,\"publicationDate\":\"2025-06-13\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Analytical Sciences\",\"FirstCategoryId\":\"92\",\"ListUrlMain\":\"https://doi.org/10.1007/s44211-025-00803-y\",\"RegionNum\":4,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q3\",\"JCRName\":\"CHEMISTRY, ANALYTICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Analytical Sciences","FirstCategoryId":"92","ListUrlMain":"https://doi.org/10.1007/s44211-025-00803-y","RegionNum":4,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"CHEMISTRY, ANALYTICAL","Score":null,"Total":0}
Analysis and quantification of tritium and other low-level radionuclides present in ALPS-treated water.
Advanced liquid processing system (ALPS)-treated water was sampled from the K4-B tank group on March 24, 2022, in the presence of staff from the International Atomic Energy Agency (IAEA) and Tokyo Electric Power Company (TEPCO) Holdings, Inc. The Nuclear Safety Research Center (NSRC) of the Japan Atomic Energy Agency analyzed ten key radionuclides (3H, 14C, 60Co, 90Sr, 99Tc, 106Ru, 125Sb, 129I, 134Cs, and 137Cs) and three additional nuclides (36Cl, 55Fe, and 79Se) in the ALPS-treated water as part of independent monitoring for the regulatory body. According to the obtained results, all radionuclide concentrations, except that for the 3H concentration, were ultralow and less than the standard values permitted for discharge. TEPCO's analytical results were evaluated using the En number, which indicated satisfactory performance. In addition, reference values and ζ scores obtained via the IAEA's interlaboratory comparisons were recalculated incorporating the NSRC's results. All ζ scores for NSRC, IAEA, and TEPCO fell between - 2 and 2, demonstrating that the results are acceptable at a 95.4% confidence level.
期刊介绍:
Analytical Sciences is an international journal published monthly by The Japan Society for Analytical Chemistry. The journal publishes papers on all aspects of the theory and practice of analytical sciences, including fundamental and applied, inorganic and organic, wet chemical and instrumental methods.
This publication is supported in part by the Grant-in-Aid for Publication of Scientific Research Result of the Japanese Ministry of Education, Culture, Sports, Science and Technology.