Armanbek Nursharip , Chingis Daulbayev , Jakpar Jandosov , Joseph C. Bear , Rosa Busquets , Vassilis J. Inglezakis , Alzhan Baimenov
{"title":"可持续生物废物衍生的碳气凝胶/MXene复合材料去除水中的汞","authors":"Armanbek Nursharip , Chingis Daulbayev , Jakpar Jandosov , Joseph C. Bear , Rosa Busquets , Vassilis J. Inglezakis , Alzhan Baimenov","doi":"10.1016/j.mtsust.2025.101132","DOIUrl":null,"url":null,"abstract":"<div><div>Mercury is a major global health concern; it is widespread across all environmental media and it affects all forms of life. There is strong interest in materials that can effectively remove Hg from water. This study investigates a novel and sustainable approach for mercury removal that consist of macroporous aerogel composite derived from rice husk lignin and modified with MXene. The composite developed high specific surface area (320 m<sup>2</sup>/g) and remarkable potential for Hg<sup>2+</sup> removal. Notably, 20 wt.% MXene modification increased the maximum adsorption capacity of the bare sorbent (lignin aerogel) from (82.4 mg Hg<sup>2+</sup>/g) to 135.8 mg Hg<sup>2+</sup>/g, which surpasses commercial adsorbents. The composite effectively removed Hg<sup>2+</sup> even from tap water spiked with high metal concentrations (10 mg/L). These findings highlight the significance of lignin-MXene aerogels for real-world application in water purification and environmental remediation.</div></div>","PeriodicalId":18322,"journal":{"name":"Materials Today Sustainability","volume":"31 ","pages":"Article 101132"},"PeriodicalIF":7.1000,"publicationDate":"2025-05-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Sustainable biowaste-derived carbon aerogel/MXene composite for mercury removal from water\",\"authors\":\"Armanbek Nursharip , Chingis Daulbayev , Jakpar Jandosov , Joseph C. Bear , Rosa Busquets , Vassilis J. Inglezakis , Alzhan Baimenov\",\"doi\":\"10.1016/j.mtsust.2025.101132\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><div>Mercury is a major global health concern; it is widespread across all environmental media and it affects all forms of life. There is strong interest in materials that can effectively remove Hg from water. This study investigates a novel and sustainable approach for mercury removal that consist of macroporous aerogel composite derived from rice husk lignin and modified with MXene. The composite developed high specific surface area (320 m<sup>2</sup>/g) and remarkable potential for Hg<sup>2+</sup> removal. Notably, 20 wt.% MXene modification increased the maximum adsorption capacity of the bare sorbent (lignin aerogel) from (82.4 mg Hg<sup>2+</sup>/g) to 135.8 mg Hg<sup>2+</sup>/g, which surpasses commercial adsorbents. The composite effectively removed Hg<sup>2+</sup> even from tap water spiked with high metal concentrations (10 mg/L). These findings highlight the significance of lignin-MXene aerogels for real-world application in water purification and environmental remediation.</div></div>\",\"PeriodicalId\":18322,\"journal\":{\"name\":\"Materials Today Sustainability\",\"volume\":\"31 \",\"pages\":\"Article 101132\"},\"PeriodicalIF\":7.1000,\"publicationDate\":\"2025-05-08\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Materials Today Sustainability\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S2589234725000612\",\"RegionNum\":3,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Materials Today Sustainability","FirstCategoryId":"88","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S2589234725000612","RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY","Score":null,"Total":0}
Sustainable biowaste-derived carbon aerogel/MXene composite for mercury removal from water
Mercury is a major global health concern; it is widespread across all environmental media and it affects all forms of life. There is strong interest in materials that can effectively remove Hg from water. This study investigates a novel and sustainable approach for mercury removal that consist of macroporous aerogel composite derived from rice husk lignin and modified with MXene. The composite developed high specific surface area (320 m2/g) and remarkable potential for Hg2+ removal. Notably, 20 wt.% MXene modification increased the maximum adsorption capacity of the bare sorbent (lignin aerogel) from (82.4 mg Hg2+/g) to 135.8 mg Hg2+/g, which surpasses commercial adsorbents. The composite effectively removed Hg2+ even from tap water spiked with high metal concentrations (10 mg/L). These findings highlight the significance of lignin-MXene aerogels for real-world application in water purification and environmental remediation.
期刊介绍:
Materials Today Sustainability is a multi-disciplinary journal covering all aspects of sustainability through materials science.
With a rapidly increasing population with growing demands, materials science has emerged as a critical discipline toward protecting of the environment and ensuring the long term survival of future generations.