铜催化C1-C3气态烷烃的光诱导羰化反应

IF 14.7 1区 综合性期刊 Q1 MULTIDISCIPLINARY SCIENCES
Le-Cheng Wang, Xiao-Feng Wu
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引用次数: 0

摘要

一氧化碳(CO)的催化转化为构建含羰基分子提供了巨大的机会。其中,气态烃原料上C-H键的直接羰基化为获得工业上重要的短链羧酸衍生物提供了一种简单的方法。在这里,我们报道了甲烷、乙烷和丙烷在室温下在蓝色LED照射下的一般和温和的直接羰基化反应,从而直接形成短链羧酸衍生物。值得注意的是,乙烷的直接羰基化为生产MMA提供了一种更具成本效益的途径。通过配体到金属电荷转移(LMCT)过程释放的铜还原和氯自由基的结合促进了气态烃以温和的原子经济模式活化。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Copper-catalyzed photoinduced carbonylation of C1-C3 gaseous alkanes

Copper-catalyzed photoinduced carbonylation of C1-C3 gaseous alkanes

The catalytic conversion of carbon monoxide (CO) provides an enormous opportunity to construct carbonyl-containing molecules. Among them, the direct carbonylation of C-H bonds on gaseous hydrocarbon feedstocks provides a straightforward approach to access industrially important short-chain carboxylic acid derivatives. Here, we report a general and mild direct carbonylation of methane, ethane, and propane under blue LED irradiation at ambient temperature, enabling the direct formation of short-chain carboxylic acid derivatives. Notably, the direct carbonylation of ethane offers the potential for a more cost-efficient route to produce MMA. The combination of copper reduction and chlorine radical released via a ligand-to-metal charge transfer (LMCT) process facilitates the activation of gaseous hydrocarbon in a mild and atom-economical mode.

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来源期刊
Nature Communications
Nature Communications Biological Science Disciplines-
CiteScore
24.90
自引率
2.40%
发文量
6928
审稿时长
3.7 months
期刊介绍: Nature Communications, an open-access journal, publishes high-quality research spanning all areas of the natural sciences. Papers featured in the journal showcase significant advances relevant to specialists in each respective field. With a 2-year impact factor of 16.6 (2022) and a median time of 8 days from submission to the first editorial decision, Nature Communications is committed to rapid dissemination of research findings. As a multidisciplinary journal, it welcomes contributions from biological, health, physical, chemical, Earth, social, mathematical, applied, and engineering sciences, aiming to highlight important breakthroughs within each domain.
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