{"title":"Kagome反铁磁体中各向异性应变印迹电可切换标量自旋手性。","authors":"Debjoty Paul, Shivesh Yadav, Shikhar Gupta, Bikash Patra, Nilesh Kulkarni, Debashis Mondal, Kaushal Gavankar, Sourav K Sahu, Biswarup Satpati, Bahadur Singh, Owen Benton, Shouvik Chatterjee","doi":"10.1002/advs.202502569","DOIUrl":null,"url":null,"abstract":"<p><p>Topological chiral antiferromagnets, such as Mn<sub>3</sub>Sn, are emerging as promising materials for next-generation spintronic devices due to their intrinsic transport properties linked to exotic magnetic configurations. Here, it is demonstrated that anisotropic strain in Mn<sub>3</sub>Sn thin films offers a novel approach to manipulate the magnetic ground state, unlocking new functionalities in this material. Anisotropic strain reduces the point group symmetry of the manganese (Mn) Kagome triangles from C<sub>3v</sub> to C<sub>1</sub>, significantly altering the energy landscape of the magnetic states in Mn<sub>3</sub>Sn. This symmetry reduction enables even a tiny in-plane Dzyaloshinskii-Moriya (DM) interaction to induce canting of the Mn spins out of the Kagome plane. The modified magnetic ground state introduces a finite scalar spin chirality and results in a significant Berry phase in momentum space. Consequently, a large anomalous Hall effect emerges in the Kagome plane at room temperature - an effect that is absent in the bulk material. Moreover, this twofold degenerate magnetic state enables the creation of multiple-stable, non-volatile anomalous Hall resistance (AHR) memory states. These states are field-stable and can be controlled by thermal-assisted current-induced magnetization switching, requiring modest current densities and small bias fields, thereby offering a compelling new functionality in Mn<sub>3</sub>Sn for spintronic applications.</p>","PeriodicalId":117,"journal":{"name":"Advanced Science","volume":" ","pages":"e02569"},"PeriodicalIF":14.1000,"publicationDate":"2025-08-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC12362762/pdf/","citationCount":"0","resultStr":"{\"title\":\"Imprinting Electrically Switchable Scalar Spin Chirality by Anisotropic Strain in a Kagome Antiferromagnet.\",\"authors\":\"Debjoty Paul, Shivesh Yadav, Shikhar Gupta, Bikash Patra, Nilesh Kulkarni, Debashis Mondal, Kaushal Gavankar, Sourav K Sahu, Biswarup Satpati, Bahadur Singh, Owen Benton, Shouvik Chatterjee\",\"doi\":\"10.1002/advs.202502569\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p><p>Topological chiral antiferromagnets, such as Mn<sub>3</sub>Sn, are emerging as promising materials for next-generation spintronic devices due to their intrinsic transport properties linked to exotic magnetic configurations. Here, it is demonstrated that anisotropic strain in Mn<sub>3</sub>Sn thin films offers a novel approach to manipulate the magnetic ground state, unlocking new functionalities in this material. Anisotropic strain reduces the point group symmetry of the manganese (Mn) Kagome triangles from C<sub>3v</sub> to C<sub>1</sub>, significantly altering the energy landscape of the magnetic states in Mn<sub>3</sub>Sn. This symmetry reduction enables even a tiny in-plane Dzyaloshinskii-Moriya (DM) interaction to induce canting of the Mn spins out of the Kagome plane. The modified magnetic ground state introduces a finite scalar spin chirality and results in a significant Berry phase in momentum space. Consequently, a large anomalous Hall effect emerges in the Kagome plane at room temperature - an effect that is absent in the bulk material. Moreover, this twofold degenerate magnetic state enables the creation of multiple-stable, non-volatile anomalous Hall resistance (AHR) memory states. These states are field-stable and can be controlled by thermal-assisted current-induced magnetization switching, requiring modest current densities and small bias fields, thereby offering a compelling new functionality in Mn<sub>3</sub>Sn for spintronic applications.</p>\",\"PeriodicalId\":117,\"journal\":{\"name\":\"Advanced Science\",\"volume\":\" \",\"pages\":\"e02569\"},\"PeriodicalIF\":14.1000,\"publicationDate\":\"2025-08-01\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC12362762/pdf/\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Advanced Science\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://doi.org/10.1002/advs.202502569\",\"RegionNum\":1,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"2025/6/10 0:00:00\",\"PubModel\":\"Epub\",\"JCR\":\"Q1\",\"JCRName\":\"CHEMISTRY, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Advanced Science","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1002/advs.202502569","RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"2025/6/10 0:00:00","PubModel":"Epub","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
Imprinting Electrically Switchable Scalar Spin Chirality by Anisotropic Strain in a Kagome Antiferromagnet.
Topological chiral antiferromagnets, such as Mn3Sn, are emerging as promising materials for next-generation spintronic devices due to their intrinsic transport properties linked to exotic magnetic configurations. Here, it is demonstrated that anisotropic strain in Mn3Sn thin films offers a novel approach to manipulate the magnetic ground state, unlocking new functionalities in this material. Anisotropic strain reduces the point group symmetry of the manganese (Mn) Kagome triangles from C3v to C1, significantly altering the energy landscape of the magnetic states in Mn3Sn. This symmetry reduction enables even a tiny in-plane Dzyaloshinskii-Moriya (DM) interaction to induce canting of the Mn spins out of the Kagome plane. The modified magnetic ground state introduces a finite scalar spin chirality and results in a significant Berry phase in momentum space. Consequently, a large anomalous Hall effect emerges in the Kagome plane at room temperature - an effect that is absent in the bulk material. Moreover, this twofold degenerate magnetic state enables the creation of multiple-stable, non-volatile anomalous Hall resistance (AHR) memory states. These states are field-stable and can be controlled by thermal-assisted current-induced magnetization switching, requiring modest current densities and small bias fields, thereby offering a compelling new functionality in Mn3Sn for spintronic applications.
期刊介绍:
Advanced Science is a prestigious open access journal that focuses on interdisciplinary research in materials science, physics, chemistry, medical and life sciences, and engineering. The journal aims to promote cutting-edge research by employing a rigorous and impartial review process. It is committed to presenting research articles with the highest quality production standards, ensuring maximum accessibility of top scientific findings. With its vibrant and innovative publication platform, Advanced Science seeks to revolutionize the dissemination and organization of scientific knowledge.