Cenyao Tang, Zefeng Lin, Shunye Gao, Jin Zhao, Xingchen Guo, Zhicheng Rao, Yigui Zhong, Xilin Feng, Jianyu Guan, Yaobo Huang, Tian Qian, Weiqiang Chen, Zhengyu Weng, Hong Ding, Kun Jiang, Kui Jin, Yujie Sun
{"title":"电子掺杂La2-xCexCuO4中扩展的奇异金属相","authors":"Cenyao Tang, Zefeng Lin, Shunye Gao, Jin Zhao, Xingchen Guo, Zhicheng Rao, Yigui Zhong, Xilin Feng, Jianyu Guan, Yaobo Huang, Tian Qian, Weiqiang Chen, Zhengyu Weng, Hong Ding, Kun Jiang, Kui Jin, Yujie Sun","doi":"10.1021/acs.nanolett.5c01385","DOIUrl":null,"url":null,"abstract":"Landau’s Fermi liquid theory offers a profound understanding of conduction electrons in metals. However, many strongly correlated materials, including heavy-fermions, cuprates, iron-based superconductors, and nickelates, exhibit non-Fermi liquid (NFL) behavior. A hallmark is the strange metal state, characterized by linear-in-temperature resistivity and a linear-in-energy single-particle decay rate. Using angle-resolved photoemission spectroscopy measurements, we systematically investigate electron-doped cuprate La<sub>2–<i>x</i></sub>Ce<sub><i>x</i></sub>CuO<sub>4</sub> (LCCO) to explore the doping, momentum, and temperature dependence of the self-energy. We observe robust linear-in-energy single-particle scattering across almost the entire momentum space, persisting at high doping levels and temperatures. The extended strange metal behavior suggests a unified normal state, in contrast to an adjacent pseudogap regime in the hole-doped cuprates. This indicates that the physics of the strange metal may be key to high-<i>T</i><sub>c</sub> superconductivity, making LCCO an ideal system for exploring quantum criticality and offering new insights into the microscopic mechanisms for high-<i>T</i><sub>c</sub> superconductivity.","PeriodicalId":53,"journal":{"name":"Nano Letters","volume":"11 1","pages":""},"PeriodicalIF":9.1000,"publicationDate":"2025-05-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Extended Strange Metal Phase in Electron-Doped La2–xCexCuO4\",\"authors\":\"Cenyao Tang, Zefeng Lin, Shunye Gao, Jin Zhao, Xingchen Guo, Zhicheng Rao, Yigui Zhong, Xilin Feng, Jianyu Guan, Yaobo Huang, Tian Qian, Weiqiang Chen, Zhengyu Weng, Hong Ding, Kun Jiang, Kui Jin, Yujie Sun\",\"doi\":\"10.1021/acs.nanolett.5c01385\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"Landau’s Fermi liquid theory offers a profound understanding of conduction electrons in metals. However, many strongly correlated materials, including heavy-fermions, cuprates, iron-based superconductors, and nickelates, exhibit non-Fermi liquid (NFL) behavior. A hallmark is the strange metal state, characterized by linear-in-temperature resistivity and a linear-in-energy single-particle decay rate. Using angle-resolved photoemission spectroscopy measurements, we systematically investigate electron-doped cuprate La<sub>2–<i>x</i></sub>Ce<sub><i>x</i></sub>CuO<sub>4</sub> (LCCO) to explore the doping, momentum, and temperature dependence of the self-energy. We observe robust linear-in-energy single-particle scattering across almost the entire momentum space, persisting at high doping levels and temperatures. The extended strange metal behavior suggests a unified normal state, in contrast to an adjacent pseudogap regime in the hole-doped cuprates. This indicates that the physics of the strange metal may be key to high-<i>T</i><sub>c</sub> superconductivity, making LCCO an ideal system for exploring quantum criticality and offering new insights into the microscopic mechanisms for high-<i>T</i><sub>c</sub> superconductivity.\",\"PeriodicalId\":53,\"journal\":{\"name\":\"Nano Letters\",\"volume\":\"11 1\",\"pages\":\"\"},\"PeriodicalIF\":9.1000,\"publicationDate\":\"2025-05-22\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Nano Letters\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://doi.org/10.1021/acs.nanolett.5c01385\",\"RegionNum\":1,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"CHEMISTRY, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Nano Letters","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1021/acs.nanolett.5c01385","RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
Extended Strange Metal Phase in Electron-Doped La2–xCexCuO4
Landau’s Fermi liquid theory offers a profound understanding of conduction electrons in metals. However, many strongly correlated materials, including heavy-fermions, cuprates, iron-based superconductors, and nickelates, exhibit non-Fermi liquid (NFL) behavior. A hallmark is the strange metal state, characterized by linear-in-temperature resistivity and a linear-in-energy single-particle decay rate. Using angle-resolved photoemission spectroscopy measurements, we systematically investigate electron-doped cuprate La2–xCexCuO4 (LCCO) to explore the doping, momentum, and temperature dependence of the self-energy. We observe robust linear-in-energy single-particle scattering across almost the entire momentum space, persisting at high doping levels and temperatures. The extended strange metal behavior suggests a unified normal state, in contrast to an adjacent pseudogap regime in the hole-doped cuprates. This indicates that the physics of the strange metal may be key to high-Tc superconductivity, making LCCO an ideal system for exploring quantum criticality and offering new insights into the microscopic mechanisms for high-Tc superconductivity.
期刊介绍:
Nano Letters serves as a dynamic platform for promptly disseminating original results in fundamental, applied, and emerging research across all facets of nanoscience and nanotechnology. A pivotal criterion for inclusion within Nano Letters is the convergence of at least two different areas or disciplines, ensuring a rich interdisciplinary scope. The journal is dedicated to fostering exploration in diverse areas, including:
- Experimental and theoretical findings on physical, chemical, and biological phenomena at the nanoscale
- Synthesis, characterization, and processing of organic, inorganic, polymer, and hybrid nanomaterials through physical, chemical, and biological methodologies
- Modeling and simulation of synthetic, assembly, and interaction processes
- Realization of integrated nanostructures and nano-engineered devices exhibiting advanced performance
- Applications of nanoscale materials in living and environmental systems
Nano Letters is committed to advancing and showcasing groundbreaking research that intersects various domains, fostering innovation and collaboration in the ever-evolving field of nanoscience and nanotechnology.