煤微孔网络对气液两相输运的影响

IF 5.3 3区 工程技术 Q2 ENERGY & FUELS
Wei Zha, Baiquan Lin*, Tong Liu, Ting Liu, Wei Yang and Wenyuan Wang, 
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引用次数: 0

摘要

为分析煤微孔对气水两相输运的影响,采用聚焦离子束扫描电镜(FIB-SEM)对660幅煤微表面图像进行扫描,并通过灰度值二值化分割技术对煤微孔进行三维建模。计算并统计分析微观结构特征,包括微孔连通性。结果表明,煤微孔结构呈网络状分布,100 ~ 500 nm是流体保持和运移的主要区域。随后,利用注水气驱-三轴原位LF-NMR实验平台,对不同注水时间下煤的低场核磁共振(LF-NMR) T2谱进行了检测,评估了时间对煤多尺度孔隙结构中气、水输运的影响,并评估了微孔连通性对气液两相输运过程的影响。结果表明,连通性增强的微孔结构容易因水堵塞和优势通道而形成气相停滞区;这种停滞气体逐渐溶解到水中,导致气液界面在规定的时间尺度内向停滞区前进。通过分子动力学建立了多孔煤基质模型,验证了这种气体保留过程,并说明了连通孔隙中气液相输运的差异。这些发现为理解煤多尺度孔隙中气相和水相输运提供了微观基础,可能有助于优化煤层注水和驱气策略。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Influence of Coal Micropore Network on Gas–Liquid Two-Phase Transport

Influence of Coal Micropore Network on Gas–Liquid Two-Phase Transport

To analyze the influence of coal micropores on gas–water two-phase transport, 660 coal microsurface images were scanned using focused ion beam-scanning electron microscopy (FIB-SEM), followed by three-dimensional (3D) modeling of coal micropores through the gray-value binarization segmentation technique. Microstructural characteristics, including micropore connectivity, were computed and statistically analyzed. Findings indicate that the coal micropore structure displays a networked distribution with the 100–500 nm pore size range serving as the primary region for fluid retention and transport. Subsequently, the low-field nuclear magnetic resonance (LF-NMR) T2 spectra of coal under varying water injection times were examined using a water injection and gas drive-triaxial in situ LF-NMR experimental platform, assessing the role of time on gas and water transport in the coal multiscale pore structure and evaluating how micropore connectivity affects the gas–liquid two-phase transport process. Results reveal that microporous structures with enhanced connectivity are prone to gas-phase stagnation areas due to water blockage and dominant channels; this stagnant gas incrementally dissolves into the water, causing the gas–liquid interface to progress toward the stagnation region over a defined time scale. A porous coal matrix model was constructed via molecular dynamics, validating this gas retention process and illustrating transport differences between the gas and liquid phases in the connected pores. These findings offer a microscale foundation for understanding gas- and water-phase transportation in coal multiscale pores, potentially aiding in optimizing water injection and gas displacement strategies in coal seams.

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来源期刊
Energy & Fuels
Energy & Fuels 工程技术-工程:化工
CiteScore
9.20
自引率
13.20%
发文量
1101
审稿时长
2.1 months
期刊介绍: Energy & Fuels publishes reports of research in the technical area defined by the intersection of the disciplines of chemistry and chemical engineering and the application domain of non-nuclear energy and fuels. This includes research directed at the formation of, exploration for, and production of fossil fuels and biomass; the properties and structure or molecular composition of both raw fuels and refined products; the chemistry involved in the processing and utilization of fuels; fuel cells and their applications; and the analytical and instrumental techniques used in investigations of the foregoing areas.
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