基于近红外(NIR)光谱的混合集成水分测量方法的研制。

IF 2.7 3区 化学 Q2 CHEMISTRY, ANALYTICAL
Guoqing Mu, Fulin Zhang, Wenjing Sun, Shuai He, Jingxiang Liu and Chenyu Wang
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引用次数: 0

摘要

为了实时测量流化床干燥(FBD)过程中产品的水分含量,提出了一种基于近红外(NIR)光谱的混合集成软测量方法。该方法的训练集是利用历史上获得的光谱数据及其相应的水分含量测量数据来开发的。该数据集随后与几种广泛使用的机器学习模型集成,包括偏最小二乘(PLS),支持向量回归(SVR)和决策树(DT),并通过粒子群优化(PSO)算法进一步优化。该方法利用不同的数据视角,构建了最优的混合集成模型,保证了鲁棒性和增强的预测性能。为了确定每个基础学习的最佳参数,采用了5倍交叉验证方法。光谱知识验证表明,通过粒子群优化得到的混合积分权值符合水分特征峰,表明混合积分软测量模型能较好地反映水分的物理知识。为了验证该方法的有效性,我们进行了三组对比实验:(1)使用独立PLS、SVR和DT模型进行预测;(2)采用Bagging-integrated PLS、SVR和DT模型进行预测;(3)利用本文提出的混合综合软测量方法进行预测。实验结果表明,所提出的混合集成软测量方法与其他方法相比具有更高的预测精度,突出了其对流化床干燥过程中水分含量实时测量的有效性。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Development of a hybrid integrated moisture content measurement method based on near-infrared (NIR) spectroscopy

To measure the moisture content of the product in the fluidized bed drying (FBD) process in real time, a hybrid integrated soft measurement method based on near-infrared (NIR) spectroscopy is proposed in this paper. The training set for the proposed method is developed using historically acquired spectral data paired with their corresponding moisture content measurements. This dataset is subsequently integrated with several widely used machine learning models, including Partial Least Squares (PLS), Support Vector Regression (SVR), and Decision Trees (DT), and further optimized through the Particle Swarm Optimization (PSO) algorithm. By leveraging diverse data perspectives, the method constructs an optimal hybrid integrated model, ensuring robustness and enhanced predictive performance. To determine the optimal parameters for each base learning, a 5-fold cross-validation approach was employed. Spectral knowledge validation showed that the optimized hybrid integration weights by PSO conformed to the characteristic peaks of moisture, demonstrating that the hybrid integration soft measurement model could reflect the physical knowledge. To validate the effectiveness of the proposed method, three sets of comparative experiments were conducted: (1) predictions using standalone PLS, SVR, and DT models; (2) predictions employing Bagging-integrated PLS, SVR, and DT models; and (3) predictions utilizing the hybrid integrated soft sensing method proposed in this study. The experimental results demonstrate that the proposed hybrid integrated soft sensing method achieves superior prediction accuracy compared to the other approaches, underscoring its efficacy for real-time moisture content measurement in the fluidized bed drying process.

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来源期刊
Analytical Methods
Analytical Methods CHEMISTRY, ANALYTICAL-FOOD SCIENCE & TECHNOLOGY
CiteScore
5.10
自引率
3.20%
发文量
569
审稿时长
1.8 months
期刊介绍: Early applied demonstrations of new analytical methods with clear societal impact
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