利用0D-2D MXene/Ag NPs复合结构实现高灵敏度宽范围应变传感

IF 5.3 2区 材料科学 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY
Jintao Zhang, Yina Yang, Ranran Wang, Jing Sun, Liangjing Shi, Yin Cheng* and Yucai Shen*, 
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引用次数: 0

摘要

可拉伸和可穿戴应变传感器在人体运动监测和健康管理方面具有巨大的潜力,但灵敏度和可拉伸性之间的相互制约仍然是一个关键的挑战。本研究提出了一种基于MXene和银纳米粒子(Ag NPs)的多维复合网络结构,以解决二维材料中由于层间堆积紧密和强相互作用力造成的应变范围有限的问题。通过在MXene的夹层中嵌入Ag NPs,可以显著扩大夹层间距,从而减弱层间力,促进有效滑移,从而协同提高传感器性能。实验结果表明,当Ag NPs掺杂量为5 wt %时,该传感器表现出优异的综合性能:在0-51.5%的应变范围内,灵敏度(测量因子,GF)超过153.28,最大可检测应变为51.5%,低检测限为0.025%,并且在5000次拉伸循环中具有鲁棒的循环稳定性。机理研究表明,银纳米粒子通过润滑作用抑制裂纹扩展,同时增加导电接触点以提高灵敏度。此外,该传感器实现了对人体生理信号(如脉搏、吞咽和关节运动)的实时监测,突出了其在可穿戴健康监测方面的潜力。这项工作为优化柔性电子器件中二维材料的性能提供了新的见解。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Achieving High-Sensitivity Wide-Range Strain Sensing with 0D-2D MXene/Ag NPs Composite Structures

Stretchable and wearable strain sensors hold significant potential in human motion monitoring and health management, yet the mutual constraints between sensitivity and stretchability remain a critical challenge. This study proposes a multidimensional composite network structure based on MXene and silver nanoparticles (Ag NPs) to address the limited strain range caused by the close interlayer stacking and strong interaction forces in two-dimensional materials. By embedding Ag NPs into the interlayers of MXene, the interlayer spacing was significantly expanded, which weakened interlayer forces and facilitated effective slippage, thereby synergistically enhancing the sensor performance. Experimental results demonstrated that with 5 wt % Ag NPs doping, the sensor exhibited exceptional comprehensive performance: a sensitivity (gauge factor, GF) exceeding 153.28 across a strain range of 0–51.5%, a maximum detectable strain of 51.5%, a low detection limit of 0.025%, and robust cyclic stability over 5000 stretching cycles. Mechanistic studies revealed that Ag NPs suppressed crack propagation through a lubricating effect while increasing conductive contact points to enhance sensitivity. Furthermore, the sensor achieved real-time monitoring of human physiological signals (e.g., pulse, swallowing, and joint movements), highlighting its potential for wearable health monitoring. This work provides novel insights into optimizing the performance of two-dimensional materials in flexible electronic devices.

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来源期刊
CiteScore
8.30
自引率
3.40%
发文量
1601
期刊介绍: ACS Applied Nano Materials is an interdisciplinary journal publishing original research covering all aspects of engineering, chemistry, physics and biology relevant to applications of nanomaterials. The journal is devoted to reports of new and original experimental and theoretical research of an applied nature that integrate knowledge in the areas of materials, engineering, physics, bioscience, and chemistry into important applications of nanomaterials.
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