评估德克萨斯州近海百万吨级地质二氧化碳储存过程中断层内的二氧化碳迁移

IF 4.6 1区 地球科学 Q2 ENVIRONMENTAL SCIENCES
Lluís Saló-Salgado, Josimar A. Silva, Lisa Lun, Christie M. Rogers, J. Steven Davis, Ruben Juanes
{"title":"评估德克萨斯州近海百万吨级地质二氧化碳储存过程中断层内的二氧化碳迁移","authors":"Lluís Saló-Salgado, Josimar A. Silva, Lisa Lun, Christie M. Rogers, J. Steven Davis, Ruben Juanes","doi":"10.1029/2024wr037059","DOIUrl":null,"url":null,"abstract":"Recent studies indicate that Miocene-age reservoirs offshore Texas are promising candidates for industrial-scale geologic carbon sequestration. Fault-bounded hydrocarbon traps are common, and faults may be less competent seals than the low-permeability sediments overlying the reservoirs; this means that faults may limit the amount of <span data-altimg=\"/cms/asset/b316c463-309b-41e5-872c-ae6113c7b39b/wrcr70040-math-0003.png\"></span><mjx-container ctxtmenu_counter=\"705\" ctxtmenu_oldtabindex=\"1\" jax=\"CHTML\" role=\"application\" sre-explorer- style=\"font-size: 103%; position: relative;\" tabindex=\"0\"><mjx-math aria-hidden=\"true\" location=\"graphic/wrcr70040-math-0003.png\"><mjx-semantics><mjx-mrow><mjx-msub data-semantic-children=\"0,1\" data-semantic- data-semantic-role=\"unknown\" data-semantic-speech=\"CO Subscript 2\" data-semantic-type=\"subscript\"><mjx-mtext data-semantic-annotation=\"clearspeak:unit\" data-semantic-font=\"normal\" data-semantic- data-semantic-parent=\"2\" data-semantic-role=\"unknown\" data-semantic-type=\"text\"><mjx-c></mjx-c><mjx-c></mjx-c></mjx-mtext><mjx-script style=\"vertical-align: -0.15em;\"><mjx-mn data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"normal\" data-semantic- data-semantic-parent=\"2\" data-semantic-role=\"integer\" data-semantic-type=\"number\" size=\"s\"><mjx-c></mjx-c></mjx-mn></mjx-script></mjx-msub></mjx-mrow></mjx-semantics></mjx-math><mjx-assistive-mml display=\"inline\" unselectable=\"on\"><math altimg=\"urn:x-wiley:00431397:media:wrcr70040:wrcr70040-math-0003\" display=\"inline\" location=\"graphic/wrcr70040-math-0003.png\" xmlns=\"http://www.w3.org/1998/Math/MathML\"><semantics><mrow><msub data-semantic-=\"\" data-semantic-children=\"0,1\" data-semantic-role=\"unknown\" data-semantic-speech=\"CO Subscript 2\" data-semantic-type=\"subscript\"><mtext data-semantic-=\"\" data-semantic-annotation=\"clearspeak:unit\" data-semantic-font=\"normal\" data-semantic-parent=\"2\" data-semantic-role=\"unknown\" data-semantic-type=\"text\">CO</mtext><mn data-semantic-=\"\" data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"normal\" data-semantic-parent=\"2\" data-semantic-role=\"integer\" data-semantic-type=\"number\">2</mn></msub></mrow>${\\text{CO}}_{2}$</annotation></semantics></math></mjx-assistive-mml></mjx-container> that can be permanently sequestered. Here, we conduct flow simulations of megatonne-scale <span data-altimg=\"/cms/asset/a70879a7-513a-43d4-ace2-9df2bf6a13b6/wrcr70040-math-0004.png\"></span><mjx-container ctxtmenu_counter=\"706\" ctxtmenu_oldtabindex=\"1\" jax=\"CHTML\" role=\"application\" sre-explorer- style=\"font-size: 103%; position: relative;\" tabindex=\"0\"><mjx-math aria-hidden=\"true\" location=\"graphic/wrcr70040-math-0004.png\"><mjx-semantics><mjx-mrow><mjx-msub data-semantic-children=\"0,1\" data-semantic- data-semantic-role=\"unknown\" data-semantic-speech=\"CO Subscript 2\" data-semantic-type=\"subscript\"><mjx-mtext data-semantic-annotation=\"clearspeak:unit\" data-semantic-font=\"normal\" data-semantic- data-semantic-parent=\"2\" data-semantic-role=\"unknown\" data-semantic-type=\"text\"><mjx-c></mjx-c><mjx-c></mjx-c></mjx-mtext><mjx-script style=\"vertical-align: -0.15em;\"><mjx-mn data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"normal\" data-semantic- data-semantic-parent=\"2\" data-semantic-role=\"integer\" data-semantic-type=\"number\" size=\"s\"><mjx-c></mjx-c></mjx-mn></mjx-script></mjx-msub></mjx-mrow></mjx-semantics></mjx-math><mjx-assistive-mml display=\"inline\" unselectable=\"on\"><math altimg=\"urn:x-wiley:00431397:media:wrcr70040:wrcr70040-math-0004\" display=\"inline\" location=\"graphic/wrcr70040-math-0004.png\" xmlns=\"http://www.w3.org/1998/Math/MathML\"><semantics><mrow><msub data-semantic-=\"\" data-semantic-children=\"0,1\" data-semantic-role=\"unknown\" data-semantic-speech=\"CO Subscript 2\" data-semantic-type=\"subscript\"><mtext data-semantic-=\"\" data-semantic-annotation=\"clearspeak:unit\" data-semantic-font=\"normal\" data-semantic-parent=\"2\" data-semantic-role=\"unknown\" data-semantic-type=\"text\">CO</mtext><mn data-semantic-=\"\" data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"normal\" data-semantic-parent=\"2\" data-semantic-role=\"integer\" data-semantic-type=\"number\">2</mn></msub></mrow>${\\text{CO}}_{2}$</annotation></semantics></math></mjx-assistive-mml></mjx-container> injection next to a major, reservoir-bounding growth fault, and evaluate (a) where fault sealing capacity is exceeded, and (b) where the <span data-altimg=\"/cms/asset/d56286c1-3c9b-467c-a70a-3e002e91a10d/wrcr70040-math-0005.png\"></span><mjx-container ctxtmenu_counter=\"707\" ctxtmenu_oldtabindex=\"1\" jax=\"CHTML\" role=\"application\" sre-explorer- style=\"font-size: 103%; position: relative;\" tabindex=\"0\"><mjx-math aria-hidden=\"true\" location=\"graphic/wrcr70040-math-0005.png\"><mjx-semantics><mjx-mrow><mjx-msub data-semantic-children=\"0,1\" data-semantic- data-semantic-role=\"unknown\" data-semantic-speech=\"CO Subscript 2\" data-semantic-type=\"subscript\"><mjx-mtext data-semantic-annotation=\"clearspeak:unit\" data-semantic-font=\"normal\" data-semantic- data-semantic-parent=\"2\" data-semantic-role=\"unknown\" data-semantic-type=\"text\"><mjx-c></mjx-c><mjx-c></mjx-c></mjx-mtext><mjx-script style=\"vertical-align: -0.15em;\"><mjx-mn data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"normal\" data-semantic- data-semantic-parent=\"2\" data-semantic-role=\"integer\" data-semantic-type=\"number\" size=\"s\"><mjx-c></mjx-c></mjx-mn></mjx-script></mjx-msub></mjx-mrow></mjx-semantics></mjx-math><mjx-assistive-mml display=\"inline\" unselectable=\"on\"><math altimg=\"urn:x-wiley:00431397:media:wrcr70040:wrcr70040-math-0005\" display=\"inline\" location=\"graphic/wrcr70040-math-0005.png\" xmlns=\"http://www.w3.org/1998/Math/MathML\"><semantics><mrow><msub data-semantic-=\"\" data-semantic-children=\"0,1\" data-semantic-role=\"unknown\" data-semantic-speech=\"CO Subscript 2\" data-semantic-type=\"subscript\"><mtext data-semantic-=\"\" data-semantic-annotation=\"clearspeak:unit\" data-semantic-font=\"normal\" data-semantic-parent=\"2\" data-semantic-role=\"unknown\" data-semantic-type=\"text\">CO</mtext><mn data-semantic-=\"\" data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"normal\" data-semantic-parent=\"2\" data-semantic-role=\"integer\" data-semantic-type=\"number\">2</mn></msub></mrow>${\\text{CO}}_{2}$</annotation></semantics></math></mjx-assistive-mml></mjx-container> migrates after it enters the fault zone. We use a geologic model that includes the key structural features of fault-bounded systems near-offshore Texas, and consider both homogeneous and layered top seals (TSs). To model fault petrophysics, we apply a new, general methodology for faults in normally-consolidated, relatively shallow (depth <span data-altimg=\"/cms/asset/75707b74-7d83-4eab-8375-9091e819cab4/wrcr70040-math-0006.png\"></span><mjx-container ctxtmenu_counter=\"708\" ctxtmenu_oldtabindex=\"1\" jax=\"CHTML\" role=\"application\" sre-explorer- style=\"font-size: 103%; position: relative;\" tabindex=\"0\"><mjx-math aria-hidden=\"true\" location=\"graphic/wrcr70040-math-0006.png\"><mjx-semantics><mjx-mrow data-semantic-children=\"3,4,2\" data-semantic-content=\"0,1\" data-semantic- data-semantic-role=\"unknown\" data-semantic-speech=\"less than tilde 3\" data-semantic-type=\"multirel\"><mjx-mrow data-semantic- data-semantic-parent=\"5\" data-semantic-role=\"unknown\" data-semantic-type=\"empty\"></mjx-mrow><mjx-mo data-semantic- data-semantic-operator=\"multirel\" data-semantic-parent=\"5\" data-semantic-role=\"inequality\" data-semantic-type=\"relation\" rspace=\"5\" space=\"5\"><mjx-c></mjx-c></mjx-mo><mjx-mrow data-semantic- data-semantic-parent=\"5\" data-semantic-role=\"unknown\" data-semantic-type=\"empty\"></mjx-mrow><mjx-mo data-semantic- data-semantic-operator=\"multirel\" data-semantic-parent=\"5\" data-semantic-role=\"equality\" data-semantic-type=\"relation\" rspace=\"5\" space=\"5\"><mjx-c></mjx-c></mjx-mo><mjx-mn data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"normal\" data-semantic- data-semantic-parent=\"5\" data-semantic-role=\"integer\" data-semantic-type=\"number\"><mjx-c></mjx-c></mjx-mn></mjx-mrow></mjx-semantics></mjx-math><mjx-assistive-mml display=\"inline\" unselectable=\"on\"><math altimg=\"urn:x-wiley:00431397:media:wrcr70040:wrcr70040-math-0006\" display=\"inline\" location=\"graphic/wrcr70040-math-0006.png\" xmlns=\"http://www.w3.org/1998/Math/MathML\"><semantics><mrow data-semantic-=\"\" data-semantic-children=\"3,4,2\" data-semantic-content=\"0,1\" data-semantic-role=\"unknown\" data-semantic-speech=\"less than tilde 3\" data-semantic-type=\"multirel\"><mrow data-semantic-=\"\" data-semantic-parent=\"5\" data-semantic-role=\"unknown\" data-semantic-type=\"empty\"></mrow><mo data-semantic-=\"\" data-semantic-operator=\"multirel\" data-semantic-parent=\"5\" data-semantic-role=\"inequality\" data-semantic-type=\"relation\">&lt;</mo><mrow data-semantic-=\"\" data-semantic-parent=\"5\" data-semantic-role=\"unknown\" data-semantic-type=\"empty\"></mrow><mo data-semantic-=\"\" data-semantic-operator=\"multirel\" data-semantic-parent=\"5\" data-semantic-role=\"equality\" data-semantic-type=\"relation\">∼</mo><mn data-semantic-=\"\" data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"normal\" data-semantic-parent=\"5\" data-semantic-role=\"integer\" data-semantic-type=\"number\">3</mn></mrow>${&lt; } \\sim 3$</annotation></semantics></math></mjx-assistive-mml></mjx-container> km) sequences that populates three-dimensional realizations of the fault core with sand and clay smears. We quantify uncertainty in the directional components of the fault permeability tensor and multiphase flow fault properties. We evaluate the sensitivity of fault <span data-altimg=\"/cms/asset/6c7de243-45c1-4451-ad46-8820a18e9306/wrcr70040-math-0007.png\"></span><mjx-container ctxtmenu_counter=\"709\" ctxtmenu_oldtabindex=\"1\" jax=\"CHTML\" role=\"application\" sre-explorer- style=\"font-size: 103%; position: relative;\" tabindex=\"0\"><mjx-math aria-hidden=\"true\" location=\"graphic/wrcr70040-math-0007.png\"><mjx-semantics><mjx-mrow><mjx-msub data-semantic-children=\"0,1\" data-semantic- data-semantic-role=\"unknown\" data-semantic-speech=\"CO Subscript 2\" data-semantic-type=\"subscript\"><mjx-mtext data-semantic-annotation=\"clearspeak:unit\" data-semantic-font=\"normal\" data-semantic- data-semantic-parent=\"2\" data-semantic-role=\"unknown\" data-semantic-type=\"text\"><mjx-c></mjx-c><mjx-c></mjx-c></mjx-mtext><mjx-script style=\"vertical-align: -0.15em;\"><mjx-mn data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"normal\" data-semantic- data-semantic-parent=\"2\" data-semantic-role=\"integer\" data-semantic-type=\"number\" size=\"s\"><mjx-c></mjx-c></mjx-mn></mjx-script></mjx-msub></mjx-mrow></mjx-semantics></mjx-math><mjx-assistive-mml display=\"inline\" unselectable=\"on\"><math altimg=\"urn:x-wiley:00431397:media:wrcr70040:wrcr70040-math-0007\" display=\"inline\" location=\"graphic/wrcr70040-math-0007.png\" xmlns=\"http://www.w3.org/1998/Math/MathML\"><semantics><mrow><msub data-semantic-=\"\" data-semantic-children=\"0,1\" data-semantic-role=\"unknown\" data-semantic-speech=\"CO Subscript 2\" data-semantic-type=\"subscript\"><mtext data-semantic-=\"\" data-semantic-annotation=\"clearspeak:unit\" data-semantic-font=\"normal\" data-semantic-parent=\"2\" data-semantic-role=\"unknown\" data-semantic-type=\"text\">CO</mtext><mn data-semantic-=\"\" data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"normal\" data-semantic-parent=\"2\" data-semantic-role=\"integer\" data-semantic-type=\"number\">2</mn></msub></mrow>${\\text{CO}}_{2}$</annotation></semantics></math></mjx-assistive-mml></mjx-container> migration to these properties, and show that the capillary entry pressure is exceeded in the lower portion of the fault. This leads to fault <span data-altimg=\"/cms/asset/6cda38a0-7422-4293-ae3e-7c4ac5069b80/wrcr70040-math-0008.png\"></span><mjx-container ctxtmenu_counter=\"710\" ctxtmenu_oldtabindex=\"1\" jax=\"CHTML\" role=\"application\" sre-explorer- style=\"font-size: 103%; position: relative;\" tabindex=\"0\"><mjx-math aria-hidden=\"true\" location=\"graphic/wrcr70040-math-0008.png\"><mjx-semantics><mjx-mrow><mjx-msub data-semantic-children=\"0,1\" data-semantic- data-semantic-role=\"unknown\" data-semantic-speech=\"CO Subscript 2\" data-semantic-type=\"subscript\"><mjx-mtext data-semantic-annotation=\"clearspeak:unit\" data-semantic-font=\"normal\" data-semantic- data-semantic-parent=\"2\" data-semantic-role=\"unknown\" data-semantic-type=\"text\"><mjx-c></mjx-c><mjx-c></mjx-c></mjx-mtext><mjx-script style=\"vertical-align: -0.15em;\"><mjx-mn data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"normal\" data-semantic- data-semantic-parent=\"2\" data-semantic-role=\"integer\" data-semantic-type=\"number\" size=\"s\"><mjx-c></mjx-c></mjx-mn></mjx-script></mjx-msub></mjx-mrow></mjx-semantics></mjx-math><mjx-assistive-mml display=\"inline\" unselectable=\"on\"><math altimg=\"urn:x-wiley:00431397:media:wrcr70040:wrcr70040-math-0008\" display=\"inline\" location=\"graphic/wrcr70040-math-0008.png\" xmlns=\"http://www.w3.org/1998/Math/MathML\"><semantics><mrow><msub data-semantic-=\"\" data-semantic-children=\"0,1\" data-semantic-role=\"unknown\" data-semantic-speech=\"CO Subscript 2\" data-semantic-type=\"subscript\"><mtext data-semantic-=\"\" data-semantic-annotation=\"clearspeak:unit\" data-semantic-font=\"normal\" data-semantic-parent=\"2\" data-semantic-role=\"unknown\" data-semantic-type=\"text\">CO</mtext><mn data-semantic-=\"\" data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"normal\" data-semantic-parent=\"2\" data-semantic-role=\"integer\" data-semantic-type=\"number\">2</mn></msub></mrow>${\\text{CO}}_{2}$</annotation></semantics></math></mjx-assistive-mml></mjx-container> migration being controlled by effective fault permeability. For the cases considered, the amount of <span data-altimg=\"/cms/asset/ad523f11-e4ec-4d34-8ff0-d6ece6c166e3/wrcr70040-math-0009.png\"></span><mjx-container ctxtmenu_counter=\"711\" ctxtmenu_oldtabindex=\"1\" jax=\"CHTML\" role=\"application\" sre-explorer- style=\"font-size: 103%; position: relative;\" tabindex=\"0\"><mjx-math aria-hidden=\"true\" location=\"graphic/wrcr70040-math-0009.png\"><mjx-semantics><mjx-mrow><mjx-msub data-semantic-children=\"0,1\" data-semantic- data-semantic-role=\"unknown\" data-semantic-speech=\"CO Subscript 2\" data-semantic-type=\"subscript\"><mjx-mtext data-semantic-annotation=\"clearspeak:unit\" data-semantic-font=\"normal\" data-semantic- data-semantic-parent=\"2\" data-semantic-role=\"unknown\" data-semantic-type=\"text\"><mjx-c></mjx-c><mjx-c></mjx-c></mjx-mtext><mjx-script style=\"vertical-align: -0.15em;\"><mjx-mn data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"normal\" data-semantic- data-semantic-parent=\"2\" data-semantic-role=\"integer\" data-semantic-type=\"number\" size=\"s\"><mjx-c></mjx-c></mjx-mn></mjx-script></mjx-msub></mjx-mrow></mjx-semantics></mjx-math><mjx-assistive-mml display=\"inline\" unselectable=\"on\"><math altimg=\"urn:x-wiley:00431397:media:wrcr70040:wrcr70040-math-0009\" display=\"inline\" location=\"graphic/wrcr70040-math-0009.png\" xmlns=\"http://www.w3.org/1998/Math/MathML\"><semantics><mrow><msub data-semantic-=\"\" data-semantic-children=\"0,1\" data-semantic-role=\"unknown\" data-semantic-speech=\"CO Subscript 2\" data-semantic-type=\"subscript\"><mtext data-semantic-=\"\" data-semantic-annotation=\"clearspeak:unit\" data-semantic-font=\"normal\" data-semantic-parent=\"2\" data-semantic-role=\"unknown\" data-semantic-type=\"text\">CO</mtext><mn data-semantic-=\"\" data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"normal\" data-semantic-parent=\"2\" data-semantic-role=\"integer\" data-semantic-type=\"number\">2</mn></msub></mrow>${\\text{CO}}_{2}$</annotation></semantics></math></mjx-assistive-mml></mjx-container> remaining in the injection formation after 1,000 years exceeds 93%, and <span data-altimg=\"/cms/asset/d290f1bf-4959-4c70-ba57-92b728d51b07/wrcr70040-math-0010.png\"></span><mjx-container ctxtmenu_counter=\"712\" ctxtmenu_oldtabindex=\"1\" jax=\"CHTML\" role=\"application\" sre-explorer- style=\"font-size: 103%; position: relative;\" tabindex=\"0\"><mjx-math aria-hidden=\"true\" location=\"graphic/wrcr70040-math-0010.png\"><mjx-semantics><mjx-mrow><mjx-msub data-semantic-children=\"0,1\" data-semantic- data-semantic-role=\"unknown\" data-semantic-speech=\"CO Subscript 2\" data-semantic-type=\"subscript\"><mjx-mtext data-semantic-annotation=\"clearspeak:unit\" data-semantic-font=\"normal\" data-semantic- data-semantic-parent=\"2\" data-semantic-role=\"unknown\" data-semantic-type=\"text\"><mjx-c></mjx-c><mjx-c></mjx-c></mjx-mtext><mjx-script style=\"vertical-align: -0.15em;\"><mjx-mn data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"normal\" data-semantic- data-semantic-parent=\"2\" data-semantic-role=\"integer\" data-semantic-type=\"number\" size=\"s\"><mjx-c></mjx-c></mjx-mn></mjx-script></mjx-msub></mjx-mrow></mjx-semantics></mjx-math><mjx-assistive-mml display=\"inline\" unselectable=\"on\"><math altimg=\"urn:x-wiley:00431397:media:wrcr70040:wrcr70040-math-0010\" display=\"inline\" location=\"graphic/wrcr70040-math-0010.png\" xmlns=\"http://www.w3.org/1998/Math/MathML\"><semantics><mrow><msub data-semantic-=\"\" data-semantic-children=\"0,1\" data-semantic-role=\"unknown\" data-semantic-speech=\"CO Subscript 2\" data-semantic-type=\"subscript\"><mtext data-semantic-=\"\" data-semantic-annotation=\"clearspeak:unit\" data-semantic-font=\"normal\" data-semantic-parent=\"2\" data-semantic-role=\"unknown\" data-semantic-type=\"text\">CO</mtext><mn data-semantic-=\"\" data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"normal\" data-semantic-parent=\"2\" data-semantic-role=\"integer\" data-semantic-type=\"number\">2</mn></msub></mrow>${\\text{CO}}_{2}$</annotation></semantics></math></mjx-assistive-mml></mjx-container> does not migrate to depths shallower than the TS. These results suggest that, in the Miocene section, faults partially offsetting the TS do not act as preferential <span data-altimg=\"/cms/asset/2f5c9e94-ff69-487e-9862-8858603bad35/wrcr70040-math-0011.png\"></span><mjx-container ctxtmenu_counter=\"713\" ctxtmenu_oldtabindex=\"1\" jax=\"CHTML\" role=\"application\" sre-explorer- style=\"font-size: 103%; position: relative;\" tabindex=\"0\"><mjx-math aria-hidden=\"true\" location=\"graphic/wrcr70040-math-0011.png\"><mjx-semantics><mjx-mrow><mjx-msub data-semantic-children=\"0,1\" data-semantic- data-semantic-role=\"unknown\" data-semantic-speech=\"CO Subscript 2\" data-semantic-type=\"subscript\"><mjx-mtext data-semantic-annotation=\"clearspeak:unit\" data-semantic-font=\"normal\" data-semantic- data-semantic-parent=\"2\" data-semantic-role=\"unknown\" data-semantic-type=\"text\"><mjx-c></mjx-c><mjx-c></mjx-c></mjx-mtext><mjx-script style=\"vertical-align: -0.15em;\"><mjx-mn data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"normal\" data-semantic- data-semantic-parent=\"2\" data-semantic-role=\"integer\" data-semantic-type=\"number\" size=\"s\"><mjx-c></mjx-c></mjx-mn></mjx-script></mjx-msub></mjx-mrow></mjx-semantics></mjx-math><mjx-assistive-mml display=\"inline\" unselectable=\"on\"><math altimg=\"urn:x-wiley:00431397:media:wrcr70040:wrcr70040-math-0011\" display=\"inline\" location=\"graphic/wrcr70040-math-0011.png\" xmlns=\"http://www.w3.org/1998/Math/MathML\"><semantics><mrow><msub data-semantic-=\"\" data-semantic-children=\"0,1\" data-semantic-role=\"unknown\" data-semantic-speech=\"CO Subscript 2\" data-semantic-type=\"subscript\"><mtext data-semantic-=\"\" data-semantic-annotation=\"clearspeak:unit\" data-semantic-font=\"normal\" data-semantic-parent=\"2\" data-semantic-role=\"unknown\" data-semantic-type=\"text\">CO</mtext><mn data-semantic-=\"\" data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"normal\" data-semantic-parent=\"2\" data-semantic-role=\"integer\" data-semantic-type=\"number\">2</mn></msub></mrow>${\\text{CO}}_{2}$</annotation></semantics></math></mjx-assistive-mml></mjx-container> conduits.","PeriodicalId":23799,"journal":{"name":"Water Resources Research","volume":"27 1","pages":""},"PeriodicalIF":4.6000,"publicationDate":"2025-05-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Assessing CO2 Migration Within Faults During Megatonne-Scale Geologic Carbon Dioxide Storage in Offshore Texas\",\"authors\":\"Lluís Saló-Salgado, Josimar A. Silva, Lisa Lun, Christie M. Rogers, J. Steven Davis, Ruben Juanes\",\"doi\":\"10.1029/2024wr037059\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"Recent studies indicate that Miocene-age reservoirs offshore Texas are promising candidates for industrial-scale geologic carbon sequestration. Fault-bounded hydrocarbon traps are common, and faults may be less competent seals than the low-permeability sediments overlying the reservoirs; this means that faults may limit the amount of <span data-altimg=\\\"/cms/asset/b316c463-309b-41e5-872c-ae6113c7b39b/wrcr70040-math-0003.png\\\"></span><mjx-container ctxtmenu_counter=\\\"705\\\" ctxtmenu_oldtabindex=\\\"1\\\" jax=\\\"CHTML\\\" role=\\\"application\\\" sre-explorer- style=\\\"font-size: 103%; position: relative;\\\" tabindex=\\\"0\\\"><mjx-math aria-hidden=\\\"true\\\" location=\\\"graphic/wrcr70040-math-0003.png\\\"><mjx-semantics><mjx-mrow><mjx-msub data-semantic-children=\\\"0,1\\\" data-semantic- data-semantic-role=\\\"unknown\\\" data-semantic-speech=\\\"CO Subscript 2\\\" data-semantic-type=\\\"subscript\\\"><mjx-mtext data-semantic-annotation=\\\"clearspeak:unit\\\" data-semantic-font=\\\"normal\\\" data-semantic- data-semantic-parent=\\\"2\\\" data-semantic-role=\\\"unknown\\\" data-semantic-type=\\\"text\\\"><mjx-c></mjx-c><mjx-c></mjx-c></mjx-mtext><mjx-script style=\\\"vertical-align: -0.15em;\\\"><mjx-mn data-semantic-annotation=\\\"clearspeak:simple\\\" data-semantic-font=\\\"normal\\\" data-semantic- data-semantic-parent=\\\"2\\\" data-semantic-role=\\\"integer\\\" data-semantic-type=\\\"number\\\" size=\\\"s\\\"><mjx-c></mjx-c></mjx-mn></mjx-script></mjx-msub></mjx-mrow></mjx-semantics></mjx-math><mjx-assistive-mml display=\\\"inline\\\" unselectable=\\\"on\\\"><math altimg=\\\"urn:x-wiley:00431397:media:wrcr70040:wrcr70040-math-0003\\\" display=\\\"inline\\\" location=\\\"graphic/wrcr70040-math-0003.png\\\" xmlns=\\\"http://www.w3.org/1998/Math/MathML\\\"><semantics><mrow><msub data-semantic-=\\\"\\\" data-semantic-children=\\\"0,1\\\" data-semantic-role=\\\"unknown\\\" data-semantic-speech=\\\"CO Subscript 2\\\" data-semantic-type=\\\"subscript\\\"><mtext data-semantic-=\\\"\\\" data-semantic-annotation=\\\"clearspeak:unit\\\" data-semantic-font=\\\"normal\\\" data-semantic-parent=\\\"2\\\" data-semantic-role=\\\"unknown\\\" data-semantic-type=\\\"text\\\">CO</mtext><mn data-semantic-=\\\"\\\" data-semantic-annotation=\\\"clearspeak:simple\\\" data-semantic-font=\\\"normal\\\" data-semantic-parent=\\\"2\\\" data-semantic-role=\\\"integer\\\" data-semantic-type=\\\"number\\\">2</mn></msub></mrow>${\\\\text{CO}}_{2}$</annotation></semantics></math></mjx-assistive-mml></mjx-container> that can be permanently sequestered. Here, we conduct flow simulations of megatonne-scale <span data-altimg=\\\"/cms/asset/a70879a7-513a-43d4-ace2-9df2bf6a13b6/wrcr70040-math-0004.png\\\"></span><mjx-container ctxtmenu_counter=\\\"706\\\" ctxtmenu_oldtabindex=\\\"1\\\" jax=\\\"CHTML\\\" role=\\\"application\\\" sre-explorer- style=\\\"font-size: 103%; position: relative;\\\" tabindex=\\\"0\\\"><mjx-math aria-hidden=\\\"true\\\" location=\\\"graphic/wrcr70040-math-0004.png\\\"><mjx-semantics><mjx-mrow><mjx-msub data-semantic-children=\\\"0,1\\\" data-semantic- data-semantic-role=\\\"unknown\\\" data-semantic-speech=\\\"CO Subscript 2\\\" data-semantic-type=\\\"subscript\\\"><mjx-mtext data-semantic-annotation=\\\"clearspeak:unit\\\" data-semantic-font=\\\"normal\\\" data-semantic- data-semantic-parent=\\\"2\\\" data-semantic-role=\\\"unknown\\\" data-semantic-type=\\\"text\\\"><mjx-c></mjx-c><mjx-c></mjx-c></mjx-mtext><mjx-script style=\\\"vertical-align: -0.15em;\\\"><mjx-mn data-semantic-annotation=\\\"clearspeak:simple\\\" data-semantic-font=\\\"normal\\\" data-semantic- data-semantic-parent=\\\"2\\\" data-semantic-role=\\\"integer\\\" data-semantic-type=\\\"number\\\" size=\\\"s\\\"><mjx-c></mjx-c></mjx-mn></mjx-script></mjx-msub></mjx-mrow></mjx-semantics></mjx-math><mjx-assistive-mml display=\\\"inline\\\" unselectable=\\\"on\\\"><math altimg=\\\"urn:x-wiley:00431397:media:wrcr70040:wrcr70040-math-0004\\\" display=\\\"inline\\\" location=\\\"graphic/wrcr70040-math-0004.png\\\" xmlns=\\\"http://www.w3.org/1998/Math/MathML\\\"><semantics><mrow><msub data-semantic-=\\\"\\\" data-semantic-children=\\\"0,1\\\" data-semantic-role=\\\"unknown\\\" data-semantic-speech=\\\"CO Subscript 2\\\" data-semantic-type=\\\"subscript\\\"><mtext data-semantic-=\\\"\\\" data-semantic-annotation=\\\"clearspeak:unit\\\" data-semantic-font=\\\"normal\\\" data-semantic-parent=\\\"2\\\" data-semantic-role=\\\"unknown\\\" data-semantic-type=\\\"text\\\">CO</mtext><mn data-semantic-=\\\"\\\" data-semantic-annotation=\\\"clearspeak:simple\\\" data-semantic-font=\\\"normal\\\" data-semantic-parent=\\\"2\\\" data-semantic-role=\\\"integer\\\" data-semantic-type=\\\"number\\\">2</mn></msub></mrow>${\\\\text{CO}}_{2}$</annotation></semantics></math></mjx-assistive-mml></mjx-container> injection next to a major, reservoir-bounding growth fault, and evaluate (a) where fault sealing capacity is exceeded, and (b) where the <span data-altimg=\\\"/cms/asset/d56286c1-3c9b-467c-a70a-3e002e91a10d/wrcr70040-math-0005.png\\\"></span><mjx-container ctxtmenu_counter=\\\"707\\\" ctxtmenu_oldtabindex=\\\"1\\\" jax=\\\"CHTML\\\" role=\\\"application\\\" sre-explorer- style=\\\"font-size: 103%; position: relative;\\\" tabindex=\\\"0\\\"><mjx-math aria-hidden=\\\"true\\\" location=\\\"graphic/wrcr70040-math-0005.png\\\"><mjx-semantics><mjx-mrow><mjx-msub data-semantic-children=\\\"0,1\\\" data-semantic- data-semantic-role=\\\"unknown\\\" data-semantic-speech=\\\"CO Subscript 2\\\" data-semantic-type=\\\"subscript\\\"><mjx-mtext data-semantic-annotation=\\\"clearspeak:unit\\\" data-semantic-font=\\\"normal\\\" data-semantic- data-semantic-parent=\\\"2\\\" data-semantic-role=\\\"unknown\\\" data-semantic-type=\\\"text\\\"><mjx-c></mjx-c><mjx-c></mjx-c></mjx-mtext><mjx-script style=\\\"vertical-align: -0.15em;\\\"><mjx-mn data-semantic-annotation=\\\"clearspeak:simple\\\" data-semantic-font=\\\"normal\\\" data-semantic- data-semantic-parent=\\\"2\\\" data-semantic-role=\\\"integer\\\" data-semantic-type=\\\"number\\\" size=\\\"s\\\"><mjx-c></mjx-c></mjx-mn></mjx-script></mjx-msub></mjx-mrow></mjx-semantics></mjx-math><mjx-assistive-mml display=\\\"inline\\\" unselectable=\\\"on\\\"><math altimg=\\\"urn:x-wiley:00431397:media:wrcr70040:wrcr70040-math-0005\\\" display=\\\"inline\\\" location=\\\"graphic/wrcr70040-math-0005.png\\\" xmlns=\\\"http://www.w3.org/1998/Math/MathML\\\"><semantics><mrow><msub data-semantic-=\\\"\\\" data-semantic-children=\\\"0,1\\\" data-semantic-role=\\\"unknown\\\" data-semantic-speech=\\\"CO Subscript 2\\\" data-semantic-type=\\\"subscript\\\"><mtext data-semantic-=\\\"\\\" data-semantic-annotation=\\\"clearspeak:unit\\\" data-semantic-font=\\\"normal\\\" data-semantic-parent=\\\"2\\\" data-semantic-role=\\\"unknown\\\" data-semantic-type=\\\"text\\\">CO</mtext><mn data-semantic-=\\\"\\\" data-semantic-annotation=\\\"clearspeak:simple\\\" data-semantic-font=\\\"normal\\\" data-semantic-parent=\\\"2\\\" data-semantic-role=\\\"integer\\\" data-semantic-type=\\\"number\\\">2</mn></msub></mrow>${\\\\text{CO}}_{2}$</annotation></semantics></math></mjx-assistive-mml></mjx-container> migrates after it enters the fault zone. We use a geologic model that includes the key structural features of fault-bounded systems near-offshore Texas, and consider both homogeneous and layered top seals (TSs). To model fault petrophysics, we apply a new, general methodology for faults in normally-consolidated, relatively shallow (depth <span data-altimg=\\\"/cms/asset/75707b74-7d83-4eab-8375-9091e819cab4/wrcr70040-math-0006.png\\\"></span><mjx-container ctxtmenu_counter=\\\"708\\\" ctxtmenu_oldtabindex=\\\"1\\\" jax=\\\"CHTML\\\" role=\\\"application\\\" sre-explorer- style=\\\"font-size: 103%; position: relative;\\\" tabindex=\\\"0\\\"><mjx-math aria-hidden=\\\"true\\\" location=\\\"graphic/wrcr70040-math-0006.png\\\"><mjx-semantics><mjx-mrow data-semantic-children=\\\"3,4,2\\\" data-semantic-content=\\\"0,1\\\" data-semantic- data-semantic-role=\\\"unknown\\\" data-semantic-speech=\\\"less than tilde 3\\\" data-semantic-type=\\\"multirel\\\"><mjx-mrow data-semantic- data-semantic-parent=\\\"5\\\" data-semantic-role=\\\"unknown\\\" data-semantic-type=\\\"empty\\\"></mjx-mrow><mjx-mo data-semantic- data-semantic-operator=\\\"multirel\\\" data-semantic-parent=\\\"5\\\" data-semantic-role=\\\"inequality\\\" data-semantic-type=\\\"relation\\\" rspace=\\\"5\\\" space=\\\"5\\\"><mjx-c></mjx-c></mjx-mo><mjx-mrow data-semantic- data-semantic-parent=\\\"5\\\" data-semantic-role=\\\"unknown\\\" data-semantic-type=\\\"empty\\\"></mjx-mrow><mjx-mo data-semantic- data-semantic-operator=\\\"multirel\\\" data-semantic-parent=\\\"5\\\" data-semantic-role=\\\"equality\\\" data-semantic-type=\\\"relation\\\" rspace=\\\"5\\\" space=\\\"5\\\"><mjx-c></mjx-c></mjx-mo><mjx-mn data-semantic-annotation=\\\"clearspeak:simple\\\" data-semantic-font=\\\"normal\\\" data-semantic- data-semantic-parent=\\\"5\\\" data-semantic-role=\\\"integer\\\" data-semantic-type=\\\"number\\\"><mjx-c></mjx-c></mjx-mn></mjx-mrow></mjx-semantics></mjx-math><mjx-assistive-mml display=\\\"inline\\\" unselectable=\\\"on\\\"><math altimg=\\\"urn:x-wiley:00431397:media:wrcr70040:wrcr70040-math-0006\\\" display=\\\"inline\\\" location=\\\"graphic/wrcr70040-math-0006.png\\\" xmlns=\\\"http://www.w3.org/1998/Math/MathML\\\"><semantics><mrow data-semantic-=\\\"\\\" data-semantic-children=\\\"3,4,2\\\" data-semantic-content=\\\"0,1\\\" data-semantic-role=\\\"unknown\\\" data-semantic-speech=\\\"less than tilde 3\\\" data-semantic-type=\\\"multirel\\\"><mrow data-semantic-=\\\"\\\" data-semantic-parent=\\\"5\\\" data-semantic-role=\\\"unknown\\\" data-semantic-type=\\\"empty\\\"></mrow><mo data-semantic-=\\\"\\\" data-semantic-operator=\\\"multirel\\\" data-semantic-parent=\\\"5\\\" data-semantic-role=\\\"inequality\\\" data-semantic-type=\\\"relation\\\">&lt;</mo><mrow data-semantic-=\\\"\\\" data-semantic-parent=\\\"5\\\" data-semantic-role=\\\"unknown\\\" data-semantic-type=\\\"empty\\\"></mrow><mo data-semantic-=\\\"\\\" data-semantic-operator=\\\"multirel\\\" data-semantic-parent=\\\"5\\\" data-semantic-role=\\\"equality\\\" data-semantic-type=\\\"relation\\\">∼</mo><mn data-semantic-=\\\"\\\" data-semantic-annotation=\\\"clearspeak:simple\\\" data-semantic-font=\\\"normal\\\" data-semantic-parent=\\\"5\\\" data-semantic-role=\\\"integer\\\" data-semantic-type=\\\"number\\\">3</mn></mrow>${&lt; } \\\\sim 3$</annotation></semantics></math></mjx-assistive-mml></mjx-container> km) sequences that populates three-dimensional realizations of the fault core with sand and clay smears. We quantify uncertainty in the directional components of the fault permeability tensor and multiphase flow fault properties. We evaluate the sensitivity of fault <span data-altimg=\\\"/cms/asset/6c7de243-45c1-4451-ad46-8820a18e9306/wrcr70040-math-0007.png\\\"></span><mjx-container ctxtmenu_counter=\\\"709\\\" ctxtmenu_oldtabindex=\\\"1\\\" jax=\\\"CHTML\\\" role=\\\"application\\\" sre-explorer- style=\\\"font-size: 103%; position: relative;\\\" tabindex=\\\"0\\\"><mjx-math aria-hidden=\\\"true\\\" location=\\\"graphic/wrcr70040-math-0007.png\\\"><mjx-semantics><mjx-mrow><mjx-msub data-semantic-children=\\\"0,1\\\" data-semantic- data-semantic-role=\\\"unknown\\\" data-semantic-speech=\\\"CO Subscript 2\\\" data-semantic-type=\\\"subscript\\\"><mjx-mtext data-semantic-annotation=\\\"clearspeak:unit\\\" data-semantic-font=\\\"normal\\\" data-semantic- data-semantic-parent=\\\"2\\\" data-semantic-role=\\\"unknown\\\" data-semantic-type=\\\"text\\\"><mjx-c></mjx-c><mjx-c></mjx-c></mjx-mtext><mjx-script style=\\\"vertical-align: -0.15em;\\\"><mjx-mn data-semantic-annotation=\\\"clearspeak:simple\\\" data-semantic-font=\\\"normal\\\" data-semantic- data-semantic-parent=\\\"2\\\" data-semantic-role=\\\"integer\\\" data-semantic-type=\\\"number\\\" size=\\\"s\\\"><mjx-c></mjx-c></mjx-mn></mjx-script></mjx-msub></mjx-mrow></mjx-semantics></mjx-math><mjx-assistive-mml display=\\\"inline\\\" unselectable=\\\"on\\\"><math altimg=\\\"urn:x-wiley:00431397:media:wrcr70040:wrcr70040-math-0007\\\" display=\\\"inline\\\" location=\\\"graphic/wrcr70040-math-0007.png\\\" xmlns=\\\"http://www.w3.org/1998/Math/MathML\\\"><semantics><mrow><msub data-semantic-=\\\"\\\" data-semantic-children=\\\"0,1\\\" data-semantic-role=\\\"unknown\\\" data-semantic-speech=\\\"CO Subscript 2\\\" data-semantic-type=\\\"subscript\\\"><mtext data-semantic-=\\\"\\\" data-semantic-annotation=\\\"clearspeak:unit\\\" data-semantic-font=\\\"normal\\\" data-semantic-parent=\\\"2\\\" data-semantic-role=\\\"unknown\\\" data-semantic-type=\\\"text\\\">CO</mtext><mn data-semantic-=\\\"\\\" data-semantic-annotation=\\\"clearspeak:simple\\\" data-semantic-font=\\\"normal\\\" data-semantic-parent=\\\"2\\\" data-semantic-role=\\\"integer\\\" data-semantic-type=\\\"number\\\">2</mn></msub></mrow>${\\\\text{CO}}_{2}$</annotation></semantics></math></mjx-assistive-mml></mjx-container> migration to these properties, and show that the capillary entry pressure is exceeded in the lower portion of the fault. This leads to fault <span data-altimg=\\\"/cms/asset/6cda38a0-7422-4293-ae3e-7c4ac5069b80/wrcr70040-math-0008.png\\\"></span><mjx-container ctxtmenu_counter=\\\"710\\\" ctxtmenu_oldtabindex=\\\"1\\\" jax=\\\"CHTML\\\" role=\\\"application\\\" sre-explorer- style=\\\"font-size: 103%; position: relative;\\\" tabindex=\\\"0\\\"><mjx-math aria-hidden=\\\"true\\\" location=\\\"graphic/wrcr70040-math-0008.png\\\"><mjx-semantics><mjx-mrow><mjx-msub data-semantic-children=\\\"0,1\\\" data-semantic- data-semantic-role=\\\"unknown\\\" data-semantic-speech=\\\"CO Subscript 2\\\" data-semantic-type=\\\"subscript\\\"><mjx-mtext data-semantic-annotation=\\\"clearspeak:unit\\\" data-semantic-font=\\\"normal\\\" data-semantic- data-semantic-parent=\\\"2\\\" data-semantic-role=\\\"unknown\\\" data-semantic-type=\\\"text\\\"><mjx-c></mjx-c><mjx-c></mjx-c></mjx-mtext><mjx-script style=\\\"vertical-align: -0.15em;\\\"><mjx-mn data-semantic-annotation=\\\"clearspeak:simple\\\" data-semantic-font=\\\"normal\\\" data-semantic- data-semantic-parent=\\\"2\\\" data-semantic-role=\\\"integer\\\" data-semantic-type=\\\"number\\\" size=\\\"s\\\"><mjx-c></mjx-c></mjx-mn></mjx-script></mjx-msub></mjx-mrow></mjx-semantics></mjx-math><mjx-assistive-mml display=\\\"inline\\\" unselectable=\\\"on\\\"><math altimg=\\\"urn:x-wiley:00431397:media:wrcr70040:wrcr70040-math-0008\\\" display=\\\"inline\\\" location=\\\"graphic/wrcr70040-math-0008.png\\\" xmlns=\\\"http://www.w3.org/1998/Math/MathML\\\"><semantics><mrow><msub data-semantic-=\\\"\\\" data-semantic-children=\\\"0,1\\\" data-semantic-role=\\\"unknown\\\" data-semantic-speech=\\\"CO Subscript 2\\\" data-semantic-type=\\\"subscript\\\"><mtext data-semantic-=\\\"\\\" data-semantic-annotation=\\\"clearspeak:unit\\\" data-semantic-font=\\\"normal\\\" data-semantic-parent=\\\"2\\\" data-semantic-role=\\\"unknown\\\" data-semantic-type=\\\"text\\\">CO</mtext><mn data-semantic-=\\\"\\\" data-semantic-annotation=\\\"clearspeak:simple\\\" data-semantic-font=\\\"normal\\\" data-semantic-parent=\\\"2\\\" data-semantic-role=\\\"integer\\\" data-semantic-type=\\\"number\\\">2</mn></msub></mrow>${\\\\text{CO}}_{2}$</annotation></semantics></math></mjx-assistive-mml></mjx-container> migration being controlled by effective fault permeability. For the cases considered, the amount of <span data-altimg=\\\"/cms/asset/ad523f11-e4ec-4d34-8ff0-d6ece6c166e3/wrcr70040-math-0009.png\\\"></span><mjx-container ctxtmenu_counter=\\\"711\\\" ctxtmenu_oldtabindex=\\\"1\\\" jax=\\\"CHTML\\\" role=\\\"application\\\" sre-explorer- style=\\\"font-size: 103%; position: relative;\\\" tabindex=\\\"0\\\"><mjx-math aria-hidden=\\\"true\\\" location=\\\"graphic/wrcr70040-math-0009.png\\\"><mjx-semantics><mjx-mrow><mjx-msub data-semantic-children=\\\"0,1\\\" data-semantic- data-semantic-role=\\\"unknown\\\" data-semantic-speech=\\\"CO Subscript 2\\\" data-semantic-type=\\\"subscript\\\"><mjx-mtext data-semantic-annotation=\\\"clearspeak:unit\\\" data-semantic-font=\\\"normal\\\" data-semantic- data-semantic-parent=\\\"2\\\" data-semantic-role=\\\"unknown\\\" data-semantic-type=\\\"text\\\"><mjx-c></mjx-c><mjx-c></mjx-c></mjx-mtext><mjx-script style=\\\"vertical-align: -0.15em;\\\"><mjx-mn data-semantic-annotation=\\\"clearspeak:simple\\\" data-semantic-font=\\\"normal\\\" data-semantic- data-semantic-parent=\\\"2\\\" data-semantic-role=\\\"integer\\\" data-semantic-type=\\\"number\\\" size=\\\"s\\\"><mjx-c></mjx-c></mjx-mn></mjx-script></mjx-msub></mjx-mrow></mjx-semantics></mjx-math><mjx-assistive-mml display=\\\"inline\\\" unselectable=\\\"on\\\"><math altimg=\\\"urn:x-wiley:00431397:media:wrcr70040:wrcr70040-math-0009\\\" display=\\\"inline\\\" location=\\\"graphic/wrcr70040-math-0009.png\\\" xmlns=\\\"http://www.w3.org/1998/Math/MathML\\\"><semantics><mrow><msub data-semantic-=\\\"\\\" data-semantic-children=\\\"0,1\\\" data-semantic-role=\\\"unknown\\\" data-semantic-speech=\\\"CO Subscript 2\\\" data-semantic-type=\\\"subscript\\\"><mtext data-semantic-=\\\"\\\" data-semantic-annotation=\\\"clearspeak:unit\\\" data-semantic-font=\\\"normal\\\" data-semantic-parent=\\\"2\\\" data-semantic-role=\\\"unknown\\\" data-semantic-type=\\\"text\\\">CO</mtext><mn data-semantic-=\\\"\\\" data-semantic-annotation=\\\"clearspeak:simple\\\" data-semantic-font=\\\"normal\\\" data-semantic-parent=\\\"2\\\" data-semantic-role=\\\"integer\\\" data-semantic-type=\\\"number\\\">2</mn></msub></mrow>${\\\\text{CO}}_{2}$</annotation></semantics></math></mjx-assistive-mml></mjx-container> remaining in the injection formation after 1,000 years exceeds 93%, and <span data-altimg=\\\"/cms/asset/d290f1bf-4959-4c70-ba57-92b728d51b07/wrcr70040-math-0010.png\\\"></span><mjx-container ctxtmenu_counter=\\\"712\\\" ctxtmenu_oldtabindex=\\\"1\\\" jax=\\\"CHTML\\\" role=\\\"application\\\" sre-explorer- style=\\\"font-size: 103%; position: relative;\\\" tabindex=\\\"0\\\"><mjx-math aria-hidden=\\\"true\\\" location=\\\"graphic/wrcr70040-math-0010.png\\\"><mjx-semantics><mjx-mrow><mjx-msub data-semantic-children=\\\"0,1\\\" data-semantic- data-semantic-role=\\\"unknown\\\" data-semantic-speech=\\\"CO Subscript 2\\\" data-semantic-type=\\\"subscript\\\"><mjx-mtext data-semantic-annotation=\\\"clearspeak:unit\\\" data-semantic-font=\\\"normal\\\" data-semantic- data-semantic-parent=\\\"2\\\" data-semantic-role=\\\"unknown\\\" data-semantic-type=\\\"text\\\"><mjx-c></mjx-c><mjx-c></mjx-c></mjx-mtext><mjx-script style=\\\"vertical-align: -0.15em;\\\"><mjx-mn data-semantic-annotation=\\\"clearspeak:simple\\\" data-semantic-font=\\\"normal\\\" data-semantic- data-semantic-parent=\\\"2\\\" data-semantic-role=\\\"integer\\\" data-semantic-type=\\\"number\\\" size=\\\"s\\\"><mjx-c></mjx-c></mjx-mn></mjx-script></mjx-msub></mjx-mrow></mjx-semantics></mjx-math><mjx-assistive-mml display=\\\"inline\\\" unselectable=\\\"on\\\"><math altimg=\\\"urn:x-wiley:00431397:media:wrcr70040:wrcr70040-math-0010\\\" display=\\\"inline\\\" location=\\\"graphic/wrcr70040-math-0010.png\\\" xmlns=\\\"http://www.w3.org/1998/Math/MathML\\\"><semantics><mrow><msub data-semantic-=\\\"\\\" data-semantic-children=\\\"0,1\\\" data-semantic-role=\\\"unknown\\\" data-semantic-speech=\\\"CO Subscript 2\\\" data-semantic-type=\\\"subscript\\\"><mtext data-semantic-=\\\"\\\" data-semantic-annotation=\\\"clearspeak:unit\\\" data-semantic-font=\\\"normal\\\" data-semantic-parent=\\\"2\\\" data-semantic-role=\\\"unknown\\\" data-semantic-type=\\\"text\\\">CO</mtext><mn data-semantic-=\\\"\\\" data-semantic-annotation=\\\"clearspeak:simple\\\" data-semantic-font=\\\"normal\\\" data-semantic-parent=\\\"2\\\" data-semantic-role=\\\"integer\\\" data-semantic-type=\\\"number\\\">2</mn></msub></mrow>${\\\\text{CO}}_{2}$</annotation></semantics></math></mjx-assistive-mml></mjx-container> does not migrate to depths shallower than the TS. These results suggest that, in the Miocene section, faults partially offsetting the TS do not act as preferential <span data-altimg=\\\"/cms/asset/2f5c9e94-ff69-487e-9862-8858603bad35/wrcr70040-math-0011.png\\\"></span><mjx-container ctxtmenu_counter=\\\"713\\\" ctxtmenu_oldtabindex=\\\"1\\\" jax=\\\"CHTML\\\" role=\\\"application\\\" sre-explorer- style=\\\"font-size: 103%; position: relative;\\\" tabindex=\\\"0\\\"><mjx-math aria-hidden=\\\"true\\\" location=\\\"graphic/wrcr70040-math-0011.png\\\"><mjx-semantics><mjx-mrow><mjx-msub data-semantic-children=\\\"0,1\\\" data-semantic- data-semantic-role=\\\"unknown\\\" data-semantic-speech=\\\"CO Subscript 2\\\" data-semantic-type=\\\"subscript\\\"><mjx-mtext data-semantic-annotation=\\\"clearspeak:unit\\\" data-semantic-font=\\\"normal\\\" data-semantic- data-semantic-parent=\\\"2\\\" data-semantic-role=\\\"unknown\\\" data-semantic-type=\\\"text\\\"><mjx-c></mjx-c><mjx-c></mjx-c></mjx-mtext><mjx-script style=\\\"vertical-align: -0.15em;\\\"><mjx-mn data-semantic-annotation=\\\"clearspeak:simple\\\" data-semantic-font=\\\"normal\\\" data-semantic- data-semantic-parent=\\\"2\\\" data-semantic-role=\\\"integer\\\" data-semantic-type=\\\"number\\\" size=\\\"s\\\"><mjx-c></mjx-c></mjx-mn></mjx-script></mjx-msub></mjx-mrow></mjx-semantics></mjx-math><mjx-assistive-mml display=\\\"inline\\\" unselectable=\\\"on\\\"><math altimg=\\\"urn:x-wiley:00431397:media:wrcr70040:wrcr70040-math-0011\\\" display=\\\"inline\\\" location=\\\"graphic/wrcr70040-math-0011.png\\\" xmlns=\\\"http://www.w3.org/1998/Math/MathML\\\"><semantics><mrow><msub data-semantic-=\\\"\\\" data-semantic-children=\\\"0,1\\\" data-semantic-role=\\\"unknown\\\" data-semantic-speech=\\\"CO Subscript 2\\\" data-semantic-type=\\\"subscript\\\"><mtext data-semantic-=\\\"\\\" data-semantic-annotation=\\\"clearspeak:unit\\\" data-semantic-font=\\\"normal\\\" data-semantic-parent=\\\"2\\\" data-semantic-role=\\\"unknown\\\" data-semantic-type=\\\"text\\\">CO</mtext><mn data-semantic-=\\\"\\\" data-semantic-annotation=\\\"clearspeak:simple\\\" data-semantic-font=\\\"normal\\\" data-semantic-parent=\\\"2\\\" data-semantic-role=\\\"integer\\\" data-semantic-type=\\\"number\\\">2</mn></msub></mrow>${\\\\text{CO}}_{2}$</annotation></semantics></math></mjx-assistive-mml></mjx-container> conduits.\",\"PeriodicalId\":23799,\"journal\":{\"name\":\"Water Resources Research\",\"volume\":\"27 1\",\"pages\":\"\"},\"PeriodicalIF\":4.6000,\"publicationDate\":\"2025-05-08\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Water Resources Research\",\"FirstCategoryId\":\"89\",\"ListUrlMain\":\"https://doi.org/10.1029/2024wr037059\",\"RegionNum\":1,\"RegionCategory\":\"地球科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"ENVIRONMENTAL SCIENCES\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Water Resources Research","FirstCategoryId":"89","ListUrlMain":"https://doi.org/10.1029/2024wr037059","RegionNum":1,"RegionCategory":"地球科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"ENVIRONMENTAL SCIENCES","Score":null,"Total":0}
引用次数: 0

摘要

最近的研究表明,德克萨斯州近海中新世储层是工业规模地质碳封存的有希望的候选者。断层封闭型油气圈闭较为普遍,断层封闭性不如储层上的低渗透沉积层;这意味着故障可能会限制可以永久隔离的CO2${\text{CO}}_{2}$的数量。在这里,我们对一条主要的储层边界生长断层附近的百万兆吨规模的CO2${\text{CO}}_{2}$注入进行了流动模拟,并评估了(a)断层封闭能力超出的地方,以及(b) CO2${\text{CO}}_{2}$进入断裂带后的运移情况。我们使用了一个地质模型,该模型包含了德克萨斯州近海断层边界系统的主要结构特征,并考虑了均质和层状顶部密封(TSs)。为了模拟断层岩石物理,我们对正常固结的、相对较浅的(深度<; ~ 3${<)断层应用了一种新的通用方法。{\ \sim 3$ km)层序,用砂和粘土层填充断层核心的三维实现。我们量化了断层渗透率张量方向分量和多相流断层性质的不确定性。我们评价了断层CO2${\text{CO}}_{2}$运移对这些性质的敏感性,并表明断层下部超过了毛细管进入压力。这导致断层CO2${\text{CO}}_{2}$运移受有效断层渗透率控制。在上述情况下,1000年后注入地层中CO2${\text{CO}}_{2}$的残留量超过93%,CO2${\text{CO}}_{2}$不会向比TS更浅的深度迁移,这表明在中新世剖面,部分抵消TS的断裂并不是优先的CO2${\text{CO}}_{2}$管道。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Assessing CO2 Migration Within Faults During Megatonne-Scale Geologic Carbon Dioxide Storage in Offshore Texas
Recent studies indicate that Miocene-age reservoirs offshore Texas are promising candidates for industrial-scale geologic carbon sequestration. Fault-bounded hydrocarbon traps are common, and faults may be less competent seals than the low-permeability sediments overlying the reservoirs; this means that faults may limit the amount of CO2${\text{CO}}_{2}$ that can be permanently sequestered. Here, we conduct flow simulations of megatonne-scale CO2${\text{CO}}_{2}$ injection next to a major, reservoir-bounding growth fault, and evaluate (a) where fault sealing capacity is exceeded, and (b) where the CO2${\text{CO}}_{2}$ migrates after it enters the fault zone. We use a geologic model that includes the key structural features of fault-bounded systems near-offshore Texas, and consider both homogeneous and layered top seals (TSs). To model fault petrophysics, we apply a new, general methodology for faults in normally-consolidated, relatively shallow (depth <3${< } \sim 3$ km) sequences that populates three-dimensional realizations of the fault core with sand and clay smears. We quantify uncertainty in the directional components of the fault permeability tensor and multiphase flow fault properties. We evaluate the sensitivity of fault CO2${\text{CO}}_{2}$ migration to these properties, and show that the capillary entry pressure is exceeded in the lower portion of the fault. This leads to fault CO2${\text{CO}}_{2}$ migration being controlled by effective fault permeability. For the cases considered, the amount of CO2${\text{CO}}_{2}$ remaining in the injection formation after 1,000 years exceeds 93%, and CO2${\text{CO}}_{2}$ does not migrate to depths shallower than the TS. These results suggest that, in the Miocene section, faults partially offsetting the TS do not act as preferential CO2${\text{CO}}_{2}$ conduits.
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来源期刊
Water Resources Research
Water Resources Research 环境科学-湖沼学
CiteScore
8.80
自引率
13.00%
发文量
599
审稿时长
3.5 months
期刊介绍: Water Resources Research (WRR) is an interdisciplinary journal that focuses on hydrology and water resources. It publishes original research in the natural and social sciences of water. It emphasizes the role of water in the Earth system, including physical, chemical, biological, and ecological processes in water resources research and management, including social, policy, and public health implications. It encompasses observational, experimental, theoretical, analytical, numerical, and data-driven approaches that advance the science of water and its management. Submissions are evaluated for their novelty, accuracy, significance, and broader implications of the findings.
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