{"title":"界面上水合物形成和生长的分子机制研究进展","authors":"Anh Phan","doi":"10.1021/acs.energyfuels.5c00942","DOIUrl":null,"url":null,"abstract":"<p><p>Hydrate-based engineering applications hold significant promise due to their physical feasibility and low energy consumption. However, key challengesincluding operating conditions, formation and growth rates, and gas storage capacitycontinue to impact their viability as sustainable technologies. This mini-review offers key insights into molecular mechanisms governing hydrate nucleation and growth at guest-water interfaces, specifically examining the role of mass transfer thermodynamics across the interface in either promoting or inhibiting gas hydrate formation. Additionally, this review highlights recent advancements, emerging research opportunities, and potential commercialization pathways for these technologies. With continued development, technologies utilizing hydrates have the capability to play a transformative role across multiple industries, offering a more sustainable alternative to existing commercial solutions.</p>","PeriodicalId":35,"journal":{"name":"Energy & Fuels","volume":"39 22","pages":"10150-10164"},"PeriodicalIF":5.3000,"publicationDate":"2025-05-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC12147157/pdf/","citationCount":"0","resultStr":"{\"title\":\"Perspectives on Molecular Mechanisms of Hydrate Formation and Growth at Interfaces: A Mini-Review.\",\"authors\":\"Anh Phan\",\"doi\":\"10.1021/acs.energyfuels.5c00942\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p><p>Hydrate-based engineering applications hold significant promise due to their physical feasibility and low energy consumption. However, key challengesincluding operating conditions, formation and growth rates, and gas storage capacitycontinue to impact their viability as sustainable technologies. This mini-review offers key insights into molecular mechanisms governing hydrate nucleation and growth at guest-water interfaces, specifically examining the role of mass transfer thermodynamics across the interface in either promoting or inhibiting gas hydrate formation. Additionally, this review highlights recent advancements, emerging research opportunities, and potential commercialization pathways for these technologies. With continued development, technologies utilizing hydrates have the capability to play a transformative role across multiple industries, offering a more sustainable alternative to existing commercial solutions.</p>\",\"PeriodicalId\":35,\"journal\":{\"name\":\"Energy & Fuels\",\"volume\":\"39 22\",\"pages\":\"10150-10164\"},\"PeriodicalIF\":5.3000,\"publicationDate\":\"2025-05-08\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC12147157/pdf/\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Energy & Fuels\",\"FirstCategoryId\":\"5\",\"ListUrlMain\":\"https://doi.org/10.1021/acs.energyfuels.5c00942\",\"RegionNum\":3,\"RegionCategory\":\"工程技术\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"2025/6/5 0:00:00\",\"PubModel\":\"eCollection\",\"JCR\":\"Q2\",\"JCRName\":\"ENERGY & FUELS\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Energy & Fuels","FirstCategoryId":"5","ListUrlMain":"https://doi.org/10.1021/acs.energyfuels.5c00942","RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"2025/6/5 0:00:00","PubModel":"eCollection","JCR":"Q2","JCRName":"ENERGY & FUELS","Score":null,"Total":0}
Perspectives on Molecular Mechanisms of Hydrate Formation and Growth at Interfaces: A Mini-Review.
Hydrate-based engineering applications hold significant promise due to their physical feasibility and low energy consumption. However, key challengesincluding operating conditions, formation and growth rates, and gas storage capacitycontinue to impact their viability as sustainable technologies. This mini-review offers key insights into molecular mechanisms governing hydrate nucleation and growth at guest-water interfaces, specifically examining the role of mass transfer thermodynamics across the interface in either promoting or inhibiting gas hydrate formation. Additionally, this review highlights recent advancements, emerging research opportunities, and potential commercialization pathways for these technologies. With continued development, technologies utilizing hydrates have the capability to play a transformative role across multiple industries, offering a more sustainable alternative to existing commercial solutions.
期刊介绍：
Energy & Fuels publishes reports of research in the technical area defined by the intersection of the disciplines of chemistry and chemical engineering and the application domain of non-nuclear energy and fuels. This includes research directed at the formation of, exploration for, and production of fossil fuels and biomass; the properties and structure or molecular composition of both raw fuels and refined products; the chemistry involved in the processing and utilization of fuels; fuel cells and their applications; and the analytical and instrumental techniques used in investigations of the foregoing areas.
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