长江三角洲典型流域地表水中微塑料的发生、驱动因素及风险评价[j]。

Q2 Environmental Science
Run-Dong Wang, Chun Hu, Chen-Xin Huang, Huzihawu Gulizila, Li-Xin Zhang, Chen-Ye Xu
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引用次数: 0

摘要

河流和湖泊是陆地微塑料(MPs)污染向海洋迁移、转化和运输的重要渠道。大量研究调查了不同流域MPs的污染特征,但很少或没有考虑基于网络分析的空间分布驱动因素。本研究以长江三角洲的太湖、太浦江、黄浦江为研究对象。采用现场取样、体视显微镜和傅里叶变换红外光谱对微塑料进行了分析。结果显示,在所有采样点,MPs的检出率均为100%。太湖地表水MPs丰度[(7 076±1 886)n·m-3]显著高于太浦江[(4 400±2 839)n·m-3]和黄浦江[(2 800±1 315)n·m-3],空间分布差异显著。MPs的粒径主要分布在0.1 ~ 0.5 mm范围内,以透明、黑色和纤维为主。聚对苯二甲酸乙二醇酯(PET)、聚苯乙烯(PS)和聚酰胺(PA)是聚合物的主要贡献者,分别占59.5%、10.4%和8.67%。相关分析表明,MPs丰度与总氮(TN)、Co (R=0.436,P<0.05)、Cd (R=0.478,P<0.05)呈显著正相关,与Cu呈负相关(R=-0.456,P<0.05)。MPs丰度也与采样点到厂区的距离呈显著负相关(R=-0.796, P<0.001)。工业点源排放对MPs的迁移和发生起着重要作用。基于网络分析,探讨了MPs、金属元素和水质指标的共现规律。TN和PS是主要影响因子。与长三角其他研究相比,该流域地表水MPs的风险污染负荷指数为1<;PLIZONE<2,表现为轻污染特征。研究流域地表水MPs的整体生态风险较低。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
[Occurrence, Driving Factors, and Risk Assessment of Microplastics in Surface Water of Typical River Basins in the Yangtze River Delta, China].

Rivers and lakes are important channels for the migration, transformation, and transportation of microplastics (MPs) pollution from land sources into the sea. A large number of studies have investigated the pollution characteristics of MPs in different watersheds, but little to none have considered the driving factors for spatial distribution based on network analysis. In this study, Taihu Lake, Taipu River, and Huangpu River in the Yangtze River Delta were selected as the target area. Microplastics were analyzed based on field sampling, stereomicroscopy, and Fourier transform infrared spectroscopy. According to the results, MPs were 100% detected at all sampling sites. The abundance of MPs in the surface water of Taihu Lake [(7 076±1 886) n·m-3] was significantly higher than that of the Taipu River [(4 400±2 839) n·m-3] and the Huangpu River [(2 800±1 315) n·m-3], indicating a significant spatial distribution difference. The particle size of MPs was mainly distributed in the range of 0.1-0.5 mm, with transparent, black color, and fibers as the main MPs. Polyethylene terephthalate (PET), polystyrene (PS), and polyamide (PA) were the major contributors of polymers, accounting for 59.5%, 10.4%, and 8.67%, respectively. Correlation analysis showed that the MPs abundance was significantly positively correlated with total nitrogen (TN), Co (R=0.436,P<0.05), and Cd (R=0.478,P<0.05), whereas they were negatively correlated with Cu (R=-0.456,P<0.05). The MPs abundance was also significantly negatively correlated with the distance from sampling points to the factory area (R=-0.796, P<0.001). Industrial point source emissions played an important role in the migration and occurrence of MPs. The co-occurrence patterns of MPs, metal elements, and water quality index were explored based on network analysis. TN and PS were the core influencing factors. Compared with other studies in the Yangtze River Delta, the risk pollution load index of surface water MPs in the watershed was 1<PLIZONE<2, which was characterized as light pollution. The overall ecological risk of MPs in the surface water of the research basin was relatively low.

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来源期刊
环境科学
环境科学 Environmental Science-Environmental Science (all)
CiteScore
4.40
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0.00%
发文量
15329
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