Zejing Wang, Shuai Wan, Yangyang Shi, Zhongyang Li
{"title":"用于单向发射和非相干全息的发光超表面矢量荧光控制","authors":"Zejing Wang, Shuai Wan, Yangyang Shi, Zhongyang Li","doi":"10.1002/adma.202502682","DOIUrl":null,"url":null,"abstract":"Ultracompact light emission manipulation is crucial for various applications, including illumination, biosensing, and quantum photonics. Despite significant advancements in lasing manipulation, achieving complex vectorial wavefront control over fluorescence emission is inherently challenging due to its incoherent, omnidirectional, unpolarized, and phase-random emission characteristics. Here, the light-emitting metasurfaces (LEMs), equipped with vectorial manipulation and complex amplitude encoding capabilities, are introduced to realize unidirectional emission and incoherent photoluminescence (PL) holography. Through engineering the interaction between the LEM and guided PL, the diffraction angle, linear polarization state, and emission intensity of PL unidirectional emission are independently controlled. Furthermore, the phase encoding capability of LEM, combined with the enhanced spatial coherence of guided PL, experimentally enabled vectorial PL holography alongside polarization-multiplexed nanoprinting. This versatile LEM platform provides a simplified approach to vectorial PL manipulation, promising multiple potential applications in nanophotonics and light-emitting devices.","PeriodicalId":114,"journal":{"name":"Advanced Materials","volume":"29 1","pages":""},"PeriodicalIF":27.4000,"publicationDate":"2025-06-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Vectorial Fluorescence Control with Light-Emitting Metasurfaces for Unidirectional Emission and Incoherent Holography\",\"authors\":\"Zejing Wang, Shuai Wan, Yangyang Shi, Zhongyang Li\",\"doi\":\"10.1002/adma.202502682\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"Ultracompact light emission manipulation is crucial for various applications, including illumination, biosensing, and quantum photonics. Despite significant advancements in lasing manipulation, achieving complex vectorial wavefront control over fluorescence emission is inherently challenging due to its incoherent, omnidirectional, unpolarized, and phase-random emission characteristics. Here, the light-emitting metasurfaces (LEMs), equipped with vectorial manipulation and complex amplitude encoding capabilities, are introduced to realize unidirectional emission and incoherent photoluminescence (PL) holography. Through engineering the interaction between the LEM and guided PL, the diffraction angle, linear polarization state, and emission intensity of PL unidirectional emission are independently controlled. Furthermore, the phase encoding capability of LEM, combined with the enhanced spatial coherence of guided PL, experimentally enabled vectorial PL holography alongside polarization-multiplexed nanoprinting. This versatile LEM platform provides a simplified approach to vectorial PL manipulation, promising multiple potential applications in nanophotonics and light-emitting devices.\",\"PeriodicalId\":114,\"journal\":{\"name\":\"Advanced Materials\",\"volume\":\"29 1\",\"pages\":\"\"},\"PeriodicalIF\":27.4000,\"publicationDate\":\"2025-06-02\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Advanced Materials\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://doi.org/10.1002/adma.202502682\",\"RegionNum\":1,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"CHEMISTRY, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Advanced Materials","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1002/adma.202502682","RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
Vectorial Fluorescence Control with Light-Emitting Metasurfaces for Unidirectional Emission and Incoherent Holography
Ultracompact light emission manipulation is crucial for various applications, including illumination, biosensing, and quantum photonics. Despite significant advancements in lasing manipulation, achieving complex vectorial wavefront control over fluorescence emission is inherently challenging due to its incoherent, omnidirectional, unpolarized, and phase-random emission characteristics. Here, the light-emitting metasurfaces (LEMs), equipped with vectorial manipulation and complex amplitude encoding capabilities, are introduced to realize unidirectional emission and incoherent photoluminescence (PL) holography. Through engineering the interaction between the LEM and guided PL, the diffraction angle, linear polarization state, and emission intensity of PL unidirectional emission are independently controlled. Furthermore, the phase encoding capability of LEM, combined with the enhanced spatial coherence of guided PL, experimentally enabled vectorial PL holography alongside polarization-multiplexed nanoprinting. This versatile LEM platform provides a simplified approach to vectorial PL manipulation, promising multiple potential applications in nanophotonics and light-emitting devices.
期刊介绍:
Advanced Materials, one of the world's most prestigious journals and the foundation of the Advanced portfolio, is the home of choice for best-in-class materials science for more than 30 years. Following this fast-growing and interdisciplinary field, we are considering and publishing the most important discoveries on any and all materials from materials scientists, chemists, physicists, engineers as well as health and life scientists and bringing you the latest results and trends in modern materials-related research every week.