V2O5掺杂nife层状双氢氧化物:能源和环境修复的双功能催化剂

IF 2.8 3区 化学 Q2 CHEMISTRY, MULTIDISCIPLINARY
Sakarapani Sarala, Palani Karthik, Velusamy Sasikala, Natarajan Prakash, Azhagurajan Mukkannan
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引用次数: 0

摘要

为了解决可持续能源生产和环境修复的双重挑战,本研究重点研究了v2o5掺杂nife层状双氢氧化物(LDHs)的开发,用于高效的水分解和光催化降解四环素。利用水热合成法,成功制备了v2o5掺杂的NiFe-LDHs。加入V2O5的目的是通过引入额外的氧化还原活性位点,提高电子导电性,并在操作循环中稳定LDH结构来提高催化性能。采用x射线衍射、扫描电镜、x射线光电子能谱等综合表征方法对合成材料的结构和形态特性进行了分析。电化学研究证明了水分解性能的显著改善,包括降低过电位和提高析氢速率。此外,还评估了v2o5掺杂的NiFe-LDHs对四环素降解的光催化活性,显示出有效去除污染物的良好结果。这些发现强调了v2o5掺杂NiFe-LDHs作为清洁能源生产和环境净化的先进材料的潜力。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
V2O5 -doped NiFe-layered double hydroxides: bifunctional catalysts for energy and environmental remediation

Addressing the dual challenges of sustainable energy production and environmental remediation, this research focuses on the development of V2O5-doped NiFe-layered double hydroxides (LDHs) for efficient water splitting and photocatalytic degradation of tetracycline. Utilizing a hydrothermal synthesis method, V2O5-doped NiFe-LDHs were successfully fabricated. The incorporation of V2O5 aims to enhance the catalytic performance by introducing additional redox-active sites, boosting electronic conductivity, and stabilizing the LDH structure during operational cycles. Comprehensive characterization, including X-ray diffraction, scanning electron microscopy, and X-ray photoelectron spectroscopy, was employed to analyze the structural and morphological properties of the synthesized materials. Electrochemical studies demonstrated significant improvements in water splitting performance, including reduced overpotentials and enhanced hydrogen evolution rates. Additionally, the photocatalytic activity of V2O5-doped NiFe-LDHs for tetracycline degradation was evaluated, showing promising results for effective pollutant removal. These findings underscore the potential of V2O5-doped NiFe-LDHs as advanced materials for both clean energy production and environmental cleanup.

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来源期刊
CiteScore
5.70
自引率
18.20%
发文量
229
审稿时长
2.6 months
期刊介绍: Research on Chemical Intermediates publishes current research articles and concise dynamic reviews on the properties, structures and reactivities of intermediate species in all the various domains of chemistry. The journal also contains articles in related disciplines such as spectroscopy, molecular biology and biochemistry, atmospheric and environmental sciences, catalysis, photochemistry and photophysics. In addition, special issues dedicated to specific topics in the field are regularly published.
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