Fangzhou Liu, Qingquan Ma, Jiahe Zhang, Jian Wang, Dheeban Govindan, Mengqiang Zhao*, Cuiling Gao, Yang Li and Wen Zhang*,
{"title":"自清洁微波响应mxene包覆过滤系统增强空气传播病毒消毒","authors":"Fangzhou Liu, Qingquan Ma, Jiahe Zhang, Jian Wang, Dheeban Govindan, Mengqiang Zhao*, Cuiling Gao, Yang Li and Wen Zhang*, ","doi":"10.1021/acsami.5c0296910.1021/acsami.5c02969","DOIUrl":null,"url":null,"abstract":"<p >The COVID-19 pandemic has highlighted the urgent demand for advanced air disinfection technologies. Traditional air filters primarily capture large airborne particles but are ineffective against submicrometer aerosols. This study introduces a microwave-enabled catalytic air filtration system using Ti<sub>3</sub>C<sub>2</sub>T<sub><i>x</i></sub> MXene-coated polypropylene filters to enhance air disinfection. With only 0.05 mg·cm<sup>–2</sup> of MXene coating, the filter surface temperature rapidly reached 104 °C within 3 s under 125 W microwave irradiation. Such surface heating led to a significantly higher log removal value (LRV) (1.86 ± 0.47) of the MS2 bacteriophage in the synthetic bioaerosol with an initial concentration of 10<sup>5</sup> PFU·mL<sup>–1</sup>, compared to 0.24–0.38 achieved by the pristine filter or the MXene-coated filter without microwave irradiation. Additionally, the filter surface exhibited promising self-cleaning behavior, as indicated by the stable viral inactivation and removal efficiency even in high-humidity environments. This innovative air filtration technology shows promising potential for preventing airborne pathogen transmission and protecting public health across diverse environmental conditions.</p>","PeriodicalId":5,"journal":{"name":"ACS Applied Materials & Interfaces","volume":"17 18","pages":"27167–27177 27167–27177"},"PeriodicalIF":8.2000,"publicationDate":"2025-04-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Self-Cleaning Microwave-Responsive MXene-Coated Filtration System for Enhanced Airborne Virus Disinfection\",\"authors\":\"Fangzhou Liu, Qingquan Ma, Jiahe Zhang, Jian Wang, Dheeban Govindan, Mengqiang Zhao*, Cuiling Gao, Yang Li and Wen Zhang*, \",\"doi\":\"10.1021/acsami.5c0296910.1021/acsami.5c02969\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p >The COVID-19 pandemic has highlighted the urgent demand for advanced air disinfection technologies. Traditional air filters primarily capture large airborne particles but are ineffective against submicrometer aerosols. This study introduces a microwave-enabled catalytic air filtration system using Ti<sub>3</sub>C<sub>2</sub>T<sub><i>x</i></sub> MXene-coated polypropylene filters to enhance air disinfection. With only 0.05 mg·cm<sup>–2</sup> of MXene coating, the filter surface temperature rapidly reached 104 °C within 3 s under 125 W microwave irradiation. Such surface heating led to a significantly higher log removal value (LRV) (1.86 ± 0.47) of the MS2 bacteriophage in the synthetic bioaerosol with an initial concentration of 10<sup>5</sup> PFU·mL<sup>–1</sup>, compared to 0.24–0.38 achieved by the pristine filter or the MXene-coated filter without microwave irradiation. Additionally, the filter surface exhibited promising self-cleaning behavior, as indicated by the stable viral inactivation and removal efficiency even in high-humidity environments. This innovative air filtration technology shows promising potential for preventing airborne pathogen transmission and protecting public health across diverse environmental conditions.</p>\",\"PeriodicalId\":5,\"journal\":{\"name\":\"ACS Applied Materials & Interfaces\",\"volume\":\"17 18\",\"pages\":\"27167–27177 27167–27177\"},\"PeriodicalIF\":8.2000,\"publicationDate\":\"2025-04-24\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"ACS Applied Materials & Interfaces\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://pubs.acs.org/doi/10.1021/acsami.5c02969\",\"RegionNum\":2,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"MATERIALS SCIENCE, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"ACS Applied Materials & Interfaces","FirstCategoryId":"88","ListUrlMain":"https://pubs.acs.org/doi/10.1021/acsami.5c02969","RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"MATERIALS SCIENCE, MULTIDISCIPLINARY","Score":null,"Total":0}
Self-Cleaning Microwave-Responsive MXene-Coated Filtration System for Enhanced Airborne Virus Disinfection
The COVID-19 pandemic has highlighted the urgent demand for advanced air disinfection technologies. Traditional air filters primarily capture large airborne particles but are ineffective against submicrometer aerosols. This study introduces a microwave-enabled catalytic air filtration system using Ti3C2Tx MXene-coated polypropylene filters to enhance air disinfection. With only 0.05 mg·cm–2 of MXene coating, the filter surface temperature rapidly reached 104 °C within 3 s under 125 W microwave irradiation. Such surface heating led to a significantly higher log removal value (LRV) (1.86 ± 0.47) of the MS2 bacteriophage in the synthetic bioaerosol with an initial concentration of 105 PFU·mL–1, compared to 0.24–0.38 achieved by the pristine filter or the MXene-coated filter without microwave irradiation. Additionally, the filter surface exhibited promising self-cleaning behavior, as indicated by the stable viral inactivation and removal efficiency even in high-humidity environments. This innovative air filtration technology shows promising potential for preventing airborne pathogen transmission and protecting public health across diverse environmental conditions.
期刊介绍:
ACS Applied Materials & Interfaces is a leading interdisciplinary journal that brings together chemists, engineers, physicists, and biologists to explore the development and utilization of newly-discovered materials and interfacial processes for specific applications. Our journal has experienced remarkable growth since its establishment in 2009, both in terms of the number of articles published and the impact of the research showcased. We are proud to foster a truly global community, with the majority of published articles originating from outside the United States, reflecting the rapid growth of applied research worldwide.