忆阻器用无机卤化物钙钛矿量子点

IF 2.1 4区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY
Hyo Min Cho, Ho Won Jang
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引用次数: 0

摘要

忆阻器是存储器和电阻器的结合,最早被提出作为第四种基本无源电路元件。虽然卤化物钙钛矿已经成为忆阻器器件的有前途的材料,但有机-无机杂化钙钛矿面临着诸如吸湿性和热不稳定性等挑战,限制了它们的长期适用性。无机卤化物钙钛矿量子点(IHPQDs)具有增强的环境稳定性和独特的性能,包括对天然缺陷的高耐受性和离子迁移能力。本文综述了IHPQDs的最新研究进展,包括其晶体结构、合成技术和在忆阻器器件中的工作机制。与之前主要探索大块卤化物钙钛矿的研究不同,我们强调了IHPQDs在电阻开关记忆和神经形态计算中的作用,强调了它们在多电平电阻状态和低功耗工作中的潜力。此外,本综述还解决了实际挑战,包括薄膜均匀性,电荷传输层集成和无铅替代品,这些对于基于ihpqds的记忆电阻器的商业化至关重要。通过提出可行的策略和未来的研究方向,我们的目标是弥合基础研究和现实应用之间的差距,将ihpqd定位为下一代电子器件的关键材料。图形抽象
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Inorganic Halide Perovskite Quantum Dots for Memristors

Memristor, a combination of memory and resistor, was first proposed as the fourth fundamental passive circuit element. While halide perovskites have emerged as promising materials for memristor devices, organic-inorganic hybrid perovskites face challenges such as hygroscopicity and thermal instability, limiting their long-term applicability. This paper focuses on inorganic halide perovskite quantum dots (IHPQDs), which offer enhanced environmental stability and unique properties, including high tolerance to native defects and ion migration capability. This paper provides a comprehensive review of recent advancements in IHPQDs, covering their crystal structures, synthesis techniques, and operational mechanisms in memristor devices. Unlike previous studies that predominantly explored bulk halide perovskites, we emphasize the role of IHPQDs in resistive switching memory and neuromorphic computing, highlighting their potential for multilevel resistance states and low-power operation. Additionally, this review addresses practical challenges, including thin-film uniformity, charge transport layer integration, and lead-free alternatives, which are critical for the commercialization of IHPQDs-based memristors. By proposing actionable strategies and future research directions, we aim to bridge the gap between fundamental research and real-world applications, positioning IHPQDs as key materials for next-generation electronic devices.

Graphical Abstract

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来源期刊
Electronic Materials Letters
Electronic Materials Letters 工程技术-材料科学:综合
CiteScore
4.70
自引率
20.80%
发文量
52
审稿时长
2.3 months
期刊介绍: Electronic Materials Letters is an official journal of the Korean Institute of Metals and Materials. It is a peer-reviewed international journal publishing print and online version. It covers all disciplines of research and technology in electronic materials. Emphasis is placed on science, engineering and applications of advanced materials, including electronic, magnetic, optical, organic, electrochemical, mechanical, and nanoscale materials. The aspects of synthesis and processing include thin films, nanostructures, self assembly, and bulk, all related to thermodynamics, kinetics and/or modeling.
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