Shimao Deng, Zishuo Zhao, Hadi Khani and Yijin Liu*,
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Multiscale Heterogeneous and Asynchronous Electrochemical Reactions in Lithium-Ion Batteries
Battery operation involves sophisticated spatiotemporal evolutions that critically govern their behaviors and degradation. Understanding and manipulating structural heterogeneity and chemical dynamics are key to improving battery performance, lifespan, and safety. This review examines spatial heterogeneity across multiple scales and explores the temporal asynchronicity characteristics of lithium-ion batteries. Furthermore, it underscores the importance of multimodal, high-throughput, and in-situ/operando characterization techniques, paired with advanced data mining methods, in advancing knowledge of battery evolution. We intend for this review to provide a systematic perspective on the spatiotemporal evolution of batteries and to inspire further research into its implications for next-generation battery research and development.
期刊介绍：
ACS Materials Letters is a journal that publishes high-quality and urgent papers at the forefront of fundamental and applied research in the field of materials science. It aims to bridge the gap between materials and other disciplines such as chemistry, engineering, and biology. The journal encourages multidisciplinary and innovative research that addresses global challenges. Papers submitted to ACS Materials Letters should clearly demonstrate the need for rapid disclosure of key results. The journal is interested in various areas including the design, synthesis, characterization, and evaluation of emerging materials, understanding the relationships between structure, property, and performance, as well as developing materials for applications in energy, environment, biomedical, electronics, and catalysis. The journal has a 2-year impact factor of 11.4 and is dedicated to publishing transformative materials research with fast processing times. The editors and staff of ACS Materials Letters actively participate in major scientific conferences and engage closely with readers and authors. The journal also maintains an active presence on social media to provide authors with greater visibility.
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