碱性CO2捕集溶剂电化学再生的集成建模方法

IF 3.9 3区 工程技术 Q2 ENGINEERING, CHEMICAL
Fariborz Shaahmadi, Katia Piscina, Sotirios Efstathios Antonoudis, Qingdian Shu, Sara Vallejo Castaño, Grigorios Itskos, Konstantinos Atsonios, Susana Garcia and Mijndert van der Spek*, 
{"title":"碱性CO2捕集溶剂电化学再生的集成建模方法","authors":"Fariborz Shaahmadi,&nbsp;Katia Piscina,&nbsp;Sotirios Efstathios Antonoudis,&nbsp;Qingdian Shu,&nbsp;Sara Vallejo Castaño,&nbsp;Grigorios Itskos,&nbsp;Konstantinos Atsonios,&nbsp;Susana Garcia and Mijndert van der Spek*,&nbsp;","doi":"10.1021/acs.iecr.5c0049710.1021/acs.iecr.5c00497","DOIUrl":null,"url":null,"abstract":"<p >This work introduces a model for electrochemical CO<sub>2</sub> capture and solvent regeneration integrated with an Aspen Plus flowsheet. The model is built in Aspen Custom Modeler and designed to seamlessly integrate with ASPEN Plus software, allowing for comprehensive simulation of the CO<sub>2</sub> capture process using an electrochemical cell to regenerate the solvent. The model includes detailed descriptions of the mass and energy balances in the electrochemical stack compartments, mass transport over the ion exchange membrane, and potential losses through the stack. The validity of the model was assessed against laboratory measurements. The model was exemplified by modeling a CO<sub>2</sub> capture pilot plant for three different flue gases, from cement, magnesite, and gas-fired CHP production. The results of the integrated absorber-electrochemical system reveal key trade-offs among CO<sub>2</sub> capture efficiency, energy consumption, and throughput, highlighting the performance differences across the three case studies.</p>","PeriodicalId":39,"journal":{"name":"Industrial & Engineering Chemistry Research","volume":"64 20","pages":"10253–10265 10253–10265"},"PeriodicalIF":3.9000,"publicationDate":"2025-05-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/epdf/10.1021/acs.iecr.5c00497","citationCount":"0","resultStr":"{\"title\":\"Integrated Modeling Approach for Electrochemical Regeneration of Alkaline CO2 Capture Solvents\",\"authors\":\"Fariborz Shaahmadi,&nbsp;Katia Piscina,&nbsp;Sotirios Efstathios Antonoudis,&nbsp;Qingdian Shu,&nbsp;Sara Vallejo Castaño,&nbsp;Grigorios Itskos,&nbsp;Konstantinos Atsonios,&nbsp;Susana Garcia and Mijndert van der Spek*,&nbsp;\",\"doi\":\"10.1021/acs.iecr.5c0049710.1021/acs.iecr.5c00497\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p >This work introduces a model for electrochemical CO<sub>2</sub> capture and solvent regeneration integrated with an Aspen Plus flowsheet. The model is built in Aspen Custom Modeler and designed to seamlessly integrate with ASPEN Plus software, allowing for comprehensive simulation of the CO<sub>2</sub> capture process using an electrochemical cell to regenerate the solvent. The model includes detailed descriptions of the mass and energy balances in the electrochemical stack compartments, mass transport over the ion exchange membrane, and potential losses through the stack. The validity of the model was assessed against laboratory measurements. The model was exemplified by modeling a CO<sub>2</sub> capture pilot plant for three different flue gases, from cement, magnesite, and gas-fired CHP production. The results of the integrated absorber-electrochemical system reveal key trade-offs among CO<sub>2</sub> capture efficiency, energy consumption, and throughput, highlighting the performance differences across the three case studies.</p>\",\"PeriodicalId\":39,\"journal\":{\"name\":\"Industrial & Engineering Chemistry Research\",\"volume\":\"64 20\",\"pages\":\"10253–10265 10253–10265\"},\"PeriodicalIF\":3.9000,\"publicationDate\":\"2025-05-08\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"https://pubs.acs.org/doi/epdf/10.1021/acs.iecr.5c00497\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Industrial & Engineering Chemistry Research\",\"FirstCategoryId\":\"5\",\"ListUrlMain\":\"https://pubs.acs.org/doi/10.1021/acs.iecr.5c00497\",\"RegionNum\":3,\"RegionCategory\":\"工程技术\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"ENGINEERING, CHEMICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Industrial & Engineering Chemistry Research","FirstCategoryId":"5","ListUrlMain":"https://pubs.acs.org/doi/10.1021/acs.iecr.5c00497","RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"ENGINEERING, CHEMICAL","Score":null,"Total":0}
引用次数: 0

摘要

这项工作介绍了一个模型的电化学二氧化碳捕获和溶剂再生集成的Aspen Plus流程。该模型内置在Aspen Custom Modeler中,可与Aspen Plus软件无缝集成,允许使用电化学电池再生溶剂对CO2捕获过程进行全面模拟。该模型包括对电化学堆室中质量和能量平衡的详细描述,离子交换膜上的质量传递以及通过堆的潜在损失。模型的有效性根据实验室测量结果进行了评估。该模型通过对水泥、菱镁矿和燃气热电联产三种不同烟气的二氧化碳捕集试验工厂进行建模来验证。综合吸收-电化学系统的结果揭示了二氧化碳捕获效率、能耗和吞吐量之间的关键权衡,突出了三个案例研究的性能差异。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Integrated Modeling Approach for Electrochemical Regeneration of Alkaline CO2 Capture Solvents

This work introduces a model for electrochemical CO2 capture and solvent regeneration integrated with an Aspen Plus flowsheet. The model is built in Aspen Custom Modeler and designed to seamlessly integrate with ASPEN Plus software, allowing for comprehensive simulation of the CO2 capture process using an electrochemical cell to regenerate the solvent. The model includes detailed descriptions of the mass and energy balances in the electrochemical stack compartments, mass transport over the ion exchange membrane, and potential losses through the stack. The validity of the model was assessed against laboratory measurements. The model was exemplified by modeling a CO2 capture pilot plant for three different flue gases, from cement, magnesite, and gas-fired CHP production. The results of the integrated absorber-electrochemical system reveal key trade-offs among CO2 capture efficiency, energy consumption, and throughput, highlighting the performance differences across the three case studies.

求助全文
通过发布文献求助,成功后即可免费获取论文全文。 去求助
来源期刊
Industrial & Engineering Chemistry Research
Industrial & Engineering Chemistry Research 工程技术-工程:化工
CiteScore
7.40
自引率
7.10%
发文量
1467
审稿时长
2.8 months
期刊介绍: ndustrial & Engineering Chemistry, with variations in title and format, has been published since 1909 by the American Chemical Society. Industrial & Engineering Chemistry Research is a weekly publication that reports industrial and academic research in the broad fields of applied chemistry and chemical engineering with special focus on fundamentals, processes, and products.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
确定
请完成安全验证×
copy
已复制链接
快去分享给好友吧!
我知道了
右上角分享
点击右上角分享
0
联系我们:info@booksci.cn Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。 Copyright © 2023 布克学术 All rights reserved.
京ICP备2023020795号-1
ghs 京公网安备 11010802042870号
Book学术文献互助
Book学术文献互助群
群 号:604180095
Book学术官方微信