[不同类型湖泊DOM光谱特征及来源的季节变化]。

Q2 Environmental Science
Jing-Tian Gao, Shi-Ke Tang, Wen-Li Liu, Feng-Ping Yu, Peng Zhang, Wei-Ping Li
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引用次数: 0

摘要

为研究不同类型湖泊中溶解有机质(DOM)的时空分布特征及来源,于2023年4月和7月采集了内蒙古乌良素海、代海和南海3个湖泊的水样。采用紫外-可见光谱、三维荧光光谱、平行因子分析等方法分析了3个湖泊中DOM的光谱特征及组成。此外,还探讨了DOM对水质因子的响应。结果表明,3个湖泊中DOM含量最高的是岱海。与春季相比,乌良素海、岱海和南海夏季溶解有机碳(DOC)平均浓度分别上升了69.57%、14.68%和85.88%。五梁苏海DOC的最高浓度从春季北部地区的15.32 mg·L-1上升到夏季中部地区的25.73 mg·L-1。代海DOM浓度最高的是中部地区,春季为56.12 mg·L-1 DOC,西部地区夏季为64.12 mg·L-1 DOC。在南海,春季进水口DOM较高,夏季出水口DOM增加一倍。此外,DOM的芳香性和疏水性在五粮素海最高,在南海最低。此外,三个湖泊的腐殖质主要以黄腐酸为主。从来源上看,五粮素海DOM春季以内源为主,夏季以外源为主,代海和南海DOM以内源为主。此外,从春季到夏季,代海DOM的外源特征增强,南海DOM的内源特征增强。3个湖泊DOM与TN、TP、DO呈显著相关。五梁素海TN、TP、Chl-a和代海TN、TP、COD的增加削弱了DOM的内源特征,而南海TN、Chl-a、DO、COD的增加增强了DOM的内源特征。不同类型湖泊DOM空间分布和来源的季节变化明显受到水文条件、外部水输入、生物活动和人为影响的影响。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
[Seasonal Variation in DOM Spectral Characteristics and Sources in Different Types of Lakes].

To study the spatio-temporal distribution characteristics and sources of dissolved organic matter (DOM) in different types of lakes, water samples were collected from the Wuliangsuhai Lake, Daihai Lake, and Nanhai Lake in Inner Mongolia in April and July 2023. The spectral characteristics and composition of DOM in the three lakes were analyzed using UV-vis spectroscopy, 3D fluorescence spectroscopy, and parallel factor analysis. Additionally, the response of DOM to water quality factors was explored. The results showed that the Daihai Lake had the highest DOM content among the three lakes. Compared to that during spring, the average concentration of dissolved organic carbon (DOC) during summer in the Wuliangsuhai Lake, Daihai Lake, and Nanhai Lake increased by 69.57%, 14.68%, and 85.88%, respectively. Additionally, the highest concentration of DOC in the Wuliangsuhai Lake increased from 15.32 mg·L-1 in the northern region during spring to 25.73 mg·L-1 in the central region during summer. The highest DOM concentration in the Daihai Lake was in the central region during spring with 56.12 mg·L-1 DOC but in the western region during summer with 64.12 mg·L-1 DOC. In the Nanhai Lake, the DOM in the inlet area was higher during spring, whereas it doubled in the outlet area during summer. Moreover, DOM in the Wuliangsuhai Lake showed the highest aromaticity and hydrophobicity, but lowest values were found in the Nanhai Lake. In addition, the humus of the three lakes mainly comprised fulvic acid. As for source, DOM was mainly endogenous during spring and exogenous during summer in the Wuliangsuhai Lake, while it was endogenous in the Daihai Lake and Nanhai Lake. Furthermore, the exogenous characteristics of DOM in the Daihai Lake were enhanced, while the endogenous characteristics of DOM in the Nanhai Lake were enhanced from spring to summer. Significant correlations were observed between DOM and TN, TP, and DO in the three lakes. The increase in TN, TP, and Chl-a in the Wuliangsuhai Lake and TN, TP, and COD in the Daihai Lake weakened the endogenous characteristics of DOM, whereas the increase in TN, Chl-a, DO, and COD in the Nanhai Lake enhanced the endogenous characteristics of DOM. The seasonal variation of spatial distribution and sources of DOM in different types of lakes were markedly influenced by hydrological conditions, external water input, biological activities, and human impacts.

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来源期刊
环境科学
环境科学 Environmental Science-Environmental Science (all)
CiteScore
4.40
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0.00%
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15329
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