新疆道路粉尘中PAHs、NPAHs和ophs的现状、来源及健康风险评价

IF 3.9 2区 综合性期刊 Q1 MULTIDISCIPLINARY SCIENCES
Xiawei Yang, Yaqin Ji, Bingbing Wang, Jingwen Shi, Wenju Xu, Jiaofan Ma, Ruixing Shen, Yan Jiang
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引用次数: 0

摘要

对新疆地区采集的260份道路粉尘样品进行了重悬浮分析,分析了多环芳烃及其衍生物的含量。PM10中∑16PAHs、∑18NPAHs和∑5ophs (ng mg-1)的浓度范围分别为22.03 ~ 179.04、0.34 ~ 3.14和0.95 ~ 17.56,中位数分别为69.09、1.14和4.37。Phe、Ace、Flt、2N-Pyr、9-FO和ATO是发现的主要物质。各城市∑16PAHs浓度中位数顺序为:阿勒泰、阿克苏、克拉玛依、伯乐、喀什、库尔勒、库尔勒、塔城、哈密、吐鲁番、乌苏、和田、奎屯、湖阳河、阿图什。各城市的∑18NPAHs浓度顺序为:阿勒泰bb0克拉玛依bb1哈密bb2库尔勒bb3伯乐bb4喀什bb5乌苏>塔城>阿克苏>呼阳河>阿图什>奎屯>和田>吐鲁番。各城市的∑5OPAHs浓度顺序为:阿勒泰、克拉玛依、塔城、奎屯、阿克苏、喀什、库尔勒、库尔勒、哈密、乌苏、伯乐、和田、和田、湖阳河、吐鲁番、阿图什。根据诊断率和PMF结果,确定了4个源因子:生物质燃烧(36.3%)、煤炭燃烧(39.0%)、汽油和柴油燃烧(13.3%)和石油燃烧(11.4%)。新疆地区道路粉尘多环芳烃暴露导致儿童、女性和男性癌症总增量危险度分别为8.2 × 10-6、1.2 × 10-5和1.2 × 10-5。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Status, sources and health risk assessment of PAHs, NPAHs and OPAHs in road dust of Xinjiang, China.

Two hundred and sixty road dust samples collected from Xinjiang, China, were resuspended and analyzed for polycyclic aromatic hydrocarbons (PAHs) and their derivatives. The concentrations of ∑16PAHs, ∑18NPAHs and ∑5OPAHs (ng mg-1) in the road dust PM10 ranged from 22.03 to 179.04, 0.34-3.14, and 0.95-17.56, with median values of 69.09, 1.14, and 4.37, respectively. Phe, Ace, Flt, 2N-Pyr, 9-FO, and ATO were the main substances found. The order of the median concentrations of ∑16PAHs in each city in the region was Altay > Aksu > Karamay > Bole > Kashgar > Korla > Tacheng > Hami > Turpan > Wusu > Hotan > Kuitun > Huyanghe > Atushi. The order of the ∑18NPAHs concentrations in each city was Altay > Karamay > Hami > Korla > Bole > Kashgar > Wusu > Tacheng > Aksu > Huyanghe > Atushi > Kuitun > Hotan > Turpan. The order of the ∑5OPAHs concentrations in each city was Altay > Karamay > Tacheng > Kuitun > Aksu > Kashgar > Korla > Hami > Wusu > Bole > Hotan > Huyanghe > Turpan > Atushi. According to the diagnostic ratio and PMF results, four source factors were identified: biomass combustion (36.3%), coal combustion (39.0%), gasoline and diesel combustion (13.3%), and petroleum (11.4%). The total incremental lifetime cancer risks (TILCR) due to human exposure to road dust PAHs in Xinjiang were 8.2 × 10-6 for children, 1.2 × 10-5 for females, and 1.2 × 10-5 for males.

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来源期刊
Scientific Reports
Scientific Reports Natural Science Disciplines-
CiteScore
7.50
自引率
4.30%
发文量
19567
审稿时长
3.9 months
期刊介绍: We publish original research from all areas of the natural sciences, psychology, medicine and engineering. You can learn more about what we publish by browsing our specific scientific subject areas below or explore Scientific Reports by browsing all articles and collections. Scientific Reports has a 2-year impact factor: 4.380 (2021), and is the 6th most-cited journal in the world, with more than 540,000 citations in 2020 (Clarivate Analytics, 2021). •Engineering Engineering covers all aspects of engineering, technology, and applied science. It plays a crucial role in the development of technologies to address some of the world''s biggest challenges, helping to save lives and improve the way we live. •Physical sciences Physical sciences are those academic disciplines that aim to uncover the underlying laws of nature — often written in the language of mathematics. It is a collective term for areas of study including astronomy, chemistry, materials science and physics. •Earth and environmental sciences Earth and environmental sciences cover all aspects of Earth and planetary science and broadly encompass solid Earth processes, surface and atmospheric dynamics, Earth system history, climate and climate change, marine and freshwater systems, and ecology. It also considers the interactions between humans and these systems. •Biological sciences Biological sciences encompass all the divisions of natural sciences examining various aspects of vital processes. The concept includes anatomy, physiology, cell biology, biochemistry and biophysics, and covers all organisms from microorganisms, animals to plants. •Health sciences The health sciences study health, disease and healthcare. This field of study aims to develop knowledge, interventions and technology for use in healthcare to improve the treatment of patients.
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