电化学催化反应中的图灵结构催化剂

IF 4.2 2区 化学 Q2 CHEMISTRY, MULTIDISCIPLINARY
Lizhou Zhu , Sizhuo Feng , Longlu Wang , Jianmei Chen
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引用次数: 0

摘要

随着相工程的发展,精确的相控制已成为优化先进催化剂性能的关键策略。与传统的在纳米尺度有机材料上构建新相拓扑的方法相比,图灵结构催化剂(tsc)提供了一种独特的构建特殊相拓扑的方法,扩大了相工程的范围。因此,迫切需要系统地回顾tsc的最新进展。本文首先对TSCs的基本概念、反应扩散过程、合成方法和双边界效应等合成机理进行了综述。其次,介绍了tsc在电化学催化反应中的应用,如析氧/析氢反应、CO2还原反应和硫氧化反应。通过分析这些应用程序背后的复杂机制,我们为它们的系统实现提供了新的见解。最后,我们展望了tsc的潜力,旨在推动tsc在广泛的催化应用中取得重大突破,并为先进催化剂领域的精确相控制的进一步发展提供深刻的指导。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Turing-structured catalysts for electrochemical catalytic reactions

Turing-structured catalysts for electrochemical catalytic reactions
With the development of phase engineering, precise phase control has become a key strategy for optimizing the performance of advanced catalysts. Compared to the traditional method of constructing new phase topologies on nanoscale organic materials, Turing-structured catalysts (TSCs) provide a unique method for constructing special phase topologies, which expands the scope of phase engineering. Therefore, there is an urgent need to systematically review the recent advances of TSCs. In this review, we first provide a comprehensive discussion on the fundamental concepts of TSCs, including their synthesis mechanisms such as reaction–diffusion processes, synthesis methods and twin boundary effects. Next, we present the applications of TSCs in electrochemical catalytic reactions such as oxygen evolution reaction/hydrogen evolution reactions, CO2 reduction reactions and sulfur oxidation reactions. By analyzing the complex mechanisms behind these applications, we provide new insights for their systematic implementation. Finally, we look ahead to the potential of TSCs, aiming to drive major breakthroughs in a wide range of catalytic applications and offer profound guidance for the further development of precise phase control in the field of advanced catalysts.
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来源期刊
Chemical Communications
Chemical Communications 化学-化学综合
CiteScore
8.60
自引率
4.10%
发文量
2705
审稿时长
1.4 months
期刊介绍: ChemComm (Chemical Communications) is renowned as the fastest publisher of articles providing information on new avenues of research, drawn from all the world''s major areas of chemical research.
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