Yali Wang , Qinshan Liu , Wenjin Xu , Xiahui Gui , Yaowen Xing
{"title":"聚并角对气泡偏离的影响:来自动态观察和模拟的见解","authors":"Yali Wang , Qinshan Liu , Wenjin Xu , Xiahui Gui , Yaowen Xing","doi":"10.1016/j.ces.2025.121765","DOIUrl":null,"url":null,"abstract":"<div><div>This study uses a self-developed 3D coalescence-induced bubble departure visualization system and numerical simulations to explore the regulatory mechanism of coalescence angle (ω) on bubble detachment. Results show that as ω decreases (90°→20°), the three-phase contact line transitions from “bidirectional synchronous contraction − asynchronous contraction − unilateral diffusion”, enhancing contact angle hysteresis and shifting bubble motion from vertical detachment to horizontal sliding. When the surface contact angle exceeds 60°, bubble detachment is fully suppressed, and ω loses its effect. Phase diagram analysis reveals that surface hydrophobicity and coalescence angle control detachment through competing adhesion forces and flow field momentum. Large ω (≥70°) generates vertical momentum (Re = 120, We = 0.27) to drive detachment, while small ω (≤45°) causes horizontal oscillations (Re = 70, We = 0.11) and energy dissipation. A critical criterion based on the balance model of surface energy and viscous resistance work quantifies the energy thresholds for bubble detachment under different operating conditions, offering insights for optimizing industrial bubble dynamics.</div></div>","PeriodicalId":271,"journal":{"name":"Chemical Engineering Science","volume":"313 ","pages":"Article 121765"},"PeriodicalIF":4.1000,"publicationDate":"2025-04-30","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"The effect of coalescence angle on bubble departure: Insights from dynamic observations and simulations\",\"authors\":\"Yali Wang , Qinshan Liu , Wenjin Xu , Xiahui Gui , Yaowen Xing\",\"doi\":\"10.1016/j.ces.2025.121765\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><div>This study uses a self-developed 3D coalescence-induced bubble departure visualization system and numerical simulations to explore the regulatory mechanism of coalescence angle (ω) on bubble detachment. Results show that as ω decreases (90°→20°), the three-phase contact line transitions from “bidirectional synchronous contraction − asynchronous contraction − unilateral diffusion”, enhancing contact angle hysteresis and shifting bubble motion from vertical detachment to horizontal sliding. When the surface contact angle exceeds 60°, bubble detachment is fully suppressed, and ω loses its effect. Phase diagram analysis reveals that surface hydrophobicity and coalescence angle control detachment through competing adhesion forces and flow field momentum. Large ω (≥70°) generates vertical momentum (Re = 120, We = 0.27) to drive detachment, while small ω (≤45°) causes horizontal oscillations (Re = 70, We = 0.11) and energy dissipation. A critical criterion based on the balance model of surface energy and viscous resistance work quantifies the energy thresholds for bubble detachment under different operating conditions, offering insights for optimizing industrial bubble dynamics.</div></div>\",\"PeriodicalId\":271,\"journal\":{\"name\":\"Chemical Engineering Science\",\"volume\":\"313 \",\"pages\":\"Article 121765\"},\"PeriodicalIF\":4.1000,\"publicationDate\":\"2025-04-30\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Chemical Engineering Science\",\"FirstCategoryId\":\"5\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S0009250925005883\",\"RegionNum\":2,\"RegionCategory\":\"工程技术\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"ENGINEERING, CHEMICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Chemical Engineering Science","FirstCategoryId":"5","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S0009250925005883","RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"ENGINEERING, CHEMICAL","Score":null,"Total":0}
The effect of coalescence angle on bubble departure: Insights from dynamic observations and simulations
This study uses a self-developed 3D coalescence-induced bubble departure visualization system and numerical simulations to explore the regulatory mechanism of coalescence angle (ω) on bubble detachment. Results show that as ω decreases (90°→20°), the three-phase contact line transitions from “bidirectional synchronous contraction − asynchronous contraction − unilateral diffusion”, enhancing contact angle hysteresis and shifting bubble motion from vertical detachment to horizontal sliding. When the surface contact angle exceeds 60°, bubble detachment is fully suppressed, and ω loses its effect. Phase diagram analysis reveals that surface hydrophobicity and coalescence angle control detachment through competing adhesion forces and flow field momentum. Large ω (≥70°) generates vertical momentum (Re = 120, We = 0.27) to drive detachment, while small ω (≤45°) causes horizontal oscillations (Re = 70, We = 0.11) and energy dissipation. A critical criterion based on the balance model of surface energy and viscous resistance work quantifies the energy thresholds for bubble detachment under different operating conditions, offering insights for optimizing industrial bubble dynamics.
期刊介绍:
Chemical engineering enables the transformation of natural resources and energy into useful products for society. It draws on and applies natural sciences, mathematics and economics, and has developed fundamental engineering science that underpins the discipline.
Chemical Engineering Science (CES) has been publishing papers on the fundamentals of chemical engineering since 1951. CES is the platform where the most significant advances in the discipline have ever since been published. Chemical Engineering Science has accompanied and sustained chemical engineering through its development into the vibrant and broad scientific discipline it is today.