Zhaoyang Shen , Qichao Wang , Feng Xu , Xiang Zhou , Lei Ni , Zhiquan Cheng , Juncheng Jiang
{"title":"扩大微通道中金属泡沫强化液-液非均质传质效果的研究","authors":"Zhaoyang Shen , Qichao Wang , Feng Xu , Xiang Zhou , Lei Ni , Zhiquan Cheng , Juncheng Jiang","doi":"10.1016/j.cep.2025.110379","DOIUrl":null,"url":null,"abstract":"<div><div>In this work, to enhance the mass transfer process between two heterogeneous phases in the enlarged microchannel, the metal foam was filled into the quartz channel. First, the homogeneous iodate system was employed to investigate the mixing efficiency of fluids flowing through the metal foam. The results indicate that the mixing efficiency improves with increasing metal foam length and pore density. Secondly, the extraction and mass transfer efficiency of metal foam was studied by using the n-butanol-succinic acid system (heterogeneous). The results showed that the extraction efficiency and mass transfer performance of metal foam with a pore density of 60 PPI and a length of 10 cm were the best, reaching 56 % and 0.297 s<sup>-1</sup>. Finally, the enhancement of metal foam on the reaction process was investigated by the oxidation process of phenylene sulfide, and the metal foam with the best mass transfer performance was selected for the experiment. Under the residence time of 15 min, the conversion of the raw material reached 86.57 %, which was nearly 4 times higher than that channel without structural inserts. Therefore, it is a very meaningful strategy to strengthen the mass transfer process by using the enlarged microchannels filled with metal foam.</div></div>","PeriodicalId":9929,"journal":{"name":"Chemical Engineering and Processing - Process Intensification","volume":"215 ","pages":"Article 110379"},"PeriodicalIF":3.9000,"publicationDate":"2025-05-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Investigation on strengthening effect of metal foams in enlarged microchannels for heterogeneous liquid-liquid mass transfer\",\"authors\":\"Zhaoyang Shen , Qichao Wang , Feng Xu , Xiang Zhou , Lei Ni , Zhiquan Cheng , Juncheng Jiang\",\"doi\":\"10.1016/j.cep.2025.110379\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><div>In this work, to enhance the mass transfer process between two heterogeneous phases in the enlarged microchannel, the metal foam was filled into the quartz channel. First, the homogeneous iodate system was employed to investigate the mixing efficiency of fluids flowing through the metal foam. The results indicate that the mixing efficiency improves with increasing metal foam length and pore density. Secondly, the extraction and mass transfer efficiency of metal foam was studied by using the n-butanol-succinic acid system (heterogeneous). The results showed that the extraction efficiency and mass transfer performance of metal foam with a pore density of 60 PPI and a length of 10 cm were the best, reaching 56 % and 0.297 s<sup>-1</sup>. Finally, the enhancement of metal foam on the reaction process was investigated by the oxidation process of phenylene sulfide, and the metal foam with the best mass transfer performance was selected for the experiment. Under the residence time of 15 min, the conversion of the raw material reached 86.57 %, which was nearly 4 times higher than that channel without structural inserts. Therefore, it is a very meaningful strategy to strengthen the mass transfer process by using the enlarged microchannels filled with metal foam.</div></div>\",\"PeriodicalId\":9929,\"journal\":{\"name\":\"Chemical Engineering and Processing - Process Intensification\",\"volume\":\"215 \",\"pages\":\"Article 110379\"},\"PeriodicalIF\":3.9000,\"publicationDate\":\"2025-05-27\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Chemical Engineering and Processing - Process Intensification\",\"FirstCategoryId\":\"5\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S0255270125002284\",\"RegionNum\":3,\"RegionCategory\":\"工程技术\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q3\",\"JCRName\":\"ENERGY & FUELS\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Chemical Engineering and Processing - Process Intensification","FirstCategoryId":"5","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S0255270125002284","RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"ENERGY & FUELS","Score":null,"Total":0}
Investigation on strengthening effect of metal foams in enlarged microchannels for heterogeneous liquid-liquid mass transfer
In this work, to enhance the mass transfer process between two heterogeneous phases in the enlarged microchannel, the metal foam was filled into the quartz channel. First, the homogeneous iodate system was employed to investigate the mixing efficiency of fluids flowing through the metal foam. The results indicate that the mixing efficiency improves with increasing metal foam length and pore density. Secondly, the extraction and mass transfer efficiency of metal foam was studied by using the n-butanol-succinic acid system (heterogeneous). The results showed that the extraction efficiency and mass transfer performance of metal foam with a pore density of 60 PPI and a length of 10 cm were the best, reaching 56 % and 0.297 s-1. Finally, the enhancement of metal foam on the reaction process was investigated by the oxidation process of phenylene sulfide, and the metal foam with the best mass transfer performance was selected for the experiment. Under the residence time of 15 min, the conversion of the raw material reached 86.57 %, which was nearly 4 times higher than that channel without structural inserts. Therefore, it is a very meaningful strategy to strengthen the mass transfer process by using the enlarged microchannels filled with metal foam.
期刊介绍:
Chemical Engineering and Processing: Process Intensification is intended for practicing researchers in industry and academia, working in the field of Process Engineering and related to the subject of Process Intensification.Articles published in the Journal demonstrate how novel discoveries, developments and theories in the field of Process Engineering and in particular Process Intensification may be used for analysis and design of innovative equipment and processing methods with substantially improved sustainability, efficiency and environmental performance.