Xin Xiao , Pengrui Jin , Yue Wang , Riri Liu , Lei Jiang , Qin Chen , Chen Zhao , Kai Sheng , Zhao Yang , Shushan Yuan , Bart Van der Bruggen
{"title":"部分碳化西瓜肉为基础的3D蒸发器,通过侧面吸热增强,高效海水淡化","authors":"Xin Xiao , Pengrui Jin , Yue Wang , Riri Liu , Lei Jiang , Qin Chen , Chen Zhao , Kai Sheng , Zhao Yang , Shushan Yuan , Bart Van der Bruggen","doi":"10.1016/j.seppur.2025.133724","DOIUrl":null,"url":null,"abstract":"<div><div>Three-dimensional (3D) carbon materials have shown great potential in solar interface evaporation devices, but salt deposition and low evaporation efficiency significantly hinder their continuous operation under seawater conditions. This work presents an all-in-one and sustainable all-biomass evaporator with unique structural advantages, in which the space between the watermelon fibers acts as micro/nanopores water transport channels, while carbonized nanosheets formed onto the outer surface transform absorbed sunlight to heat. As a result, the biomass foam evaporator achieved an excellent evaporation rate of up to 2.35 kg·m<sup>−2</sup>·h<sup>−1</sup> in pure water and 2.0 kg·m<sup>−2</sup>·h<sup>−1</sup> in 3.5 wt% NaCl solution under 1 sun irradiation, and similarly exhibited a high efficiency and stable operation and superior anti-salt performance in 25 wt% NaCl solution, as well as a remarkable wastewater purification performance. This is attributed to the fast water replenishment facilitated by multi-layered porous structures and hydrophilic groups, efficient thermal management provided by the<!--> <!-->three-dimensional cylindrical shape, and the<!--> <!-->capture of environmental energy from the<!--> <!-->cold side surface of the<!--> <!-->3D evaporator. This research not only highlights the potential of incompletely carbonized watermelon as a low-cost biomass material for seawater desalination during solar steam generation but also provides insights for improving the water transport properties of 3D biochar evaporators.</div></div>","PeriodicalId":427,"journal":{"name":"Separation and Purification Technology","volume":"374 ","pages":"Article 133724"},"PeriodicalIF":8.1000,"publicationDate":"2025-05-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Partially carbonized watermelon flesh-based 3D evaporator enhanced by side heat absorption for efficient seawater desalination\",\"authors\":\"Xin Xiao , Pengrui Jin , Yue Wang , Riri Liu , Lei Jiang , Qin Chen , Chen Zhao , Kai Sheng , Zhao Yang , Shushan Yuan , Bart Van der Bruggen\",\"doi\":\"10.1016/j.seppur.2025.133724\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><div>Three-dimensional (3D) carbon materials have shown great potential in solar interface evaporation devices, but salt deposition and low evaporation efficiency significantly hinder their continuous operation under seawater conditions. This work presents an all-in-one and sustainable all-biomass evaporator with unique structural advantages, in which the space between the watermelon fibers acts as micro/nanopores water transport channels, while carbonized nanosheets formed onto the outer surface transform absorbed sunlight to heat. As a result, the biomass foam evaporator achieved an excellent evaporation rate of up to 2.35 kg·m<sup>−2</sup>·h<sup>−1</sup> in pure water and 2.0 kg·m<sup>−2</sup>·h<sup>−1</sup> in 3.5 wt% NaCl solution under 1 sun irradiation, and similarly exhibited a high efficiency and stable operation and superior anti-salt performance in 25 wt% NaCl solution, as well as a remarkable wastewater purification performance. This is attributed to the fast water replenishment facilitated by multi-layered porous structures and hydrophilic groups, efficient thermal management provided by the<!--> <!-->three-dimensional cylindrical shape, and the<!--> <!-->capture of environmental energy from the<!--> <!-->cold side surface of the<!--> <!-->3D evaporator. This research not only highlights the potential of incompletely carbonized watermelon as a low-cost biomass material for seawater desalination during solar steam generation but also provides insights for improving the water transport properties of 3D biochar evaporators.</div></div>\",\"PeriodicalId\":427,\"journal\":{\"name\":\"Separation and Purification Technology\",\"volume\":\"374 \",\"pages\":\"Article 133724\"},\"PeriodicalIF\":8.1000,\"publicationDate\":\"2025-05-24\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Separation and Purification Technology\",\"FirstCategoryId\":\"5\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S1383586625023214\",\"RegionNum\":1,\"RegionCategory\":\"工程技术\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"ENGINEERING, CHEMICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Separation and Purification Technology","FirstCategoryId":"5","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S1383586625023214","RegionNum":1,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"ENGINEERING, CHEMICAL","Score":null,"Total":0}
Partially carbonized watermelon flesh-based 3D evaporator enhanced by side heat absorption for efficient seawater desalination
Three-dimensional (3D) carbon materials have shown great potential in solar interface evaporation devices, but salt deposition and low evaporation efficiency significantly hinder their continuous operation under seawater conditions. This work presents an all-in-one and sustainable all-biomass evaporator with unique structural advantages, in which the space between the watermelon fibers acts as micro/nanopores water transport channels, while carbonized nanosheets formed onto the outer surface transform absorbed sunlight to heat. As a result, the biomass foam evaporator achieved an excellent evaporation rate of up to 2.35 kg·m−2·h−1 in pure water and 2.0 kg·m−2·h−1 in 3.5 wt% NaCl solution under 1 sun irradiation, and similarly exhibited a high efficiency and stable operation and superior anti-salt performance in 25 wt% NaCl solution, as well as a remarkable wastewater purification performance. This is attributed to the fast water replenishment facilitated by multi-layered porous structures and hydrophilic groups, efficient thermal management provided by the three-dimensional cylindrical shape, and the capture of environmental energy from the cold side surface of the 3D evaporator. This research not only highlights the potential of incompletely carbonized watermelon as a low-cost biomass material for seawater desalination during solar steam generation but also provides insights for improving the water transport properties of 3D biochar evaporators.
期刊介绍:
Separation and Purification Technology is a premier journal committed to sharing innovative methods for separation and purification in chemical and environmental engineering, encompassing both homogeneous solutions and heterogeneous mixtures. Our scope includes the separation and/or purification of liquids, vapors, and gases, as well as carbon capture and separation techniques. However, it's important to note that methods solely intended for analytical purposes are not within the scope of the journal. Additionally, disciplines such as soil science, polymer science, and metallurgy fall outside the purview of Separation and Purification Technology. Join us in advancing the field of separation and purification methods for sustainable solutions in chemical and environmental engineering.