{"title":"基于半导体纳米结构的表面增强拉曼散射传感器研究进展。","authors":"Sirsendu Ghosal, Sanju Nandi, P K Giri","doi":"10.1088/1361-6528/adcbaf","DOIUrl":null,"url":null,"abstract":"<p><p>Surface-enhanced Raman scattering (SERS) has become a transformative analytical tool, attracting growing interest for its wide-ranging applications. The development of SERS-active materials is now a central research area, spurring innovation in various types of SERS substrates. While noble metal-based substrates remain extensively studied, semiconductor-based, non-metal substrates are garnering attention due to their unique advantages: excellent chemical stability, high carrier mobility, biocompatibility, and precise fabrication control. However, their generally weaker enhancement effects limit their utility, underscoring the need for strategies to boost their SERS activity. Understanding the complex enhancement mechanisms in semiconductor-based SERS substrates is critical for designing next-generation materials with metal-like enhancement factors (EFs). The interplay of charge transfer, localized surface plasmon resonance, and photonic effects makes the enhancement process inherently challenging to unravel. Therefore, the search for new materials with exciting optoelectronic properties, as well as more innovative solutions to increase their SERS sensitivity, continues to grow. In this review, we explore the latest advancements in semiconductor-based SERS substrates, dissecting the complex enhancement mechanisms and various modification strategies aimed at achieving metal-like high EFs. We present a comprehensive analysis of the methods used to improve the SERS performance of semiconductor substrates and conclude with potential future directions for advancing this dynamic field.</p>","PeriodicalId":19035,"journal":{"name":"Nanotechnology","volume":"36 20","pages":""},"PeriodicalIF":2.8000,"publicationDate":"2025-04-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Recent advances in semiconductor nanostructure-based surface-enhanced Raman scattering sensors.\",\"authors\":\"Sirsendu Ghosal, Sanju Nandi, P K Giri\",\"doi\":\"10.1088/1361-6528/adcbaf\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p><p>Surface-enhanced Raman scattering (SERS) has become a transformative analytical tool, attracting growing interest for its wide-ranging applications. The development of SERS-active materials is now a central research area, spurring innovation in various types of SERS substrates. While noble metal-based substrates remain extensively studied, semiconductor-based, non-metal substrates are garnering attention due to their unique advantages: excellent chemical stability, high carrier mobility, biocompatibility, and precise fabrication control. However, their generally weaker enhancement effects limit their utility, underscoring the need for strategies to boost their SERS activity. Understanding the complex enhancement mechanisms in semiconductor-based SERS substrates is critical for designing next-generation materials with metal-like enhancement factors (EFs). The interplay of charge transfer, localized surface plasmon resonance, and photonic effects makes the enhancement process inherently challenging to unravel. Therefore, the search for new materials with exciting optoelectronic properties, as well as more innovative solutions to increase their SERS sensitivity, continues to grow. In this review, we explore the latest advancements in semiconductor-based SERS substrates, dissecting the complex enhancement mechanisms and various modification strategies aimed at achieving metal-like high EFs. We present a comprehensive analysis of the methods used to improve the SERS performance of semiconductor substrates and conclude with potential future directions for advancing this dynamic field.</p>\",\"PeriodicalId\":19035,\"journal\":{\"name\":\"Nanotechnology\",\"volume\":\"36 20\",\"pages\":\"\"},\"PeriodicalIF\":2.8000,\"publicationDate\":\"2025-04-25\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Nanotechnology\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://doi.org/10.1088/1361-6528/adcbaf\",\"RegionNum\":4,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q3\",\"JCRName\":\"MATERIALS SCIENCE, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Nanotechnology","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1088/1361-6528/adcbaf","RegionNum":4,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"MATERIALS SCIENCE, MULTIDISCIPLINARY","Score":null,"Total":0}
Recent advances in semiconductor nanostructure-based surface-enhanced Raman scattering sensors.
Surface-enhanced Raman scattering (SERS) has become a transformative analytical tool, attracting growing interest for its wide-ranging applications. The development of SERS-active materials is now a central research area, spurring innovation in various types of SERS substrates. While noble metal-based substrates remain extensively studied, semiconductor-based, non-metal substrates are garnering attention due to their unique advantages: excellent chemical stability, high carrier mobility, biocompatibility, and precise fabrication control. However, their generally weaker enhancement effects limit their utility, underscoring the need for strategies to boost their SERS activity. Understanding the complex enhancement mechanisms in semiconductor-based SERS substrates is critical for designing next-generation materials with metal-like enhancement factors (EFs). The interplay of charge transfer, localized surface plasmon resonance, and photonic effects makes the enhancement process inherently challenging to unravel. Therefore, the search for new materials with exciting optoelectronic properties, as well as more innovative solutions to increase their SERS sensitivity, continues to grow. In this review, we explore the latest advancements in semiconductor-based SERS substrates, dissecting the complex enhancement mechanisms and various modification strategies aimed at achieving metal-like high EFs. We present a comprehensive analysis of the methods used to improve the SERS performance of semiconductor substrates and conclude with potential future directions for advancing this dynamic field.
期刊介绍:
The journal aims to publish papers at the forefront of nanoscale science and technology and especially those of an interdisciplinary nature. Here, nanotechnology is taken to include the ability to individually address, control, and modify structures, materials and devices with nanometre precision, and the synthesis of such structures into systems of micro- and macroscopic dimensions such as MEMS based devices. It encompasses the understanding of the fundamental physics, chemistry, biology and technology of nanometre-scale objects and how such objects can be used in the areas of computation, sensors, nanostructured materials and nano-biotechnology.