Joseph E. Jacobs*, C. Heath Stanfield*, Quin R. S. Miller, Matthew A. Villante, José Marcial, Emily T. Nienhuis, Joshua A. Silverstein, Ellen G. Polites, Madeline F. Bartels, Brad T. Gooch, Jian Liu, Joyashish Thakurta, Nabajit Lahiri and H. Todd Schaef,
{"title":"西北太平洋地区碳矿化的技术经济潜力与关键矿物的提高回收","authors":"Joseph E. Jacobs*, C. Heath Stanfield*, Quin R. S. Miller, Matthew A. Villante, José Marcial, Emily T. Nienhuis, Joshua A. Silverstein, Ellen G. Polites, Madeline F. Bartels, Brad T. Gooch, Jian Liu, Joyashish Thakurta, Nabajit Lahiri and H. Todd Schaef, ","doi":"10.1021/acssusresmgt.4c0054110.1021/acssusresmgt.4c00541","DOIUrl":null,"url":null,"abstract":"<p >Commitments to limit the effects of global climate change require the implementation of renewable energy, along with a significant reduction of CO<sub>2</sub> emissions. To facilitate this transition, the active removal of atmospheric CO<sub>2</sub> by the development and deployment of new carbon management infrastructure and technologies is needed. Additionally, the world is projected to require an unprecedented amount of critical minerals, yet current high-grade ore supplies and existing mining technologies are unable to meet this demand. This study analyzes the feasibility of a novel CO<sub>2</sub> mineralization and enhanced mineral recovery (CO<sub>2</sub>-EMR) technology designed to target low-grade, historically uneconomical resources for in situ mining. The Josephine Ophiolite in Northern California and Twin Sisters Dunite in Northwest Washington are promising ultramafic reservoirs for implementing this new mining technology. Ultramafic, olivine-rich rocks from these two sites were characterized pre- and postreaction with CO<sub>2</sub>, with both samples showing rapid carbonation in the form of magnesite. Furthermore, the fluid sampled shows a high recovery of nickel, a designated critical mineral. These experimental findings were then implemented in a technoeconomic analysis to assess the viability of field-scale implementation of this technology in the Pacific Northwest and beyond.</p>","PeriodicalId":100015,"journal":{"name":"ACS Sustainable Resource Management","volume":"2 5","pages":"775–785 775–785"},"PeriodicalIF":0.0000,"publicationDate":"2025-04-30","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Technoeconomic Potential for Carbon Mineralization with Enhanced Recovery of Critical Minerals in the Pacific Northwest\",\"authors\":\"Joseph E. Jacobs*, C. Heath Stanfield*, Quin R. S. Miller, Matthew A. Villante, José Marcial, Emily T. Nienhuis, Joshua A. Silverstein, Ellen G. Polites, Madeline F. Bartels, Brad T. Gooch, Jian Liu, Joyashish Thakurta, Nabajit Lahiri and H. Todd Schaef, \",\"doi\":\"10.1021/acssusresmgt.4c0054110.1021/acssusresmgt.4c00541\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p >Commitments to limit the effects of global climate change require the implementation of renewable energy, along with a significant reduction of CO<sub>2</sub> emissions. To facilitate this transition, the active removal of atmospheric CO<sub>2</sub> by the development and deployment of new carbon management infrastructure and technologies is needed. Additionally, the world is projected to require an unprecedented amount of critical minerals, yet current high-grade ore supplies and existing mining technologies are unable to meet this demand. This study analyzes the feasibility of a novel CO<sub>2</sub> mineralization and enhanced mineral recovery (CO<sub>2</sub>-EMR) technology designed to target low-grade, historically uneconomical resources for in situ mining. The Josephine Ophiolite in Northern California and Twin Sisters Dunite in Northwest Washington are promising ultramafic reservoirs for implementing this new mining technology. Ultramafic, olivine-rich rocks from these two sites were characterized pre- and postreaction with CO<sub>2</sub>, with both samples showing rapid carbonation in the form of magnesite. Furthermore, the fluid sampled shows a high recovery of nickel, a designated critical mineral. These experimental findings were then implemented in a technoeconomic analysis to assess the viability of field-scale implementation of this technology in the Pacific Northwest and beyond.</p>\",\"PeriodicalId\":100015,\"journal\":{\"name\":\"ACS Sustainable Resource Management\",\"volume\":\"2 5\",\"pages\":\"775–785 775–785\"},\"PeriodicalIF\":0.0000,\"publicationDate\":\"2025-04-30\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"ACS Sustainable Resource Management\",\"FirstCategoryId\":\"1085\",\"ListUrlMain\":\"https://pubs.acs.org/doi/10.1021/acssusresmgt.4c00541\",\"RegionNum\":0,\"RegionCategory\":null,\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"\",\"JCRName\":\"\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"ACS Sustainable Resource Management","FirstCategoryId":"1085","ListUrlMain":"https://pubs.acs.org/doi/10.1021/acssusresmgt.4c00541","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"","JCRName":"","Score":null,"Total":0}
Technoeconomic Potential for Carbon Mineralization with Enhanced Recovery of Critical Minerals in the Pacific Northwest
Commitments to limit the effects of global climate change require the implementation of renewable energy, along with a significant reduction of CO2 emissions. To facilitate this transition, the active removal of atmospheric CO2 by the development and deployment of new carbon management infrastructure and technologies is needed. Additionally, the world is projected to require an unprecedented amount of critical minerals, yet current high-grade ore supplies and existing mining technologies are unable to meet this demand. This study analyzes the feasibility of a novel CO2 mineralization and enhanced mineral recovery (CO2-EMR) technology designed to target low-grade, historically uneconomical resources for in situ mining. The Josephine Ophiolite in Northern California and Twin Sisters Dunite in Northwest Washington are promising ultramafic reservoirs for implementing this new mining technology. Ultramafic, olivine-rich rocks from these two sites were characterized pre- and postreaction with CO2, with both samples showing rapid carbonation in the form of magnesite. Furthermore, the fluid sampled shows a high recovery of nickel, a designated critical mineral. These experimental findings were then implemented in a technoeconomic analysis to assess the viability of field-scale implementation of this technology in the Pacific Northwest and beyond.