全生物质衍生的纳米复合薄膜

IF 9.1 1区材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY

Nano Letters Pub Date : 2025-05-01 DOI:10.1021/acs.nanolett.5c0084610.1021/acs.nanolett.5c00846

Junchao Ren, Rui Tan, Chenglei Huang, Jianlong Chen, Mengde Huang, Lu Wang, Hanwu Lei, Fang Wang* and Qingfa Zhang*,

{"title":"全生物质衍生的纳米复合薄膜","authors":"Junchao Ren, Rui Tan, Chenglei Huang, Jianlong Chen, Mengde Huang, Lu Wang, Hanwu Lei, Fang Wang* and Qingfa Zhang*, ","doi":"10.1021/acs.nanolett.5c0084610.1021/acs.nanolett.5c00846","DOIUrl":null,"url":null,"abstract":"Achieving simultaneous sustainability and property is a great challenge for current thermally managed composite films. The study proposes to prepare all-biomass derived nanocomposite films with excellent mechanical, thermal, and degradation properties by self-assembling carbon quantum dots (CQDs) and carbon nanosheets (CNSs) from cellulose nanofibers (CNFs). The results showed that the nanocomposite film with CQDs1@CNSs1/CF exhibited the best comprehensive properties with thermal conductivity of 0.817 W m–1 K–1, tensile strength of 39.60 MPa, elongation at break of 6.26%, tensile modulus of 5.34 GPa, degradation residual rate in water of 86.02%, degradation residual rate in PBS of 66.67%, and degradation residual rate in buried of 52%. The all-biomass derived nanocomposite films regarding the excellent thermal conductivity, biodegradability, and mechanical properties can be available with thermal management and excellent sustainability.","PeriodicalId":53,"journal":{"name":"Nano Letters","volume":"25 19","pages":"7810–7817 7810–7817"},"PeriodicalIF":9.1000,"publicationDate":"2025-05-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"All-Biomass Derived Nanocomposite Films\",\"authors\":\"Junchao Ren, Rui Tan, Chenglei Huang, Jianlong Chen, Mengde Huang, Lu Wang, Hanwu Lei, Fang Wang* and Qingfa Zhang*, \",\"doi\":\"10.1021/acs.nanolett.5c0084610.1021/acs.nanolett.5c00846\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"Achieving simultaneous sustainability and property is a great challenge for current thermally managed composite films. The study proposes to prepare all-biomass derived nanocomposite films with excellent mechanical, thermal, and degradation properties by self-assembling carbon quantum dots (CQDs) and carbon nanosheets (CNSs) from cellulose nanofibers (CNFs). The results showed that the nanocomposite film with CQDs1@CNSs1/CF exhibited the best comprehensive properties with thermal conductivity of 0.817 W m–1 K–1, tensile strength of 39.60 MPa, elongation at break of 6.26%, tensile modulus of 5.34 GPa, degradation residual rate in water of 86.02%, degradation residual rate in PBS of 66.67%, and degradation residual rate in buried of 52%. The all-biomass derived nanocomposite films regarding the excellent thermal conductivity, biodegradability, and mechanical properties can be available with thermal management and excellent sustainability.\",\"PeriodicalId\":53,\"journal\":{\"name\":\"Nano Letters\",\"volume\":\"25 19\",\"pages\":\"7810–7817 7810–7817\"},\"PeriodicalIF\":9.1000,\"publicationDate\":\"2025-05-01\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Nano Letters\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://pubs.acs.org/doi/10.1021/acs.nanolett.5c00846\",\"RegionNum\":1,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"CHEMISTRY, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Nano Letters","FirstCategoryId":"88","ListUrlMain":"https://pubs.acs.org/doi/10.1021/acs.nanolett.5c00846","RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}

引用次数: 0

摘要

同时实现可持续性和性能是当前热管理复合薄膜的一个巨大挑战。本研究提出利用纤维素纳米纤维（CNFs）自组装碳量子点（CQDs）和碳纳米片（CNSs），制备具有优异力学、热学和降解性能的全生物质纳米复合薄膜。结果表明：CQDs1@CNSs1/CF纳米复合膜综合性能最佳，导热系数为0.817 W m-1 K-1，抗拉强度为39.60 MPa，断裂伸长率为6.26%，拉伸模量为5.34 GPa，水中降解残余率为86.02%，PBS中降解残余率为66.67%，埋地降解残余率为52%。全生物质纳米复合膜具有优异的导热性、生物降解性和力学性能，具有良好的热管理和可持续性。

本文章由计算机程序翻译，如有差异，请以英文原文为准。

All-Biomass Derived Nanocomposite Films

查看原文本刊更多论文

All-Biomass Derived Nanocomposite Films

Achieving simultaneous sustainability and property is a great challenge for current thermally managed composite films. The study proposes to prepare all-biomass derived nanocomposite films with excellent mechanical, thermal, and degradation properties by self-assembling carbon quantum dots (CQDs) and carbon nanosheets (CNSs) from cellulose nanofibers (CNFs). The results showed that the nanocomposite film with CQDs₁@CNSs₁/CF exhibited the best comprehensive properties with thermal conductivity of 0.817 W m^–1 K^–1, tensile strength of 39.60 MPa, elongation at break of 6.26%, tensile modulus of 5.34 GPa, degradation residual rate in water of 86.02%, degradation residual rate in PBS of 66.67%, and degradation residual rate in buried of 52%. The all-biomass derived nanocomposite films regarding the excellent thermal conductivity, biodegradability, and mechanical properties can be available with thermal management and excellent sustainability.

求助全文

通过发布文献求助，成功后即可免费获取论文全文。去求助

来源期刊

Nano Letters 工程技术-材料科学：综合

CiteScore

16.80

自引率

2.80%

发文量

1182

审稿时长

1.4 months

期刊介绍： Nano Letters serves as a dynamic platform for promptly disseminating original results in fundamental, applied, and emerging research across all facets of nanoscience and nanotechnology. A pivotal criterion for inclusion within Nano Letters is the convergence of at least two different areas or disciplines, ensuring a rich interdisciplinary scope. The journal is dedicated to fostering exploration in diverse areas, including: - Experimental and theoretical findings on physical, chemical, and biological phenomena at the nanoscale - Synthesis, characterization, and processing of organic, inorganic, polymer, and hybrid nanomaterials through physical, chemical, and biological methodologies - Modeling and simulation of synthetic, assembly, and interaction processes - Realization of integrated nanostructures and nano-engineered devices exhibiting advanced performance - Applications of nanoscale materials in living and environmental systems Nano Letters is committed to advancing and showcasing groundbreaking research that intersects various domains, fostering innovation and collaboration in the ever-evolving field of nanoscience and nanotechnology.