{"title":"利用0D-2D MXene/Ag NPs复合结构实现高灵敏度宽范围应变传感","authors":"Jintao Zhang, Yina Yang, Ranran Wang, Jing Sun, Liangjing Shi, Yin Cheng* and Yucai Shen*, ","doi":"10.1021/acsanm.5c0143810.1021/acsanm.5c01438","DOIUrl":null,"url":null,"abstract":"<p >Stretchable and wearable strain sensors hold significant potential in human motion monitoring and health management, yet the mutual constraints between sensitivity and stretchability remain a critical challenge. This study proposes a multidimensional composite network structure based on MXene and silver nanoparticles (Ag NPs) to address the limited strain range caused by the close interlayer stacking and strong interaction forces in two-dimensional materials. By embedding Ag NPs into the interlayers of MXene, the interlayer spacing was significantly expanded, which weakened interlayer forces and facilitated effective slippage, thereby synergistically enhancing the sensor performance. Experimental results demonstrated that with 5 wt % Ag NPs doping, the sensor exhibited exceptional comprehensive performance: a sensitivity (gauge factor, GF) exceeding 153.28 across a strain range of 0–51.5%, a maximum detectable strain of 51.5%, a low detection limit of 0.025%, and robust cyclic stability over 5000 stretching cycles. Mechanistic studies revealed that Ag NPs suppressed crack propagation through a lubricating effect while increasing conductive contact points to enhance sensitivity. Furthermore, the sensor achieved real-time monitoring of human physiological signals (e.g., pulse, swallowing, and joint movements), highlighting its potential for wearable health monitoring. This work provides novel insights into optimizing the performance of two-dimensional materials in flexible electronic devices.</p>","PeriodicalId":6,"journal":{"name":"ACS Applied Nano Materials","volume":"8 19","pages":"10022–10032 10022–10032"},"PeriodicalIF":5.3000,"publicationDate":"2025-05-07","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Achieving High-Sensitivity Wide-Range Strain Sensing with 0D-2D MXene/Ag NPs Composite Structures\",\"authors\":\"Jintao Zhang, Yina Yang, Ranran Wang, Jing Sun, Liangjing Shi, Yin Cheng* and Yucai Shen*, \",\"doi\":\"10.1021/acsanm.5c0143810.1021/acsanm.5c01438\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p >Stretchable and wearable strain sensors hold significant potential in human motion monitoring and health management, yet the mutual constraints between sensitivity and stretchability remain a critical challenge. This study proposes a multidimensional composite network structure based on MXene and silver nanoparticles (Ag NPs) to address the limited strain range caused by the close interlayer stacking and strong interaction forces in two-dimensional materials. By embedding Ag NPs into the interlayers of MXene, the interlayer spacing was significantly expanded, which weakened interlayer forces and facilitated effective slippage, thereby synergistically enhancing the sensor performance. Experimental results demonstrated that with 5 wt % Ag NPs doping, the sensor exhibited exceptional comprehensive performance: a sensitivity (gauge factor, GF) exceeding 153.28 across a strain range of 0–51.5%, a maximum detectable strain of 51.5%, a low detection limit of 0.025%, and robust cyclic stability over 5000 stretching cycles. Mechanistic studies revealed that Ag NPs suppressed crack propagation through a lubricating effect while increasing conductive contact points to enhance sensitivity. Furthermore, the sensor achieved real-time monitoring of human physiological signals (e.g., pulse, swallowing, and joint movements), highlighting its potential for wearable health monitoring. This work provides novel insights into optimizing the performance of two-dimensional materials in flexible electronic devices.</p>\",\"PeriodicalId\":6,\"journal\":{\"name\":\"ACS Applied Nano Materials\",\"volume\":\"8 19\",\"pages\":\"10022–10032 10022–10032\"},\"PeriodicalIF\":5.3000,\"publicationDate\":\"2025-05-07\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"ACS Applied Nano Materials\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://pubs.acs.org/doi/10.1021/acsanm.5c01438\",\"RegionNum\":2,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"MATERIALS SCIENCE, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"ACS Applied Nano Materials","FirstCategoryId":"88","ListUrlMain":"https://pubs.acs.org/doi/10.1021/acsanm.5c01438","RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"MATERIALS SCIENCE, MULTIDISCIPLINARY","Score":null,"Total":0}
Stretchable and wearable strain sensors hold significant potential in human motion monitoring and health management, yet the mutual constraints between sensitivity and stretchability remain a critical challenge. This study proposes a multidimensional composite network structure based on MXene and silver nanoparticles (Ag NPs) to address the limited strain range caused by the close interlayer stacking and strong interaction forces in two-dimensional materials. By embedding Ag NPs into the interlayers of MXene, the interlayer spacing was significantly expanded, which weakened interlayer forces and facilitated effective slippage, thereby synergistically enhancing the sensor performance. Experimental results demonstrated that with 5 wt % Ag NPs doping, the sensor exhibited exceptional comprehensive performance: a sensitivity (gauge factor, GF) exceeding 153.28 across a strain range of 0–51.5%, a maximum detectable strain of 51.5%, a low detection limit of 0.025%, and robust cyclic stability over 5000 stretching cycles. Mechanistic studies revealed that Ag NPs suppressed crack propagation through a lubricating effect while increasing conductive contact points to enhance sensitivity. Furthermore, the sensor achieved real-time monitoring of human physiological signals (e.g., pulse, swallowing, and joint movements), highlighting its potential for wearable health monitoring. This work provides novel insights into optimizing the performance of two-dimensional materials in flexible electronic devices.
期刊介绍:
ACS Applied Nano Materials is an interdisciplinary journal publishing original research covering all aspects of engineering, chemistry, physics and biology relevant to applications of nanomaterials. The journal is devoted to reports of new and original experimental and theoretical research of an applied nature that integrate knowledge in the areas of materials, engineering, physics, bioscience, and chemistry into important applications of nanomaterials.