{"title":"竹笋启发的超高锥形多孔蒸发器用于高盐度海水的淡化","authors":"Mingzhu Xie, Zicheng Qian, Jiyuan Yu, Xiaolong Wang, Yinfeng Li, Ziheng Zhan, Xiaowei Wang, Yong Shuai, Huaduo Gu, Zhaolong Wang","doi":"10.1016/j.cej.2025.164253","DOIUrl":null,"url":null,"abstract":"Solar-driven seawater evaporation is sustainable for freshwater but limited by water sources, wastes tolerance, and durability. Here, we propose a bamboo shoot inspired conical porous evaporation made of multiwall carbon nanotube-based composite materials, which demonstrates ultra-high-water transportation, high evaporation efficiency and salt-rejecting properties under high salinity and contaminated conditions. Its bioinspired microchannels’ capillary effect can drive liquid up to 126.0 mm, offering continuous water supply for evaporation and reducing liquid surface pressure, thus increasing evaporation efficiency with a capacity up to 2.54 kg m<sup>-2</sup>h<sup>−1</sup>. Meanwhile, the three-dimensional structure generates a temperature gradient, which induces Marangoni convection and facilitates the flow of saline water from high-concentration areas to low-concentration areas. This convection and capillary fluid replenishment work together to maintain salt concentration balance, enabling long-term seawater desalination over 200 h in 20 wt% saline water without cleaning.","PeriodicalId":270,"journal":{"name":"Chemical Engineering Journal","volume":"5 1","pages":""},"PeriodicalIF":13.3000,"publicationDate":"2025-05-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Bamboo shoot inspired ultra-high conical porous evaporator for desalination of seawater with high salinity\",\"authors\":\"Mingzhu Xie, Zicheng Qian, Jiyuan Yu, Xiaolong Wang, Yinfeng Li, Ziheng Zhan, Xiaowei Wang, Yong Shuai, Huaduo Gu, Zhaolong Wang\",\"doi\":\"10.1016/j.cej.2025.164253\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"Solar-driven seawater evaporation is sustainable for freshwater but limited by water sources, wastes tolerance, and durability. Here, we propose a bamboo shoot inspired conical porous evaporation made of multiwall carbon nanotube-based composite materials, which demonstrates ultra-high-water transportation, high evaporation efficiency and salt-rejecting properties under high salinity and contaminated conditions. Its bioinspired microchannels’ capillary effect can drive liquid up to 126.0 mm, offering continuous water supply for evaporation and reducing liquid surface pressure, thus increasing evaporation efficiency with a capacity up to 2.54 kg m<sup>-2</sup>h<sup>−1</sup>. Meanwhile, the three-dimensional structure generates a temperature gradient, which induces Marangoni convection and facilitates the flow of saline water from high-concentration areas to low-concentration areas. This convection and capillary fluid replenishment work together to maintain salt concentration balance, enabling long-term seawater desalination over 200 h in 20 wt% saline water without cleaning.\",\"PeriodicalId\":270,\"journal\":{\"name\":\"Chemical Engineering Journal\",\"volume\":\"5 1\",\"pages\":\"\"},\"PeriodicalIF\":13.3000,\"publicationDate\":\"2025-05-29\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Chemical Engineering Journal\",\"FirstCategoryId\":\"5\",\"ListUrlMain\":\"https://doi.org/10.1016/j.cej.2025.164253\",\"RegionNum\":1,\"RegionCategory\":\"工程技术\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"ENGINEERING, CHEMICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Chemical Engineering Journal","FirstCategoryId":"5","ListUrlMain":"https://doi.org/10.1016/j.cej.2025.164253","RegionNum":1,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"ENGINEERING, CHEMICAL","Score":null,"Total":0}
引用次数: 0
摘要
太阳能驱动的海水蒸发对淡水来说是可持续的,但受到水源、废物容忍度和持久性的限制。本文提出了一种以竹笋为材料的多壁碳纳米管复合材料锥形多孔蒸发装置,该装置在高盐度和高污染条件下具有超高水分输送、高蒸发效率和拒盐性能。其仿生微通道的毛细效应可驱动液体至126.0 mm,为蒸发提供连续的供水量,降低液体表面压力,从而提高蒸发效率,容量可达2.54 kg m-2h−1。同时,三维结构产生温度梯度,诱导Marangoni对流,有利于盐水从高浓度区向低浓度区流动。这种对流和毛细管流体补充一起工作,保持盐浓度平衡,使海水在20 wt%的盐水中长期淡化200 h而无需清洗。
Bamboo shoot inspired ultra-high conical porous evaporator for desalination of seawater with high salinity
Solar-driven seawater evaporation is sustainable for freshwater but limited by water sources, wastes tolerance, and durability. Here, we propose a bamboo shoot inspired conical porous evaporation made of multiwall carbon nanotube-based composite materials, which demonstrates ultra-high-water transportation, high evaporation efficiency and salt-rejecting properties under high salinity and contaminated conditions. Its bioinspired microchannels’ capillary effect can drive liquid up to 126.0 mm, offering continuous water supply for evaporation and reducing liquid surface pressure, thus increasing evaporation efficiency with a capacity up to 2.54 kg m-2h−1. Meanwhile, the three-dimensional structure generates a temperature gradient, which induces Marangoni convection and facilitates the flow of saline water from high-concentration areas to low-concentration areas. This convection and capillary fluid replenishment work together to maintain salt concentration balance, enabling long-term seawater desalination over 200 h in 20 wt% saline water without cleaning.
期刊介绍:
The Chemical Engineering Journal is an international research journal that invites contributions of original and novel fundamental research. It aims to provide an international platform for presenting original fundamental research, interpretative reviews, and discussions on new developments in chemical engineering. The journal welcomes papers that describe novel theory and its practical application, as well as those that demonstrate the transfer of techniques from other disciplines. It also welcomes reports on carefully conducted experimental work that is soundly interpreted. The main focus of the journal is on original and rigorous research results that have broad significance. The Catalysis section within the Chemical Engineering Journal focuses specifically on Experimental and Theoretical studies in the fields of heterogeneous catalysis, molecular catalysis, and biocatalysis. These studies have industrial impact on various sectors such as chemicals, energy, materials, foods, healthcare, and environmental protection.