Tao Hu , Yuxuan Zhou , Tianyi Lu , Meng Sun , Weilong Tu , Cong Zhang , Xiao Li , Zhonghua Ni
{"title":"一种具有创新多通道结构的3d打印微流体燃料电池,用于增强能量收集","authors":"Tao Hu , Yuxuan Zhou , Tianyi Lu , Meng Sun , Weilong Tu , Cong Zhang , Xiao Li , Zhonghua Ni","doi":"10.1016/j.elecom.2025.107947","DOIUrl":null,"url":null,"abstract":"<div><div>The architecture design of MFCs is pivotal for fuel transport and utilization, thus necessitating the development of straightforward and adaptable fabrication techniques. This work employs the straightforward editing and rapid prototyping capabilities of 3D printing to develop a MFC with multi-channel structural geometries that can be internally cascaded, thereby reducing the complexity of the device and enhancing its overall performance and reliability. Pt/C-modified carbon cloth was produced as an anode and characterized by microscopically studies and elemental mapping, which substantiated a uniform distribution of the catalyst loading. In an alkaline environment, a glucose‑oxygen electrolyte undergoes a redox reaction at the catalytic electrode, which is observed and recorded using an electrochemical workstation. The single-cell microfluidic fuel cell (S-MFC) exhibited a performance comparable to enzyme biofuel cells, with an open-circuit potential of 0.46 V and maximum power density of 213 μW/cm<sup>2</sup>. The anode of one cell is connected to the cathode of the other cell via a carbon film, and this connection is then repeated to form a multi-stage series microfluidic fuel cell (M-MFC). The M-MFC demonstrated a significant performance improvement of 24 %, achieving a voltage of 0.87 V and a power density of 265 μW/cm<sup>2</sup>. Finally, a printed circuit board (PCB) was designed and fabricated aimed at harvesting and boosting the voltage of cell to power conventional electronic components. The as-proposed MFC significantly advances the field of energy harvesting for portable electronic devices.</div></div>","PeriodicalId":304,"journal":{"name":"Electrochemistry Communications","volume":"177 ","pages":"Article 107947"},"PeriodicalIF":4.7000,"publicationDate":"2025-05-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"A 3D-printed microfluidic fuel cell with innovative multichannel structure for enhanced energy harvesting\",\"authors\":\"Tao Hu , Yuxuan Zhou , Tianyi Lu , Meng Sun , Weilong Tu , Cong Zhang , Xiao Li , Zhonghua Ni\",\"doi\":\"10.1016/j.elecom.2025.107947\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><div>The architecture design of MFCs is pivotal for fuel transport and utilization, thus necessitating the development of straightforward and adaptable fabrication techniques. This work employs the straightforward editing and rapid prototyping capabilities of 3D printing to develop a MFC with multi-channel structural geometries that can be internally cascaded, thereby reducing the complexity of the device and enhancing its overall performance and reliability. Pt/C-modified carbon cloth was produced as an anode and characterized by microscopically studies and elemental mapping, which substantiated a uniform distribution of the catalyst loading. In an alkaline environment, a glucose‑oxygen electrolyte undergoes a redox reaction at the catalytic electrode, which is observed and recorded using an electrochemical workstation. The single-cell microfluidic fuel cell (S-MFC) exhibited a performance comparable to enzyme biofuel cells, with an open-circuit potential of 0.46 V and maximum power density of 213 μW/cm<sup>2</sup>. The anode of one cell is connected to the cathode of the other cell via a carbon film, and this connection is then repeated to form a multi-stage series microfluidic fuel cell (M-MFC). The M-MFC demonstrated a significant performance improvement of 24 %, achieving a voltage of 0.87 V and a power density of 265 μW/cm<sup>2</sup>. Finally, a printed circuit board (PCB) was designed and fabricated aimed at harvesting and boosting the voltage of cell to power conventional electronic components. The as-proposed MFC significantly advances the field of energy harvesting for portable electronic devices.</div></div>\",\"PeriodicalId\":304,\"journal\":{\"name\":\"Electrochemistry Communications\",\"volume\":\"177 \",\"pages\":\"Article 107947\"},\"PeriodicalIF\":4.7000,\"publicationDate\":\"2025-05-02\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Electrochemistry Communications\",\"FirstCategoryId\":\"5\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S1388248125000864\",\"RegionNum\":3,\"RegionCategory\":\"工程技术\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"ELECTROCHEMISTRY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Electrochemistry Communications","FirstCategoryId":"5","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S1388248125000864","RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"ELECTROCHEMISTRY","Score":null,"Total":0}
A 3D-printed microfluidic fuel cell with innovative multichannel structure for enhanced energy harvesting
The architecture design of MFCs is pivotal for fuel transport and utilization, thus necessitating the development of straightforward and adaptable fabrication techniques. This work employs the straightforward editing and rapid prototyping capabilities of 3D printing to develop a MFC with multi-channel structural geometries that can be internally cascaded, thereby reducing the complexity of the device and enhancing its overall performance and reliability. Pt/C-modified carbon cloth was produced as an anode and characterized by microscopically studies and elemental mapping, which substantiated a uniform distribution of the catalyst loading. In an alkaline environment, a glucose‑oxygen electrolyte undergoes a redox reaction at the catalytic electrode, which is observed and recorded using an electrochemical workstation. The single-cell microfluidic fuel cell (S-MFC) exhibited a performance comparable to enzyme biofuel cells, with an open-circuit potential of 0.46 V and maximum power density of 213 μW/cm2. The anode of one cell is connected to the cathode of the other cell via a carbon film, and this connection is then repeated to form a multi-stage series microfluidic fuel cell (M-MFC). The M-MFC demonstrated a significant performance improvement of 24 %, achieving a voltage of 0.87 V and a power density of 265 μW/cm2. Finally, a printed circuit board (PCB) was designed and fabricated aimed at harvesting and boosting the voltage of cell to power conventional electronic components. The as-proposed MFC significantly advances the field of energy harvesting for portable electronic devices.
期刊介绍:
Electrochemistry Communications is an open access journal providing fast dissemination of short communications, full communications and mini reviews covering the whole field of electrochemistry which merit urgent publication. Short communications are limited to a maximum of 20,000 characters (including spaces) while full communications and mini reviews are limited to 25,000 characters (including spaces). Supplementary information is permitted for full communications and mini reviews but not for short communications. We aim to be the fastest journal in electrochemistry for these types of papers.