{"title":"用数值模型研究了大气微塑料在自由大气中的远距离分散","authors":"Matteo M. Musso , Silvia Trini Castelli","doi":"10.1016/j.atmosenv.2025.121308","DOIUrl":null,"url":null,"abstract":"<div><div>In recent studies available in literature, long-range transport was suggested to play a main role in the motion of microplastics in the free atmosphere, whereas emission sources are located in the planetary boundary layer. In this framework, the Lagrangian particle dispersion model MILORD was used both in forward and in backward modes to investigate the potential effectiveness of the transport and exchange of microplastics between the boundary layer and the free atmosphere. Two pioneering case studies from the literature were considered. The first where microplastics were detected in the free atmosphere above Madrid region, the second where microplastics were collected in the air at the top-mountain site of Pic Du Midi in the French Pyrenees. The simulations showed that the long-range transport plays the main role in determining the presence of microplastics in the free atmosphere above Madrid, while the emissions from the city affect mostly the air in the boundary layer, at regional scale in the surrounding area. The long-range transport towards Pic Du Midi site pointed out also potential contributions connected to the exchange between the marine environments and the atmosphere and to possible dust events from North Africa.</div></div>","PeriodicalId":250,"journal":{"name":"Atmospheric Environment","volume":"358 ","pages":"Article 121308"},"PeriodicalIF":3.7000,"publicationDate":"2025-06-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Investigating the long-range dispersion of atmospheric microplastics in the free atmosphere with a numerical model\",\"authors\":\"Matteo M. Musso , Silvia Trini Castelli\",\"doi\":\"10.1016/j.atmosenv.2025.121308\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><div>In recent studies available in literature, long-range transport was suggested to play a main role in the motion of microplastics in the free atmosphere, whereas emission sources are located in the planetary boundary layer. In this framework, the Lagrangian particle dispersion model MILORD was used both in forward and in backward modes to investigate the potential effectiveness of the transport and exchange of microplastics between the boundary layer and the free atmosphere. Two pioneering case studies from the literature were considered. The first where microplastics were detected in the free atmosphere above Madrid region, the second where microplastics were collected in the air at the top-mountain site of Pic Du Midi in the French Pyrenees. The simulations showed that the long-range transport plays the main role in determining the presence of microplastics in the free atmosphere above Madrid, while the emissions from the city affect mostly the air in the boundary layer, at regional scale in the surrounding area. The long-range transport towards Pic Du Midi site pointed out also potential contributions connected to the exchange between the marine environments and the atmosphere and to possible dust events from North Africa.</div></div>\",\"PeriodicalId\":250,\"journal\":{\"name\":\"Atmospheric Environment\",\"volume\":\"358 \",\"pages\":\"Article 121308\"},\"PeriodicalIF\":3.7000,\"publicationDate\":\"2025-06-04\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Atmospheric Environment\",\"FirstCategoryId\":\"93\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S1352231025002833\",\"RegionNum\":2,\"RegionCategory\":\"环境科学与生态学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"ENVIRONMENTAL SCIENCES\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Atmospheric Environment","FirstCategoryId":"93","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S1352231025002833","RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"ENVIRONMENTAL SCIENCES","Score":null,"Total":0}
引用次数: 0
摘要
在最近的文献研究中,远程输运被认为在自由大气中微塑料的运动中起主要作用,而排放源位于行星边界层。在此框架下,拉格朗日粒子色散模型MILORD在正向和反向模式下被用于研究微塑料在边界层和自由大气之间的输运和交换的潜在有效性。考虑了文献中的两个开创性案例研究。第一次是在马德里地区上空的自由大气中检测到微塑料,第二次是在法国比利牛斯山脉山顶的Pic Du Midi收集空气中的微塑料。模拟结果表明,在确定马德里上空自由大气中微塑料存在的主要因素是远程传输,而城市排放主要影响周边区域尺度的边界层空气。向Pic Du Midi站点的远程迁移也指出了与海洋环境和大气之间的交换以及可能来自北非的沙尘事件有关的潜在贡献。
Investigating the long-range dispersion of atmospheric microplastics in the free atmosphere with a numerical model
In recent studies available in literature, long-range transport was suggested to play a main role in the motion of microplastics in the free atmosphere, whereas emission sources are located in the planetary boundary layer. In this framework, the Lagrangian particle dispersion model MILORD was used both in forward and in backward modes to investigate the potential effectiveness of the transport and exchange of microplastics between the boundary layer and the free atmosphere. Two pioneering case studies from the literature were considered. The first where microplastics were detected in the free atmosphere above Madrid region, the second where microplastics were collected in the air at the top-mountain site of Pic Du Midi in the French Pyrenees. The simulations showed that the long-range transport plays the main role in determining the presence of microplastics in the free atmosphere above Madrid, while the emissions from the city affect mostly the air in the boundary layer, at regional scale in the surrounding area. The long-range transport towards Pic Du Midi site pointed out also potential contributions connected to the exchange between the marine environments and the atmosphere and to possible dust events from North Africa.
期刊介绍:
Atmospheric Environment has an open access mirror journal Atmospheric Environment: X, sharing the same aims and scope, editorial team, submission system and rigorous peer review.
Atmospheric Environment is the international journal for scientists in different disciplines related to atmospheric composition and its impacts. The journal publishes scientific articles with atmospheric relevance of emissions and depositions of gaseous and particulate compounds, chemical processes and physical effects in the atmosphere, as well as impacts of the changing atmospheric composition on human health, air quality, climate change, and ecosystems.